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arXiv:2307.06225 · Optics Continuum

Practical quantum imaging with undetected photons

Emma J. Pearce, Nathan R. Gemmell, Jefferson Flórez, Jiaye Ding, Rupert F. Oulton, Alex S. Clark, Chris C. Phillips

Published Oct 26, 2023• 30 citations
arXivHTMLPDF

Abstract

Infrared (IR) imaging is invaluable across many scientific disciplines, from material analysis to diagnostic medicine. However, applications are often limited by detector cost, resolution and sensitivity, noise caused by the thermal IR background, and the cost, portability and tunability of infrared sources. Here, we describe a compact, portable, and low-cost system that is able to image objects at IR wavelengths without an IR source or IR detector. This imaging with undetected photons (IUP) approach uses quantum interference and correlations between entangled photon pairs to transfer image information from the IR to a wavelength which can be detected with a standard silicon camera. We also demonstrate a rapid analysis approach to acquire both phase and transmission image information. These developments provide an important step towards making IUP a commercially viable technique.

DOI
10.1364/optcon.507154

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Infrared (IR) imaging is invaluable across many scientific disciplines, from material analysis to diagnostic medicine. However, applications are often limited by detector cost, resolution and sensitivity, noise caused by the thermal IR background, and the cost, portability and tunability of infrared sources. Here, we describe a compact, portable, and low-cost system that is able to image objects at IR wavelengths without an IR source or IR detector. This imaging with undetected photons (IUP) approach uses quantum interference and correlations between entangled photon pairs to transfer image information from the IR to a wavelength which can be detected with a standard silicon camera. We also demonstrate a rapid analysis approach to acquire both phase and transmission image information. These developments provide an important step towards making IUP a commercially viable technique.
Spectroscopy and imaging in the mid-infrared ($2.5\phantom{\rule{4pt}{0ex}}\textmu{}\mathrm{m}\ensuremath{\sim}\ensuremath{\lambda}\ensuremath{\sim}25\phantom{\rule{4pt}{0ex}}\textmu{}\mathrm{m}$) is bedeviled by the presence of a strong 300-K thermal background at room temperature that makes infrared (IR) detectors decades noisier than can be readily achieved in the visible. The technique of imaging with undetected photons (IUP) exploits the quantum correlations between entangled photon pairs to transfer image information from one spectral region to another, and here we show that it does so in a way that is immune to the thermal background. This means that IUP can be used to perform high-speed photon-counting measurements across the mid-IR spectrum, using uncooled visible detectors that are many times cheaper, faster, and more sensitive than their IR counterparts.
Infrared (IR) imaging sees a wide range of applications due to its ability to probe molecular vibrations but is limited by detector technology available in this part of the spectrum. Imaging with undetected photons [1] offers an alternative. Using a nonlinear interferometer producing visible-IR photon pairs, transmission and phase information of an object in the IR can be observed by monitoring the interference of visible photons. No IR detection or laser is required. Recently there has been a move towards increasing the technology readiness levels of this approach, considering size, stability, and speed [2–4].
Quantum imaging with undetected photons (QIUP) allows an object to be probed at mid-infrared frequencies by only measuring interference in the visible range, thus leveraging silicon camera technology. We show that non-collinear phase-matching in a silver thiogallate (AgGaS2_22​) crystal enables wide-field QIUP in the wavelength range of 6-10 μμμm (1670-1000 cm−1^{-1}−1). A combination of coherent detection and infrared photons being ``undetected'' enables imaging at ${\sim}$100 times better than the background-limited infrared photodetection (BLIP) limit. At 8 μμμm, our images have over 8000 ±\pm± 100 resolvable elements with a 297 ±\pm± 5 μμμm resolution, and 10 s acquisition time. Our results pave the way to fast, background-noise-free, room-temperature, spectrally-selective mid-infrared imaging.
Owing to its capacity for unique (bio)-chemical specificity, microscopy with mid-infrared (IR) illumination holds tremendous promise for a wide range of biomedical and industrial applications. The primary limitation, however, remains detection, with current mid-IR detection technology often marrying inferior technical capabilities with prohibitive costs. Here, we experimentally show how nonlinear interferometry with entangled light can provide a powerful tool for mid-IR microscopy while only requiring near-IR detection with a silicon-based camera. In this proof-of-principle implementation, we demonstrate widefield imaging over a broad wavelength range covering 3.4 to 4.3 μm and demonstrate a spatial resolution of 35 μm for images containing 650 resolved elements. Moreover, we demonstrate that our technique is suitable for acquiring microscopic images of biological tissue samples in the mid-IR. These results form a fresh perspective for potential relevance of quantum imaging techniques in the life sciences.
Quantum sensing in the infrared regime often demands the use of expensive and cryogenically operated detectors. Nonlinear interferometry has paved the way for information transfer from the infrared to the near--infrared or visible regime in various quantum technologies. A particularly interesting application of these interferometers involves spectrally--resolved quantum imaging using undetected photons, enabled by the use of temperature--tunable parametric amplifiers. In this work, we demonstrate spectrally resolved transmission imaging with undetected photons around 1550 nm using a spontaneous parametric down conversion based folded nonlinear interferometric scheme, registering the attenuation of a zebrafish larva as a biological feasibility test. We characterize and calibrate the interferometer, having achieved spectrally resolved interference fringes with a maximum baseline visibility of ∼74%\sim 74\%∼74% in the near--infrared regime. Phase--stepped readout of a grating spectrometer gives a resolving power of ∼1460\sim1460∼1460 (from the spectrometer's point spread function) at 1550 nm, and ∼730\sim 730∼730 from the coherence length, the finest reported for imaging with undetected photons, over an instantaneous spectral window of ≈51\approx 51≈51 cm−1^{-1}−1.
Sensing with undetected photons has become a vibrant, application-driven research domain with a special focus on the mid-infrared (mid-IR) wavelength region. Since the mid-IR contains spectral bands with highly specific and strong molecular absorbance signatures, often referred to as fingerprints, a multitude of different samples and their compositions can be detected and quantified spectroscopically. Enhancing this spectroscopic method with imaging capabilities leads to a powerful technique for environmental monitoring and biomedical applications that enables automated diagnostics while omitting time-consuming and non-reversible labeling steps. To evade the shortcomings of state-of-the-art instruments for mid-IR hyperspectral microscopy—namely cost, complexity, power consumption, and performance, which stem from technological challenges in mid-IR detection and light sources—we construct a proof-of-concept nonlinear interferometer in a wide-field imaging arrangement. This nominally narrowband imaging technique is then expanded to acquire broadband spectral information through capturing images for varying interferometer displacement and applying a pixelwise Fourier-transform of the resulting interferograms, yielding high-resolution infrared spectra for each camera pixel. For the broadband range of 2300−3100cm −1 , covering the important CH-stretch band, we perform hyperspectral imaging that simultaneously resolves 3500 spatial modes, each with a spectral resolution of 10cm −1 , leveraging in total around 10 5 spatio-spectrally entangled photon modes. Our image acquisition uses a commercial sCMOS camera, while a medium-power and compact continuous-wave pump laser is the only necessary light source. For a moderate speed of 360 voxel/s, we obtain a predominantly shot-noise-influenced signal-to-noise ratio (SNR) of 50. We further demonstrate the practicality of our novel hyperspectral imaging technique for microplastics detection and bio-imaging tasks and outline engineering solutions to increase its speed by several orders of magnitude. This shows that our quantum imaging technique is highly promising for applications requiring compact, cost-effective label-free analyses.