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arXiv:2008.05870 · Physical Review Letters

Mixed Bubbles in Bose-Bose Mixtures

Pascal Naidon, Dmitry S. Petrov

Published Mar 18, 2021• 38 citations
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Abstract

Repulsive Bose-Bose mixtures are known to either mix or phase separate into pure components. Here we predict a mixed-bubble regime in which bubbles of the mixed phase coexist with a pure phase of one of the components. This is a beyond-mean-field effect that occurs for unequal masses or unequal intraspecies coupling constants and is due to a competition between the mean-field term, quadratic in densities, and a nonquadratic beyond-mean-field correction. We find parameters of the mixed-bubble regime in all dimensions and discuss implications for current experiments.

DOI
10.1103/physrevlett.126.115301

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Repulsive Bose-Bose mixtures are known to either mix or phase separate into pure components. Here we predict a mixed-bubble regime in which bubbles of the mixed phase coexist with a pure phase of one of the components. This is a beyond-mean-field effect that occurs for unequal masses or unequal intraspecies coupling constants and is due to a competition between the mean-field term, quadratic in densities, and a nonquadratic beyond-mean-field correction. We find parameters of the mixed-bubble regime in all dimensions and discuss implications for current experiments.
In mean-field theory, the ground state of a two-component Bose-Einstein condensate (BEC) in a uniform system is either uniformly mixed or totally separated. Beyond-mean-field effects introduce an additional phase, the mixed-bubble state, in which the two components remain mixed within one of the separated domains. Here we show that a mixed-bubble state can emerge in a binary mixture of spin-1 7Li{}^{7}{\rm{Li}}7Li and 23Na{}^{23}{\rm{Na}}23Na BECs even within the mean-field framework. We further demonstrate the existence of a metastable uniformly-mixed state, which undergoes a transition to the mixed-bubble state triggered by a local perturbation.
We investigate a Bose-Bose mixture across the miscible-immiscible phase transition governed by quantum fluctuations in one dimension. We find the recently predicted so-called mixed bubbles as ground states close to the mean-field miscible-immiscible threshold. These bubbles form a pocket of miscibility, separated by one of the components. The collective excitations reflect the symmetry breaking resulting from the bubble formation. The partial miscibility of the system allows for persistent currents in an annular confinement. Intriguingly, the mixed bubble acts like an intrinsic weak link, connecting the rotational behavior of the mixed bubble state to current efforts in atomtronic applications.
Abstract A three-component bosonic mixture is capable of demonstrating a significantly rich phase diagram in comparison with a two-component mixture or a single-component fluid. With experimental studies of multi-component mixtures gaining momentum and comparatively few theoretical efforts, we consider an interacting three-component Bose gas on a lattice and, via a strong coupling expansion of the Bose–Hubbard model, look into a variety of situations, such as the intraspecies and intraspecies interactions being the same and different, attractive and repulsive, etc. A scenario of rich phase diagrams emerges where one species of atoms can be in the superfluid phase while the other two may be in insulating phases. Such a mixed-phase diagram with different species coexisting in different phases is an exciting one: a possibility that can be explored in experiments. Numerical solution of the mean field equations has further demonstrated the occurrence of insulating phases with fractional filling of each species of atoms. Such insulating phases with fractional occupancies are counterintuitive in the context of incompressible phases.
Mixing two kinds of particles that repel each other usually results in either a homogeneous mixture when the repulsion is weak, or a complete phase separation of the two kinds when their repulsion is too strong. It is shown however that there is an intermediate regime where the two kinds can coexist in their ground state as a bubble immersed in a gas of one kind. Such a situation is obtained by adding heavy repulsive impurities into a Bose-Einstein condensate. Above a certain strength of the mutual repulsion, a stable bubble of impurities and bosons can be formed, resulting from the equilibrium between the interactions induced by the bosons inside the bubble and the outside pressure from the surrounding bosons. At some particular strength, the effective interactions between the impurities consist of only three-body interactions. Finally, above a critical strength, the bosons are ejected from the bubble and the impurities collapse into a pure bubble of impurities. This phenomenon could be observed with an imbalanced mixture of ultra-cold atoms of different masses. Moreover, it appears possible to reach a regime where the impurities form a dense bubble of strongly-interacting particles.
In this thesis we investigate the properties of mixtures of Bose gases in one dimensions at zero temperature using quantum Monte-Carlo methods. First we investigate the limiting case of an impurity interacting with an atomic bath. We characterize the impurity, by calculating its effective mass, binding energy as well as the contact parameter between the impurity and the bath. In particular, we find that the effective mass rapidly increases to very large values when the impurity gets strongly coupled to an otherwise weakly repulsive bath. Then we describe uniform balanced mixtures with repulsive interactions. We investigate the miscibility phase diagram of the two components and find that correlations do not alter the phase diagram predicted by mean-field theories. We investigate the Andreev-Bashkin effect , a non-dissipative drag between the the two components of the gas and find that the drag becomes very large in the strongly interacting regime. In non-homogeneous systems we also investigate the frequency of the spin-dipole mode. Finally we describe mixtures with attractive inter-species interactions, where one can obtain a liquid ground state because of the competition between the inter-species attraction and intra-species repulsion. We characterize the the liquid and we find that the liquid state can be formed if the ratio of coupling strengths between inter-species attractive and intra-species repulsive interactions exceeds a critical value.
We study the thermodynamic properties of binary Bose mixtures by developing a beyond mean-field Popov theory which properly includes the effects of quantum and thermal fluctuations in both the density and spin channels. Results for key thermodynamic quantities, such as the isothermal compressibility and the magnetic susceptibility, are derived from a perturbative calculation of the grand-canonical potential. We find that thermal fluctuations can play a crucial role on the miscibility condition of a binary mixture, favoring phase separation at finite temperature even if the mixture is soluble at zero temperature, as already anticipated in a previous work [M. Ota et al., Phys. Rev. Lett. 123, 075301 (2019)]. We further investigate the miscibility condition for binary mixtures in the presence of asymmetry in the intraspecies interactions, as well as in the masses of the two components. Furthermore, we discuss the superfluid behavior of the mixture and the temperature dependence of the Andreev-Bashkin effect.