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arXiv:2310.12117 · Physical review. B./Physical review. B

Effects of intralayer correlations on electron-hole double-layer superfluidity

Filippo Pascucci, Sara Conti, Andrea Perali, Jacques Tempere, David T. Neilson

Published Mar 18, 2024• 5 citations
arXivHTMLPDF

Abstract

We investigate the intralayer correlations acting within the layers in a superfluid system of electron-hole spatially separated layers. In this system, superfluidity is predicted to be almost exclusively confined to the Bose-Einstein condensate (BEC) and crossover regimes where the electron-hole pairs are well localized. In this case, Hartree-Fock is an excellent approximation for the intralayer correlations. We find in the BEC regime that the effect of the intralayer correlations on superfluid properties is negligible but in the BCS-BEC crossover regime the superfluid gap is significantly weakened by the intralayer correlations. This is caused by the intralayer correlations boosting the number of low-energy particle-hole excitations that drive the screening. We further find that the intralayer correlations suppress the predicted phenomenon in which the average pair size passes through a minimum as the crossover regime is traversed.

DOI
10.1103/physrevb.109.094512

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We investigate the intralayer correlations acting within the layers in a superfluid system of electron-hole spatially separated layers. In this system, superfluidity is predicted to be almost exclusively confined to the Bose-Einstein condensate (BEC) and crossover regimes where the electron-hole pairs are well localized. In this case, Hartree-Fock is an excellent approximation for the intralayer correlations. We find in the BEC regime that the effect of the intralayer correlations on superfluid properties is negligible but in the BCS-BEC crossover regime the superfluid gap is significantly weakened by the intralayer correlations. This is caused by the intralayer correlations boosting the number of low-energy particle-hole excitations that drive the screening. We further find that the intralayer correlations suppress the predicted phenomenon in which the average pair size passes through a minimum as the crossover regime is traversed.
Superfluidity in coupled electron-hole sheets of bilayer graphene is predicted here to be multicomponent because of the conduction and valence bands. We investigate the superfluid crossover properties as functions of the tunable carrier densities and the tunable energy band gap E_{g}. For small band gaps there is a significant boost in the two superfluid gaps, but the interaction-driven excitations from the valence to the conduction band can weaken the superfluidity, even blocking the system from entering the Bose-Einstein condensate (BEC) regime at low densities. At a given larger density, a band gap E_{g}∼80-120 meV can carry the system into the strong-pairing multiband BCS-BEC crossover regime, the optimal range for realization of high-T_{c} superfluidity.
We report quantum Monte Carlo evidence of the existence of large gap superfluidity in electron-hole double layers over wide density ranges. The superfluid parameters evolve from normal state to BEC with decreasing density, with the BCS state restricted to a tiny range of densities due to the strong screening of Coulomb interactions, which causes the gap to rapidly become large near the onset of superfluidity. The superfluid properties exhibit similarities to ultracold fermions and iron-based superconductors, suggesting an underlying universal behavior of BCS-BEC crossovers in pairing systems.
We predict enhanced electron-hole superfluidity in two coupled electron-hole armchair-edge terminated graphene nanoribbons separated by a thin insulating barrier. In contrast to graphene monolayers, the multiple subbands of the nanoribbons are parabolic at low energy with a gap between the conduction and valence bands, and with lifted valley degeneracy. These properties make screening of the electron-hole interaction much weaker than for coupled electron-hole monolayers, thus boosting the pairing strength and enhancing the superfluid properties. The pairing strength is further boosted by the quasi one-dimensional quantum confinement of the carriers, as well as by the large density of states near the bottom of each subband. The latter magnifies superfluid shape resonances caused by the quantum confinement. Several superfluid partial condensates are present for finite-width nanoribbons with multiple subbands. We find that superfluidity is predominately in the strongly-coupled BEC and BCS-BEC crossover regimes, with large superfluid gaps up to 100 meV and beyond. When the gaps exceed the subband spacing, there is significant mixing of the subbands, a rounding of the shape resonances, and a resulting reduction in the one-dimensional nature of the system.
We investigate the BCS-BEC crossover in a bilayer system of fermionic dipoles at zero temperature using the fixed-node diffusion Monte Carlo technique. The dipoles are confined on two parallel planes separated by a distance $\ensuremath{\lambda}$ and are aligned perpendicular to the planes by an external field. The interlayer pairing, which is responsible for the superfluid behavior of the system, crosses from a weak- to a strong-coupling regime by reducing the separation distance $\ensuremath{\lambda}$. For a fixed in-plane density equal in the two layers, we calculate the ground-state energy, the chemical potential, the pairing gap, and the quasiparticle dispersion as a function of the interlayer separation. At large $\ensuremath{\lambda}$ one recovers the ground-state energy of a single layer of fermions, and at small $\ensuremath{\lambda}$ one recovers that of a single layer of composite bosons with twice the particle mass and the dipole moment. The superfluid gap varies from the exponentially small BCS result to half of the large two-body binding energy in the Bose-Einstein condensate (BEC) regime of strong interlayer pairing. Results are compared with the predictions of the simplest mean-field theory valid in the low-density limit, and deviations are observed both in the BCS regime, where in-plane repulsions are important, and in the BEC regime, where the mean-field approach fails to describe the physics of composite dipolar bosons.
We investigate the quantum and thermal phase diagram of fermionic polar molecules loaded in a bilayer trapping potential with perpendicular dipole moment. We use both a BCS-theory approach that is most reliable at weak coupling and a strong-coupling approach that considers the two-body bound dimer states with one molecule in each layer as the relevant degree of freedom. The system ground state is a Bose-Einstein condensate (BEC) of dimer bound states in the low-density limit and a paired superfluid (BCS) state in the high-density limit. At zero temperature, the intralayer repulsion is found to broaden the regime of BCS-BEC crossover and can potentially induce system collapse through the softening of roton excitations. The BCS theory and the strongly coupled dimer picture yield similar predictions for the parameters of the crossover regime. The Berezinskii-Kosterlitz-Thouless transition temperature of the dimer superfluid is also calculated. The crossover can be driven by many-body effects and is strongly affected by the intralayer interaction which was ignored in previous studies.
BCS-Bose-Einstein condensation (BEC) crossover is effected by increasing pairing strength between fermions from weak to strong in the particle-particle channel, and has attracted a lot of attention since the experimental realization of quantum degenerate atomic Fermi gases. Here we study the effect of the (often dropped) particle-hole channel on the zero T gap Δ(0), superfluid transition temperature Tc, the pseudogap at Tc, and the mean-field ratio 2Δ(0)/, from BCS through BEC regimes, using a pairing fluctuation theory which includes self-consistently the contributions of finite-momentum pairs and features a pseudogap in single particle excitation spectrum. Summing over the infinite particle-hole ladder diagrams, we find a complex dynamical structure for the particle-hole susceptibility χph, and conclude that neglecting the self-energy feedback causes a serious over-estimate of χph. While our result in the BCS limit agrees with Gor'kov et al., the particle-hole channel effect becomes more complex and pronounced in the crossover regime, where χph is reduced by both a smaller Fermi surface and a big (pseudo)gap. Deep in the BEC regime, the particle-hole channel contributions drop to zero. We predict a density dependence of the magnetic field at the Feshbach resonance, which can be used to quantify χph and test different theories.