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arXiv:2310.10924 · Physica Scripta

Resonance fluorescence in Λ, V and Ξ - type three-level configurations

Surajit Sen, Tushar Kanti Dey, Bimalendu Deb

Published Oct 12, 2023• 6 citations
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Abstract

Abstract We theoretically study the resonance fluorescence spectra of the lambda (Λ), vee (V) and cascade (Ξ) type three-level configurations. It is shown that each system with two detuning frequencies can be modelled using the SU(3) symmetry group to derive a generalized optical Bloch equation. For each configuration, this equation is solved to calculate the two-time correlation function by invoking the quantum regression theorem. The incoherent part of the power spectra gives the characteristic multi-peak fluorescence profiles which are different for different configurations. We also discuss how the dressed-state structure of such system can explain the origin of quintuplet profile of the fluorescent spectrum.

DOI
10.1088/1402-4896/ad02c8

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Abstract We theoretically study the resonance fluorescence spectra of the lambda (Λ), vee (V) and cascade (Ξ) type three-level configurations. It is shown that each system with two detuning frequencies can be modelled using the SU(3) symmetry group to derive a generalized optical Bloch equation. For each configuration, this equation is solved to calculate the two-time correlation function by invoking the quantum regression theorem. The incoherent part of the power spectra gives the characteristic multi-peak fluorescence profiles which are different for different configurations. We also discuss how the dressed-state structure of such system can explain the origin of quintuplet profile of the fluorescent spectrum.
The cascade, lambda and vee type of three-level systems are shown to be described by three different Hamiltonians in the SU(3) basis. We investigate the Bloch space structure of each configuration by solving the corresponding Bloch equation and show that at resonance, the seven-dimensional Bloch sphere S7{\mathcal S}^7S7 is broken into two distinct subspaces S2×S4{\mathcal S}^2{\times}{\mathcal S}^4S2×S4 due to the existence of a pair of quadratic constants. We also give a possible representation of the qutrit wave function and discuss its equivalence with the three-level system.
The fluorescence field from one of the two allowed transitions in a three-level atom can sense squeezed fluctuations of a vacuum field coupled to the other transition. We examine the fluorescence spectra of strongly driven three-level atoms in \ensuremath{\Lambda}, V, and cascade configurations in which one of the two one-photon transitions is coupled to a finite-bandwidth squeezed vacuum field, when the bandwidth is much smaller than the difference in the atomic transition frequencies, though much larger than atomic decay rates and Rabi frequencies of the driving fields. The driving fields are on one-photon resonance, and the squeezed vacuum field is generated by a degenerate parameter oscillator. Details are only given for the \ensuremath{\Lambda} configuration. The extension to the V and cascade configurations is straightforward. We find that in all configurations the fluorescence spectra of the transition not coupled to the squeezed vacuum field are composed of five lines, one central and two pairs of sidebands, with intensities and widths strongly influenced by the squeezed vacuum field. However, only the central component and the outer sidebands exhibit a dependence on the squeezing phase. We also examine the fluorescence spectrum for the cascade configuration with a squeezed vacuum field on resonance with the two-photon transition between the ground and the most excited states and now generated by a nondegenerate parametric oscillator. In this case, where the squeezed vacuum field can be made coupled to both transitions, all spectral lines depend on the squeezing phase. The spectral features are explained in terms of the dressed-atom model of the system. We show that the coherent mixing of the atomic states by the strong driving fields modifies transition rates between the dressed states, which results in the selective phase dependence of the spectral features. \textcopyright{} 1996 The American Physical Society.
We generalize our earlier formalism to treat the effects of both the finite-bandwidth excitations and finite arbitrary detunings, on the fluorescent spectra and second-order intensity correlation functions in optical double resonance. It is assumed that the bandwidth arises from the phase and/or amplitude fluctuations in the fields driving a three-level atom in cascade configuration. Under the conditions that one or both of these fields are intense, secular approximation and the theory of multiplicative stochastic processes are invoked to derive a Markovian master equation for the atomic-density operator averaged over both phase and amplitude. The quantum regression theorem is used to derive analytical expressions for the fluorescent spectra and the second-order intensity correlation functions which explicitly display the effects due to detunings and fluctuations.
This paper is concerned with two rather basic phenomena: the incoherent fluorescence spectrum of an atom driven by an intense laser field and the coupling of the atom to the (empty) modes of the radiation field. The sum of the many-photon processes gives rise to the inelastic part of the atomic fluorescence, which, for a two-level system, has a well-known characteristic three-peak structure known as the Mollow spectrum. From a theoretical point of view, the Mollow spectrum finds a natural interpretation in terms of transitions among laser-dressed states which are the energy eigenstates of a second-quantized two-level system strongly coupled to a driving laser field. As recently shown, the quasi-energies of the laser-dressed states receive radiative corrections which are nontrivially different from the results which one would expect from an investigation of the coupling of the bare states to the vacuum modes. In this article, we briefly review the basic elements required for the analysis of the dynamic radiative corrections, and we generalize the treatment of the radiative corrections to the incoherent part of the steady-state fluorescence to a three-level system consisting of 1S, 3P and 2S states.
The resonance fluorescence of a three-level system is studied in each of its three possible configurations—ladder, lambda and vee—when it also interacts with broad band squeezed vacua and the applied fields are resonant. We obtain general expressions which apply for any configuration and do not make use of the secular approximation. Detailed results are presented which depend upon the degree of squeezing and the squeezing phase, in addition to the intensities of the applied fields. It is shown that asymmetric spectra may be obtained in certain circumstances. These are interpreted in terms of coherent and incoherent transitions induced by the squeezed fields. We also take the opportunity to assess the accuracy of the secular approximation.
Although the resonance fluorescence spectrum of coherent light scattering from a two-level atom has been discussed in many papers, the effects of longitudinal, transverse relaxation and optical pumping have not yet been considered simultaneously in the motion equations. By solving the optical Bloch equations including the longitudinal relaxation time T 1 , transverse relaxation time T 2 and optical pumping parameter Δ 0 , in the case T 2 /T 1 <<1, we obtain the spectrum with dip in the central peak besides the familiar spectrum of three peaks. In addition, we find that the parameter Δ 0 and detuning Δω have influence on the symmetry, height and width of the spectrum of the three peaks.