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arXiv:2306.06055 · Physical Review A

Cooperative photon emission rates in random atomic clouds

Viviana Viggiano, Romain Bachelard, Fabio Deelan Cunden, Paolo Facchi A, Robin Kaiser, Saverio Pascazio, Francesco Vincenzo Pepe

Published Dec 1, 2023• 3 citations
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Abstract

We investigate the properties of the cooperative decay modes of a cold atomic cloud, characterized by a Gaussian distribution in three dimensions, initially excited by a laser in the linear regime. We study the properties of the decay rate matrix $S$, whose dimension coincides with the number of atoms in the cloud, in order to get a deeper insight into properties of cooperative photon emission. Since the atomic positions are random, $S$ is a Euclidean random matrix whose entries are a function of the atom distances. We show that in the limit of a large number of atoms in the cloud, the eigenvalue distribution of $S$ depends on a single parameter ${b}_{0}$, called the cooperativeness parameter, which can be viewed as a quantifier of the number of atoms that are coherently involved in an emission process. For very small values of ${b}_{0}$, we find that the limit eigenvalue density is approximately triangular. We also study the nearest-neighbor spacing distribution and the eigenvector statistics, finding that although the decay rate matrices are Euclidean, the bulk of their spectra mostly behaves according to the expectations of classical random matrix theory. In particular, in the bulk, there is level repulsion and the eigenvectors are delocalized, therefore exhibiting the universal behavior of chaotic quantum systems.

DOI
10.1103/physreva.108.063701

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We investigate the properties of the cooperative decay modes of a cold atomic cloud, characterized by a Gaussian distribution in three dimensions, initially excited by a laser in the linear regime. We study the properties of the decay rate matrix SSS, whose dimension coincides with the number of atoms in the cloud, in order to get a deeper insight into properties of cooperative photon emission. Since the atomic positions are random, SSS is a Euclidean random matrix whose entries are a function of the atom distances. We show that in the limit of a large number of atoms in the cloud, the eigenvalue distribution of SSS depends on a single parameter b0{b}_{0}b0​, called the cooperativeness parameter, which can be viewed as a quantifier of the number of atoms that are coherently involved in an emission process. For very small values of b0{b}_{0}b0​, we find that the limit eigenvalue density is approximately triangular. We also study the nearest-neighbor spacing distribution and the eigenvector statistics, finding that although the decay rate matrices are Euclidean, the bulk of their spectra mostly behaves according to the expectations of classical random matrix theory. In particular, in the bulk, there is level repulsion and the eigenvectors are delocalized, therefore exhibiting the universal behavior of chaotic quantum systems.
In the collective photon emission from atomic clouds both the atomic transition frequency and the decay rate are modified compared to a single isolated atom, leading to the effects of superradiance and subradiance. In this article, we analyze the properties of the Euclidean random matrix associated with the radiative dynamics of a cold atomic cloud, previously investigated in the contexts of photon localization and Dicke super- and subradiance. We present evidence of a phase transition, surprisingly controlled by the cooperativeness parameter, rather than the spatial density or the diagonal disorder. The numerical results corroborate the occurrence of such a phase transition at a critical value of the cooperativeness parameter, above which the lower edge of the spectrum vanishes, exhibiting a macroscopic accumulation of eigenvalues. Independent evaluations based on the two phenomena provide the same value for the critical cooperativeness parameter.
We present a framework to investigate the collective properties of atomic lattices in one, two, and three dimensions. We analyze the single-photon band structure and associated atomic decay rates, revealing a fundamental dependence on dimensionality. One- and two-dimensional arrays are shown to be inherently radiative, exhibiting band gaps and decay rates that oscillate between superradiant and subradiant regimes, as a function of lattice spacing. In contrast, three-dimensional lattices are found to be fundamentally non-radiative due to the inhibition of spontaneous emission, with decay only at discrete Bragg resonances. Furthermore, we demonstrate that this structural difference dictates the system dynamics, which crosses over from dissipative decay in lower dimensions to coherent transport in three dimensions. Our results provide insight into cooperative effects in atomic arrays at the single-photon level.
We consider collective emission of a single photon from a cloud of NNN two-level atoms (one excited, $N\ensuremath{-}1$ ground state). For a dense cloud the problem is reduced to finding eigenfunctions and eigenvalues of an integral equation. We discuss an exact analytical solution of this many-atom problem for a spherically symmetric atomic cloud. Some eigenstates decay much faster then the single atom decay rate, while the others undergo very slow decay. We show that virtual processes yield a small effect on the evolution of rapidly decaying states. However, they change the long time dynamics from exponential decay into a power-law behavior which can be observed experimentally. For trapped states virtual processes are much more important yielding additional decay channels which results in a slow decay of the otherwise trapped states. We also show that quantum mechanical treatment of spontaneous emission of weakly excited atomic ensemble is analogous to emission of NNN classical harmonic oscillators.
Cooperative emission is well understood for idealized symmetric systems, but its fundamental limits in spatially extended, free-space ensembles remain an open question. Here, we derive a universal law for the scaling of the maximum photon emission rate with system size that unifies both ordered arrays and disordered atomic clouds in arbitrary dimensions at fixed density. We demonstrate that, for a fixed atomic density, the maximum emission rate scales universally as the product of the atom number and the system's geometric optical depth. The geometric optical depth differs from the result of the Beer-Lambert law at high density and encodes the dimensional scaling across all regimes from independent emission to the Dicke limit. Furthermore, we establish a scaling law for directional detection, revealing that the observed rate depends on the detector's numerical aperture: small apertures yield Dicke-like quadratic scaling, whereas large apertures recover our integrated universal bound. Our results establish optical depth as the parameter governing many-body cooperative emission in both ordered and disordered ensembles, and reveal that directional and total-emission scalings must be carefully distinguished in experimental settings.
We study emission of a single photon from a spherically symmetric cloud of NNN atoms (one atom is excited; $N\ensuremath{-}1$ are in the ground state) and present an exact analytical expression for eigenvalues and eigenstates of this many-body problem. We found that some states decay much faster than the single-atom decay rate, while other states are trapped and undergo very slow decay. When the size of the atomic cloud is small compared with the radiation wavelength, we found that the radiation frequency undergoes a large shift.
We study cooperative single-photon spontaneous emission from three multilevel atoms with one of them being excited for different atomic configurations in optical vector theory. The dynamic evolution is solved by finding the eigenvalues of a 3 \ifmmode\times\else\texttimes\fi{} 3 matrix, and then the relevant decay rates and Lamb shifts are obtained analytically. It is shown that the symmetry of atomic configuration has a big influence on the super-radiance of the system. To obtain strong super-radiance requires not only the distances among the three atoms to be much shorter than the wavelength, but also to have symmetrical distribution. We also calculate the emission spectra and find that it normally has three peaks, but it has two peaks under the equilateral-triangle configuration.