Dissipationless nonlinearities for three-wave mixing are a key component of many superconducting quantum devices, such as amplifiers and bosonic qubits. So far, such third-order nonlinearities have been primarily achieved with circuits of concatenated Josephson tunnel junctions. In this work, we theoretically develop an alternative approach to realize third-order nonlinearities from gate-tunable and intrinsically symmetry-broken quantum material Josephson junctions. We illustrate this approach on two examples, an Andreev interferometer and a magnetic Josephson junction. Our results show that both setups enable Kerr-free three-wave mixing for a broad range of frequencies, an attribute that is highly desirable for amplifier applications. Moreover, we also find that the magnetic junction constitutes a paradigmatic example for three-wave mixing in a minimal single-junction device without the need for any external biases. We hope that our work will guide the search of dissipationless nonlinearities in quantum material superconducting devices and inspire other ways of characterizing symmetry breaking in quantum materials with microwave techniques.
Dissipationless nonlinearities for three-wave mixing are a key component of many superconducting quantum devices, such as amplifiers and bosonic qubits. So far, such third-order nonlinearities have been primarily achieved with circuits of concatenated Josephson tunnel junctions. In this work, we theoretically develop an alternative approach to realize third-order nonlinearities from gate-tunable and intrinsically symmetry-broken quantum material Josephson junctions. We illustrate this approach on two examples, an Andreev interferometer and a magnetic Josephson junction. Our results show that both setups enable Kerr-free three-wave mixing for a broad range of frequencies, an attribute that is highly desirable for amplifier applications. Moreover, we also find that the magnetic junction constitutes a paradigmatic example for three-wave mixing in a minimal single-junction device without the need for any external biases. We hope that our work will guide the search of dissipationless nonlinearities in quantum material superconducting devices and inspire other ways of characterizing symmetry breaking in quantum materials with microwave techniques.
Three-wave mixing devices, i.e. non-linear circuits converting power among three microwave signals, are key elements of analog information processing in the microwave domain. However, they are based on dissipative components such as semiconductor diodes, or SIS tunnel junctions biased near the superconducting gap. The loss of signal limits their operation and also introduces noise above the minimum required by quantum mechanics. By using Josephson junctions and superconducting resonators, we've been able to build such a quantum device. In its amplification mode, this device can be used as a preamplifier in many experiments where a few photon wide microwave signals must be measured by commercial instruments, which are sensitive to powers several orders of magnitude larger. The price to pay for this amplification is the necessary degradation of information. Indeed, an extension of the no-cloning theorem imposes that a linear phase preserving amplifier adds at least half a quantum of noise to the signal. By amplifying the finite frequency noise emitted by an NIN tunnel junction, we demonstrated that the total measurement chain adds less than 2.3 quanta to this limit thanks to our device. The operating principle of this device is based on Josephson parametric amplification. I will explain this mechanism and show preliminary results which illustrate that it can generate quantum correlated pairs of spatially separated photons with different wavelengths known as two-mode squeezed states. This experiment exploits the tunability of our device and the ease-of-use inherent to micro-wave circuits to perform a quantum optics experiment demonstrating this entanglement.
Three-wave mixing devices, i.e. non-linear circuits converting power among three microwave signals, are key elements of analog information processing in the microwave domain. However, they are based on dissipative components such as semiconductor diodes, or SIS tunnel junctions biased near the superconducting gap. The loss of signal limits their operation and also introduces noise above the minimum required by quantum mechanics. By using Josephson junctions and superconducting resonators, we've been able to build such a quantum device. In its amplification mode, this device can be used as a preamplifier in many experiments where a few photon wide microwave signals must be measured by commercial instruments, which are sensitive to powers several orders of magnitude larger. The price to pay for this amplification is the necessary degradation of information. Indeed, an extension of the no-cloning theorem imposes that a linear phase preserving amplifier adds at least half a quantum of noise to the signal. By amplifying the finite frequency noise emitted by an NIN tunnel junction, we demonstrated that the total measurement chain adds less than 2.3 quanta to this limit thanks to our device. The operating principle of this device is based on Josephson parametric amplification. I will explain this mechanism and present results which illustrate that it can generate quantum correlated pairs of spatially separated photons with different wavelengths known as two-mode squeezed states. This experiment exploits the tunability of our device and the ease-of-use inherent to micro-wave circuits to perform a quantum optics experiment demonstrating this entanglement.
Josephson junction (JJ) is a key nonlinear element in superconducting devices such as qubits, amplifiers, and bolometers. Recently, gate-tunable JJs based on graphene and semiconductors have gained interest due to their rich Andreev physics and wide applications in circuit quantum electrodynamics devices. In addition to gate tunability, it offers many advantages over conventional JJs, such as exceptional thermal properties for bolometric sensors, magnetic-field compatibility, and operability at elevated temperatures above 1 K. Like conventional Al–AlOx–Al JJs, graphene JJs also act as nonlinear inductors, and at their heart lies the Kerr nonlinearity. Additionally, in graphene JJs, the nonlinearity is tunable via external knobs in a single device. However, a detailed experimental exploration of the tunable Kerr nonlinearity in graphene JJs has never been performed. In this work, we study the dependence of the Kerr nonlinearity on gate voltage, temperature, and DC bias—an interesting knob that has been less explored. Using these parameters, we show that the magnitude of the Kerr coefficient can be tuned over a wide range, from ∼200 kHz to 1.2 MHz. Our work will be a valuable resource for further understanding of the nonlinearity in graphene JJs and for the design of next-generation amplifiers and sensors, with enhanced performance.
Metamaterials are artificially designed materials to exhibit properties not available in natural materials by engineering the constituting elements at sub-wavelength scales, enabling unique interactions of matter with electromagnetic waves or coupling modes of electromagnetic waves. Examples of such novel optics phenomenons include negative index of refraction, cloaking, and super-resolution imaging. The study of superconducting metamaterials operating in the microwave frequency domain has recently generated significant interest in the framework of quantum technologies due to a wide range of direct applications, e.g., exploration of novel quantum optics phenomena, non-destructive quantum sensing, quantum-limited amplification, quantum information processing, and quantum illumination. In contrast to their normal metal and semiconducting counterparts, superconducting metamaterials offer some unique advantages. The most relevant of these for Josephson junction based metamaterials are low losses, flux quantization, and Josephson effects. The Josephson effect in a superconducting loop can also be exploited to exact more control over the nonlinearities of the meta-material.In this thesis, we present Josephson junction based metamaterials with in-situ tunability of second and third-order (Kerr) nonlinearities. We optimized the Josephson junction composites SNAILs, well-known in the superconducting circuits community, for the specific use case of building blocks for an impedance-matched nonlinear meta-material. In such devices, the strong third-order (Kerr) nonlinearity can be tuned from positive to negative values. To demonstrate the efficacy of this phenomenon, we have shown a use case of the meta-material as a TWPA with a new phase-matching mechanism: reversed Kerr phase matching, which utilizes the sign reversal of the Kerr nonlinearity to correct for the dispersion curvature of such devices arising due to its finite plasma. The meta-material operated as reversed Kerr TWPA exhibits up to 4 GHz wide combined amplification band with 8 GHz dynamic band tunability, -98 dBm saturation (1 dB compression point) around 20 dB gain, and amplifier added noise close to the standard quantum limit. The absence of any gaps in the transmission can provide a continuous amplification band with significantly lower gain ripples in contrast to the previously demonstrated TWPAs with dispersion engineering.We also present the generation of entanglement utilizing the metamaterials to demonstrate their versatility and further emphasize their potential in the general framework of nonlinear microwave quantum optics. Due to their large bandwidth, these devices have been identified as promising for generating two-mode squeezing and broadband entanglement. With a device optimized for the generation of broadband entanglement, we observed entanglement between two modes separated by up to 400 MHz. We measured logarithmic negativity between 0.27 and 0.51, and the collective quadrature squeezing below the vacuum limit between 1.5 and 2.1 dB. The presented proof-of-principle results can pave the way towards the implementation of Josephson junction based metamaterials in novel applications, including non-destructive single-photon detection, single-photon measurement and control in c-QED, photon-based quantum computing, precision sensing, the detection of dark matter, and quantum illumination.
Nearly quantum limited Josephson parametric amplifiers (JPAs) are essential components in superconducting quantum circuits. However, higher order nonlinearities of the Josephson cosine potential are known to cause gain compression, therefore limiting scalability. In an effort to reduce the fourth order, or Kerr nonlinearity, we realize a parametric amplifier with an Al-InAs superconductor–semiconductor hybrid Josephson junction (JJ). We extract the Kerr nonlinearity of the Al-InAs JJ from two different devices and show that it is three orders of magnitude lower compared to an Al-AlOX junction with identical Josephson inductance. We then demonstrate a four-wave-mixing (4WM) parametric amplifier made with an Al-InAs junction that achieves more than 20 dB of gain and −119 dBm of compression power, which outperforms single resonant JPAs based on Al junctions.
Nonlinear microwave resonators are a versatile tool in quantum information processing, enabling parametric amplification, continuous variable quantum computing, and engineered mode interactions. Many of these applications especially benefit from cubic nonlinearities enabling three-wave mixing; at the same time, they are limited by quartic nonlinearities giving rise to undesired Kerr effects. A recurrent challenge is therefore to engineer resonators with a finite cubic nonlinearity while suppressing quartic terms. Here, we investigate a superconducting resonator hosting two weak links fabricated from an aluminum-capped indium arsenide nanowire. We characterize the Kerr nonlinearity as a function of magnetic flux and gate bias, showing that it can be tuned to zero with either control parameter. Furthermore, we experimentally demonstrate three-wave mixing in a semiconductor-superconductor hybrid device, establishing nonzero cubic nonlinearity. An effective model based on Andreev bound states qualitatively captures the observed trends. Our results validate semiconductor-superconductor hybrid devices as a promising platform for tunable nonlinear superconducting circuits, with applications in parametric amplification, quantum control of bosonic modes, and engineering interactions between microwave modes.