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arXiv:2309.11553 · Physical Review X

Hybrid Quantum-Classical Stochastic Approach to Dissipative Spin-Boson Models

Naushad Ahmad Kamar, Mohammad F. Maghrebi

Published May 29, 2025• 5 citations
arXivHTMLPDF

Abstract

Spin-boson models involving many interacting spins and bosons are ubiquitous in quantum simulation platforms. At the same time, characterizing the dynamics of these quantum systems represents a significant challenge. Here, we consider general spin-boson models where bosons are subject to Markovian dissipation (e.g., due to cavity loss). We present an exact hybrid quantum-classical stochastic approach where the solution of a classical stochastic equation—mimicking the bosonic modes—is input into a quantum stochastic equation for the spins. Furthermore, the spins are effectively decoupled for each stochastic realization, which nevertheless comes at the expense of sampling over unphysical states. In contrast with existing stochastic approaches based on the influence functional formalism, we place no restriction (factorizability or Gaussianity) on the initial state, or the spin-boson coupling (except that it be linear in the bosonic operator). Markovian dissipation, being at the heart of our approach, renders the stochastic equations Markovian even in the strong coupling regime. Furthermore, it ensures hermiticity (though not positivity) of the density matrix for each realization, thus improving the convergence of stochastic sampling. Interestingly, we find a condition on the classical simulability of the system based solely on the single atom cooperativity even in a many-body setting. We benchmark and showcase the utility of our approach in several examples, specifically in cases where a direct numerical computation is unfeasible.

DOI
10.1103/physrevx.15.021073

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Spin-boson models involving many interacting spins and bosons are ubiquitous in quantum simulation platforms. At the same time, characterizing the dynamics of these quantum systems represents a significant challenge. Here, we consider general spin-boson models where bosons are subject to Markovian dissipation (e.g., due to cavity loss). We present an exact hybrid quantum-classical stochastic approach where the solution of a classical stochastic equation—mimicking the bosonic modes—is input into a quantum stochastic equation for the spins. Furthermore, the spins are effectively decoupled for each stochastic realization, which nevertheless comes at the expense of sampling over unphysical states. In contrast with existing stochastic approaches based on the influence functional formalism, we place no restriction (factorizability or Gaussianity) on the initial state, or the spin-boson coupling (except that it be linear in the bosonic operator). Markovian dissipation, being at the heart of our approach, renders the stochastic equations Markovian even in the strong coupling regime. Furthermore, it ensures hermiticity (though not positivity) of the density matrix for each realization, thus improving the convergence of stochastic sampling. Interestingly, we find a condition on the classical simulability of the system based solely on the single atom cooperativity even in a many-body setting. We benchmark and showcase the utility of our approach in several examples, specifically in cases where a direct numerical computation is unfeasible.
The spin-boson model, describing a two-level system coupled to a bosonic bath, is extensively studied as a paradigmatic dissipative quantum system, exhibiting rich dynamical behavior and even a localization transition in the strong coupling regime. Here, we additionally consider dephasing as a source of Markovian dissipation on top of the non-Markovian dynamics due to an Ohmic bath, and investigate the dynamics of the spin. We show that the characteristic frequency of the spin dynamics, while strongly renormalized by the bosonic bath, changes in a simple fashion (or does not change at all) with dephasing. To obtain these results, we develop an exact nonperturbative method known as the stochastic Schr\"odinger equation, mimicking the Ohmic bath via a stochastic magnetic field combined with the Lindblad quantum master equation due to dephasing, which allows us to numerically compute the dynamics. Furthermore, we derive weak-coupling analytic results utilizing the well-known noninteracting blip approximation. Our findings are relevant to quantum simulation of the spin-boson model in the regime of strong coupling in trapped ions and circuit QED architectures among others.
Applications of quantum devices and simulators require an accurate understanding of their dynamics as well as the effects of environmental noise. While some sources of noise can be modeled as Markovian dissipation, coupling to resonators or vibrational modes often produces non-Markovian dynamics as well, making it difficult to characterize the system, particularly for interacting many-body systems. Here, we identify a broad class of exactly solvable many-body quantum systems with both non-Markovian dynamics and Markovian dissipation. We consider a prototypical model of spins coupled to lossy bosonic modes that mediate Ising-type interactions. We exclude a transverse field but allow local spin dissipation that need not commute with the interactions, including dephasing, relaxation, pumping, and even processes that generate coherences. Using an exact stochastic representation, we decouple the many-body dynamics into the evolution of individual spins, yielding exact spin observables and correlations without adiabatically eliminating the bosons. In the Markovian limit, our solutions describe Ising models with correlated dephasing and nonreciprocal interactions. An example of spin squeezing shows that both the achievable squeezing and its optimal preparation time depend strongly on the interplay between non-Markovian dynamics and Markovian dissipation.
We introduce and apply a numerically exact method for investigating the real-time dissipative dynamics of quantum impurities embedded in a macroscopic environment beyond the weak-coupling limit. We focus on the spin-boson Hamiltonian that describes a two-level system interacting with a bosonic bath of harmonic oscillators. This model is archetypal for investigating dissipation in quantum systems, and tunable experimental realizations exist in mesoscopic and cold-atom systems. It finds abundant applications in physics ranging from the study of decoherence in quantum computing and quantum optics to extended dynamical mean-field theory. Starting from the real-time Feynman-Vernon path integral, we derive an exact stochastic Schr\"odinger equation that allows us to compute the full spin density matrix and spin-spin correlation functions beyond weak coupling. We greatly extend our earlier work [P. P. Orth, A. Imambekov, and K. Le Hur, Phys. Rev. A 82, 032118 (2010)] by fleshing out the core concepts of the method and by presenting a number of interesting applications. Methodologically, we present an analogy between the dissipative dynamics of a quantum spin and that of a classical spin in a random magnetic field. This analogy is used to recover the well-known noninteracting-blip approximation in the weak-coupling limit. We explain in detail how to compute spin-spin autocorrelation functions. As interesting applications of our method, we explore the non-Markovian effects of the initial spin-bath preparation on the dynamics of the coherence ${\ensuremath{\sigma}}^{x}(t)$ and of ${\ensuremath{\sigma}}^{z}(t)$ under a Landau-Zener sweep of the bias field. We also compute to a high precision the asymptotic long-time dynamics of ${\ensuremath{\sigma}}^{z}(t)$ without bias and demonstrate the wide applicability of our approach by calculating the spin dynamics at nonzero bias and different temperatures.
Classical Brownian motion has well been investigated since the pioneering work of Einstein, which inspired mathematicians to lay the theoretical foundation of stochastic processes. A stochastic formulation for quantum dynamics of dissipative systems described by the system-plus-bath model has been developed and found many applications in chemical dynamics, spectroscopy, quantum transport, and other fields. This article provides a tutorial review of the stochastic formulation for quantum dissipative dynamics. The key idea is to decouple the interaction between the system and the bath by virtue of the Hubbard-Stratonovich transformation or Itô calculus so that the system and the bath are not directly entangled during evolution, rather they are correlated due to the complex white noises introduced. The influence of the bath on the system is thereby defined by an induced stochastic field, which leads to the stochastic Liouville equation for the system. The exact reduced density matrix can be calculated as the stochastic average in the presence of bath-induced fields. In general, the plain implementation of the stochastic formulation is only useful for short-time dynamics, but not efficient for long-time dynamics as the statistical errors go very fast. For linear and other specific systems, the stochastic Liouville equation is a good starting point to derive the master equation. For general systems with decomposable bath-induced processes, the hierarchical approach in the form of a set of deterministic equations of motion is derived based on the stochastic formulation and provides an effective means for simulating the dissipative dynamics. A combination of the stochastic simulation and the hierarchical approach is suggested to solve the zero-temperature dynamics of the spin-boson model. This scheme correctly describes the coherent-incoherent transition (Toulouse limit) at moderate dissipation and predicts a rate dynamics in the overdamped regime. Challenging problems such as the dynamical description of quantum phase transition (local- ization) and the numerical stability of the trace-conserving, nonlinear stochastic Liouville equation are outlined.
We extend a standard stochastic theory to study open quantum systems coupled to a generic quantum environment. We exemplify the general framework by studying a two-level quantum system coupled bilinearly to the three fundamental classes of non-interacting particles: bosons, fermions, and spins. In this unified stochastic approach, the generalized stochastic Liouville equation (SLE) formally captures the exact quantum dissipations when noise variables with appropriate statistics for different bath models are applied. Anharmonic effects of a non-Gaussian bath are precisely encoded in the bath multi-time correlation functions that noise variables have to satisfy. Starting from the SLE, we devise a family of generalized hierarchical equations by averaging out the noise variables and expand bath multi-time correlation functions in a complete basis of orthonormal functions. The general hierarchical equations constitute systems of linear equations that provide numerically exact simulations of quantum dynamics. For bosonic bath models, our general hierarchical equation of motion reduces exactly to an extended version of hierarchical equation of motion which allows efficient simulation for arbitrary spectral densities and temperature regimes. Similar efficiency and flexibility can be achieved for the fermionic bath models within our formalism. The spin bath models can be simulated with two complementary approaches in the present formalism. (I) They can be viewed as an example of non-Gaussian bath models and be directly handled with the general hierarchical equation approach given their multi-time correlation functions. (II) Alternatively, each bath spin can be first mapped onto a pair of fermions and be treated as fermionic environments within the present formalism.
The exact dynamics of a system coupled to an environment can be described by an integro-differential stochastic equation for the reduced density. The influence of the environment is incorporated through a mean field which is both stochastic and nonlocal in time and where the standard two-time correlation functions of the environment appear naturally. Since no approximation is made, the presented theory incorporates exactly dissipative and non-Markovian effects. Applications to the spin-boson model coupled to a heat bath with various coupling regimes and temperature show that the presented stochastic theory can be a valuable tool to simulate exactly the dynamics of open quantum systems. Links with the stochastic Schrödinger equation method and possible extensions to "imaginary time" propagation are discussed.