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arXiv:1601.06942 · Scientific Reports

Large gap electron-hole superfluidity and shape resonances in coupled graphene nanoribbons

M. Zarenia, A. Perali, François Maria Peeters, D. Neilson

Published Apr 25, 2016• 9 citations
arXivHTMLPDF

Abstract

We predict enhanced electron-hole superfluidity in two coupled electron-hole armchair-edge terminated graphene nanoribbons separated by a thin insulating barrier. In contrast to graphene monolayers, the multiple subbands of the nanoribbons are parabolic at low energy with a gap between the conduction and valence bands, and with lifted valley degeneracy. These properties make screening of the electron-hole interaction much weaker than for coupled electron-hole monolayers, thus boosting the pairing strength and enhancing the superfluid properties. The pairing strength is further boosted by the quasi one-dimensional quantum confinement of the carriers, as well as by the large density of states near the bottom of each subband. The latter magnifies superfluid shape resonances caused by the quantum confinement. Several superfluid partial condensates are present for finite-width nanoribbons with multiple subbands. We find that superfluidity is predominately in the strongly-coupled BEC and BCS-BEC crossover regimes, with large superfluid gaps up to 100 meV and beyond. When the gaps exceed the subband spacing, there is significant mixing of the subbands, a rounding of the shape resonances, and a resulting reduction in the one-dimensional nature of the system.

DOI
10.1038/srep24860

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We predict enhanced electron-hole superfluidity in two coupled electron-hole armchair-edge terminated graphene nanoribbons separated by a thin insulating barrier. In contrast to graphene monolayers, the multiple subbands of the nanoribbons are parabolic at low energy with a gap between the conduction and valence bands, and with lifted valley degeneracy. These properties make screening of the electron-hole interaction much weaker than for coupled electron-hole monolayers, thus boosting the pairing strength and enhancing the superfluid properties. The pairing strength is further boosted by the quasi one-dimensional quantum confinement of the carriers, as well as by the large density of states near the bottom of each subband. The latter magnifies superfluid shape resonances caused by the quantum confinement. Several superfluid partial condensates are present for finite-width nanoribbons with multiple subbands. We find that superfluidity is predominately in the strongly-coupled BEC and BCS-BEC crossover regimes, with large superfluid gaps up to 100 meV and beyond. When the gaps exceed the subband spacing, there is significant mixing of the subbands, a rounding of the shape resonances, and a resulting reduction in the one-dimensional nature of the system.
Superfluidity in coupled electron-hole sheets of bilayer graphene is predicted here to be multicomponent because of the conduction and valence bands. We investigate the superfluid crossover properties as functions of the tunable carrier densities and the tunable energy band gap E_{g}. For small band gaps there is a significant boost in the two superfluid gaps, but the interaction-driven excitations from the valence to the conduction band can weaken the superfluidity, even blocking the system from entering the Bose-Einstein condensate (BEC) regime at low densities. At a given larger density, a band gap E_{g}∼80-120 meV can carry the system into the strong-pairing multiband BCS-BEC crossover regime, the optimal range for realization of high-T_{c} superfluidity.
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Two-band electronic structures with a valence and a conduction band separated by a tunable energy gap and with pairing of electrons in different channels can be relevant to investigate the properties of two-dimensional multiband superconductors and electron-hole superfluids, such as monolayer FeSe, recently discovered superconducting bilayer graphene, and double-bilayer graphene electron-hole systems. This electronic configuration also allows us to study the coexistence of superconductivity and charge-density waves in connection with underdoped cuprates and transition metal dichalcogenides. By using a mean-field approach to study the system mentioned above, we have obtained numerical results for superconducting gaps, chemical potential, condensate fractions, coherence lengths, and superconducting mean-field critical temperature, considering a tunable band gap and different fillings of the conduction band, for a parametric choice of the pairing interactions. By tuning these quantities, the electrons redistribute among valence and conduction band in a complex way, leading to a new physics with respect to single-band superconductors, such as density-induced and band-selective BCS-BEC crossover, quantum phase transitions, and hidden criticalities. At finite temperature, this phenomenon is also responsible for the nonmonotonic behavior of the superconducting gaps resulting in a superconducting-normal state reentrant transition, without the need of disorder or magnetic effects.
We investigate the intralayer correlations acting within the layers in a superfluid system of electron-hole spatially separated layers. In this system, superfluidity is predicted to be almost exclusively confined to the Bose-Einstein condensate (BEC) and crossover regimes where the electron-hole pairs are well localized. In this case, Hartree-Fock is an excellent approximation for the intralayer correlations. We find in the BEC regime that the effect of the intralayer correlations on superfluid properties is negligible but in the BCS-BEC crossover regime the superfluid gap is significantly weakened by the intralayer correlations. This is caused by the intralayer correlations boosting the number of low-energy particle-hole excitations that drive the screening. We further find that the intralayer correlations suppress the predicted phenomenon in which the average pair size passes through a minimum as the crossover regime is traversed.
We report quantum Monte Carlo evidence of the existence of large gap superfluidity in electron-hole double layers over wide density ranges. The superfluid parameters evolve from normal state to BEC with decreasing density, with the BCS state restricted to a tiny range of densities due to the strong screening of Coulomb interactions, which causes the gap to rapidly become large near the onset of superfluidity. The superfluid properties exhibit similarities to ultracold fermions and iron-based superconductors, suggesting an underlying universal behavior of BCS-BEC crossovers in pairing systems.
Flat-band systems such as magic-angle twisted bilayer graphene host strong-correlation superconductivity at vanishingly weak coupling, yet how quantum geometry and pairing fluctuations conspire to drive this phenomenon remains an open question. We investigate finite-temperature superfluidity in a quasi-two-dimensional Lieb lattice using a pairing fluctuation theory with a band-uniform attractive interaction g<0g<0g<0 that isolates the intrinsic quantum geometric contributions. Quantum geometry significantly amplifies superfluidity; the geometric pair hopping integral surpasses its conventional counterpart, and the geometric superfluid density becomes the dominant in-plane transport component. When the Fermi level enters the flat band, the BCS paradigm breaks down entirely; the pairing gap and TcT_\text{c}Tc​ shift from exponential to anomalous power-law scaling Δ,Tc∝∣g∣νΔ, T_\text{c} \propto |g|^νΔ,Tc​∝∣g∣ν (ν>1ν>1ν>1), and the superfluid density inherits an unconventional power-law temperature dependence at low temperatures. In the 2D limit (tz=0t_z=0tz​=0), the pseudogap at TcT_\text{c}Tc​ nearly saturates the zero-temperature gap even at ∣g∣/t=0.001|g|/t=0.001∣g∣/t=0.001, placing the system in a strong-pseudogap regime that would otherwise require unitary or BEC-scale interactions. These findings establish a microscopic mechanism for flat-band enhanced superfluidity and offer testable predictions for ultracold atom experiments.