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arXiv:2307.10537 · Physical Review Letters

Wide-Band Unambiguous Quantum Sensing via Geodesic Evolution

Ke Zeng, Xiaohui Yu, Martin Bodo Plenio, Zhenyu Wang

Published Jun 20, 2024• 9 citations
arXivHTMLPDF

Abstract

We present a quantum sensing technique that utilizes a sequence of π pulses to cyclically drive the qubit dynamics along a geodesic path of adiabatic evolution. This approach effectively suppresses the effects of both decoherence noise and control errors while simultaneously removing unwanted resonance terms, such as higher harmonics and spurious responses commonly encountered in dynamical decoupling control. As a result, our technique offers robust, wide-band, unambiguous, and high-resolution quantum sensing capabilities for signal detection and individual addressing of quantum systems, including spins. To demonstrate its versatility, we showcase successful applications of our method in both low-frequency and high-frequency sensing scenarios. The significance of this quantum sensing technique extends to the detection of complex signals and the control of intricate quantum environments. By enhancing detection accuracy and enabling precise manipulation of quantum systems, our method holds considerable promise for a variety of practical applications.

DOI
10.1103/physrevlett.132.250801

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We present a quantum sensing technique that utilizes a sequence of π pulses to cyclically drive the qubit dynamics along a geodesic path of adiabatic evolution. This approach effectively suppresses the effects of both decoherence noise and control errors while simultaneously removing unwanted resonance terms, such as higher harmonics and spurious responses commonly encountered in dynamical decoupling control. As a result, our technique offers robust, wide-band, unambiguous, and high-resolution quantum sensing capabilities for signal detection and individual addressing of quantum systems, including spins. To demonstrate its versatility, we showcase successful applications of our method in both low-frequency and high-frequency sensing scenarios. The significance of this quantum sensing technique extends to the detection of complex signals and the control of intricate quantum environments. By enhancing detection accuracy and enabling precise manipulation of quantum systems, our method holds considerable promise for a variety of practical applications.
We develop theoretically and demonstrate experimentally a universal dynamical decoupling method for robust quantum sensing with unambiguous signal identification. Our method uses randomization of control pulses to simultaneously suppress two types of errors in the measured spectra that would otherwise lead to false signal identification. These are spurious responses due to finite-width π pulses, as well as signal distortion caused by π pulse imperfections. For the cases of nanoscale nuclear-spin sensing and ac magnetometry, we benchmark the performance of the protocol with a single nitrogen vacancy center in diamond against widely used nonrandomized pulse sequences. Our method is general and can be combined with existing multipulse quantum sensing sequences to enhance their performance.
Accurate frequency estimation of oscillating signals over a broad bandwidth is a central task in quantum sensing, yet it is often compromised by spurious responses to higher-order harmonics in realistic multi-frequency environments. Here we experimentally demonstrate a high-accuracy and broadband quantum frequency sensing protocol based on geodesic control, implemented using the electron spin of a single nitrogen-vacancy center in diamond. By engineering an intrinsically single-frequency response, geodesic control enables bias-free frequency estimation with strong suppression of harmonic-induced systematic errors across a wide spectral range spanning from the megahertz to the gigahertz regime. Furthermore, by incorporating synchronized readout, we achieve millihertz-level frequency resolution under noisy signal conditions. Our results provide systematic experimental benchmarking of geodesic control for quantum frequency sensing and establish it as a practical approach for high-accuracy metrology in realistic environments.
Sensing, localizing, and identifying individual nuclear spins or frequency components of a signal in the presence of a noisy environment requires the development of robust and selective methods of dynamical decoupling. An important challenge that remains to be addressed in this context are spurious higher-order resonances in current dynamical decoupling sequences as they can lead to the misidentification of nuclei or of different frequency components of external signals. Here we overcome this challenge with engineered quantum sensing sequences that achieve both enhanced robustness and the simultaneous suppression of higher-order-harmonic resonances. We experimentally demonstrate the principle using a single nitrogen-vacancy center spin sensor which we apply to the unambiguous detection of external protons.
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Abstract The field of quantum control and sensing encounters challenges due to various forms of time-dependent noise. We introduce a generalized filter-function framework that treats noise coupling strength as a tunable control parameter, enabling target noise suppression across user-defined frequency bands. By optimizing this generalized filter function, we design band-selective control pulses that achieve high fidelity of single- and two-qubit gates under strong noise with diverse spectral profiles. We further extend the method to selectively enhance the signal-to-noise ratio for quantum sensing of AC signals with an enhanced precision of up to 12.58 dB. The resulting control pulses are experimentally feasible, offering a practical pathway toward robust quantum operations and high-precision sensing under spectrally complex noises.
We propose a scheme for sensing of an oscillating field in systems with large inhomogeneous broadening and driving field variation by applying sequences of phased, adiabatic, chirped pulses.These act as a double filter for dynamical decoupling, where the adiabatic changes of the mixing angle during the pulses rectify the signal and partially remove frequency noise.The sudden changes between the pulses act as instantaneous π pulses in the adiabatic basis for additional noise suppression.We also use the pulses' phases to correct for other errors, e.g., due to nonadiabatic couplings.Our technique improves significantly the coherence time in comparison to standard XY8 dynamical decoupling in realistic simulations in NV centers with large inhomogeneous broadening.Beyond the theoretical proposal, we also present proof-of-principle experimental results for quantum sensing of an oscillating field in NV centers in diamond, demonstrating superior performance compared to the standard technique.