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arXiv:2309.14728 · Physical Review Letters

Engineering Mixing Properties of Fluids by Spatial Modulations

Abid Ali, Hiroki Saito

Published Apr 23, 2024• 2 citations
arXivHTMLPDF

Abstract

We propose a method to change the effective interaction between two fluids by modulation of their local density distributions with external periodic potentials, whereby the mixing properties can be controlled. This method is applied to a mixture of dilute bosonic gases, and binodal and spinodal curves emerge in the phase diagram. Spinodal decomposition into a mixed-bubble state becomes possible, in which one of the coexisting phases has a finite mixing ratio. A metastable mixture is also realized, which undergoes phase separation via nucleation.

DOI
10.1103/physrevlett.132.173402

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We propose a method to change the effective interaction between two fluids by modulation of their local density distributions with external periodic potentials, whereby the mixing properties can be controlled. This method is applied to a mixture of dilute bosonic gases, and binodal and spinodal curves emerge in the phase diagram. Spinodal decomposition into a mixed-bubble state becomes possible, in which one of the coexisting phases has a finite mixing ratio. A metastable mixture is also realized, which undergoes phase separation via nucleation.
In mean-field theory, the ground state of a two-component Bose-Einstein condensate (BEC) in a uniform system is either uniformly mixed or totally separated. Beyond-mean-field effects introduce an additional phase, the mixed-bubble state, in which the two components remain mixed within one of the separated domains. Here we show that a mixed-bubble state can emerge in a binary mixture of spin-1 7Li{}^{7}{\rm{Li}}7Li and 23Na{}^{23}{\rm{Na}}23Na BECs even within the mean-field framework. We further demonstrate the existence of a metastable uniformly-mixed state, which undergoes a transition to the mixed-bubble state triggered by a local perturbation.
We study the ground-state properties of mixtures of strongly interacting bosonic atoms in an optical lattice. Applying a mean-field approximation to the Hubbard model for Bose-Bose mixtures, we calculate the densities and superfluid order parameters for both species. Due to the repulsive interaction between the two species, the system exhibits phase separation. First, in the extreme limit of the zero-hopping case, we derive analytical expressions for the phase boundaries. In particular, we derive the conditions for phase separation in the Mott insulator phase. We find that the conditions for the phase separation depend on the on-site interactions as well as the occupation numbers. In particular, we show that the coexisting state appears by varying the on-site inter-species interaction. We also show the phase diagram of the finite hopping case. Second, we calculate the spatial density profile of 87^{87}87Rb-41^{41}41K mixtures in the combined potential of a parabolic trap and an optical lattice using the local density approximation. We fixed the number of 87^{87}87Rb and varied the number of 41^{41}41K, and used the parameters estimated by experiments. We show that the phase separated 87^{87}87Rb-41^{41}41K mixtures distribute like in a parabolic trap case. Furthermore, we find that phase separated mixtures distribute a nesting structure.
Repulsive Bose-Bose mixtures are known to either mix or phase separate into pure components. Here we predict a mixed-bubble regime in which bubbles of the mixed phase coexist with a pure phase of one of the components. This is a beyond-mean-field effect that occurs for unequal masses or unequal intraspecies coupling constants and is due to a competition between the mean-field term, quadratic in densities, and a nonquadratic beyond-mean-field correction. We find parameters of the mixed-bubble regime in all dimensions and discuss implications for current experiments.
We investigated the spatial phase separation of the two components forming a bosonic mixture distributed in a four-well lattice with a ring geometry. We studied the ground state of this system, described by means of a binary Bose–Hubbard Hamiltonian, by implementing a well-known coherent-state picture which allowed us to find the semi-classical equations determining the distribution of boson components in the ring lattice. Their fully analytic solutions, in the limit of large boson numbers, provide the boson populations at each well as a function of the interspecies interaction and of other significant model parameters, while allowing to reconstruct the non-trivial architecture of the ground-state four-well phase diagram. The comparison with the L-well (L=2,3) phase diagrams highlights how increasing the number of wells considerably modifies the phase diagram structure and the transition mechanism from the full-mixing to the full-demixing phase controlled by the interspecies interaction. Despite the fact that the phase diagrams for L=2,3,4 share various general properties, we show that, unlike attractive binary mixtures, repulsive mixtures do not feature a transition mechanism which can be extended to an arbitrary lattice of size L.
By studying the dynamic stability of Bose-Einstein-condensed binary mixtures trapped on the surface of an ideal two-dimensional spherical bubble, we show how the Rabi coupling between the species can modulate the interactions leading to parametric resonances. In this spherical geometry, the discrete unstable angular modes drive both phase separations and spatial patterns, with Faraday waves emerging and coexisting with an immiscible phase. Noticeable is the fact that, in the context of discrete kinetic energy spectrum, the only parameters to drive the emergence of Faraday waves are the $s\text{\ensuremath{-}}wave$ contact interactions and the Rabi coupling. Once analytical solutions for population dynamics are obtained, the stability of homogeneous miscible species is investigated through Bogoliubov--de Gennes and Floquet methods, with predictions being analyzed by full numerical solutions applied to the corresponding time-dependent coupled formalism.
These lecture notes contain an introduction to quantum simulation of bosonic systems in the continuum, focusing on weakly interacting Bose-Bose mixtures with competing mean-field interactions. When the values of such interactions are fine-tuned to almost completely cancel the mean-field energy, quantum fluctuations become apparent and dominate the behavior of the system, stabilizing an ultradilute quantum liquid phase. An analogous situation appears in single-component dipolar quantum gases. We review the mechanism that gives rise to this exotic quantum liquid, which can form droplets that are self-bound in the absence of any external confinement, and discuss their properties and dynamics in both the mixture and the dipolar cases. In dipolar gases, arrays of dipolar droplets stabilized by quantum fluctuations can establish global phase coherence and form supersolids. In bosonic mixtures, supersolidity can emerge already at the mean-field level through spin-orbit coupling. We discuss the properties of such spin-orbit-coupled supersolids, comparing them to their dipolar counterparts. Specifically, we focus on their periodic density modulation, phase coherence, and peculiar excitation spectrum, which hosts both superfluid and crystal excitations. Finally, we conclude by discussing open research directions in the areas of quantum liquid droplets and spin-orbit-coupled supersolids, in particular at the interface of the two research topics.