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arXiv:2306.05467 · Communications Physics

Charge-4e supercurrent in a two-dimensional InAs-Al superconductor-semiconductor heterostructure

Carlo Ciaccia, R. Haller, A. C. C. Drachmann, Tyler Lindemann, Michael J. Manfra, Constantin Schrade, Christian Schönenberger

Published Jan 22, 2024• 31 citations
arXivHTMLPDF

Abstract

Abstract Superconducting qubits with intrinsic noise protection offer a promising approach to improve the coherence of quantum information. Crucial to such protected qubits is the encoding of the logical quantum states into wavefunctions with disjoint support. Such encoding can be achieved by a Josephson element with an unusual charge-4e supercurrent emerging from the coherent transfer of pairs of Cooper-pairs. In this work, we demonstrate the controlled conversion of a conventional charge-2e dominated to a charge-4e dominated supercurrent in a superconducting quantum interference device (SQUID) consisting of gate-tunable planar Josephson junctions. We investigate the ac Josephson effect of the SQUID and measure a dominant photon emission at twice the fundamental Josephson frequency together with a doubling of the number of Shapiro steps, both consistent with the appearance of charge-4e supercurrent. Our results present a step towards protected superconducting qubits based on superconductor-semiconductor hybrid materials.

DOI
10.1038/s42005-024-01531-x

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•Sep 25, 2024•0 citations
Abstract Superconducting qubits with intrinsic noise protection offer a promising approach to improve the coherence of quantum information. Crucial to such protected qubits is the encoding of the logical quantum states into wavefunctions with disjoint support. Such encoding can be achieved by a Josephson element with an unusual charge-4e supercurrent emerging from the coherent transfer of pairs of Cooper-pairs. In this work, we demonstrate the controlled conversion of a conventional charge-2e dominated to a charge-4e dominated supercurrent in a superconducting quantum interference device (SQUID) consisting of gate-tunable planar Josephson junctions. We investigate the ac Josephson effect of the SQUID and measure a dominant photon emission at twice the fundamental Josephson frequency together with a doubling of the number of Shapiro steps, both consistent with the appearance of charge-4e supercurrent. Our results present a step towards protected superconducting qubits based on superconductor-semiconductor hybrid materials.
Abstract Hybrid superconductor-semiconductor Josephson field-effect transistors (JoFETs) function as Josephson junctions with a gate-tunable critical current. Additionally, they can feature a non- sinusoidal current-phase relation (CPR) containing multiple harmonics of the superconducting phase difference, a so-far underutilized property. In this work, we exploit this multi-harmonicity to create a Josephson circuit element with an almost perfectly π-periodic CPR, indicative of a largely dominant charge-4e supercurrent transport. Such a Josephson element was recently proposed as the basic building block of a protected superconducting qubit. Here, it is realized using a superconducting quantum interference device (SQUID) with low-inductance aluminum arms and two nominally identical JoFETs. The latter are fabricated from a SiGe/Ge/SiGe quantum-well heterostructure embedding a high-mobility two-dimensional hole gas. By carefully adjusting the JoFET gate voltages and finely tuning the magnetic flux through the SQUID close to half a flux quantum, we achieve a regime where the sin(2φ) component accounts for more than 95 % of the total supercurrent. This result demonstrates a new promising route for the realization of superconducting qubits with enhanced coherence properties.
Hybrid superconductor(S)-semiconductor(Sm) devices bring a range of functionalities into superconducting circuits. In particular, hybrid parity-protected qubits and Josephson diodes were recently proposed and experimentally demonstrated. Such devices leverage the nonsinusoidal character of the Josephson current-phase relation (CPR) in highly transparent S-Sm-S junctions. Here, we report an experimental study of superconducting quantum-interference devices (SQUIDs) embedding Josephson field-effect transistors fabricated from a SiGe/Ge/SiGe heterostructure grown on a 200-mm silicon wafer. The single-junction CPR shows up to three harmonics with gate-tunable amplitude. In the presence of microwave irradiation, the ratio of the first two dominant harmonics, corresponding to single and double Cooper-pair transport processes, is consistently reflected in relative weight of integer and half-integer Shapiro steps. A combination of magnetic-flux and gate-voltage control enables tuning the SQUID functionality from a nonreciprocal Josephson-diode regime with 27% asymmetry to a π -periodic Josephson regime suitable for the implementation of parity-protected superconducting qubits. These results illustrate the potential of Ge-based hybrid devices as versatile and scalable building blocks of superconducting quantum circuits. Published by the American Physical Society 2024
Superconducting quantum circuits derive their nonlinearity from the Josephson energy-phase relation. Besides the fundamental cos⁡φ\cosφcosφ term, this relation can also contain higher Fourier harmonics cos⁡(kφ)\cos(kφ)cos(kφ) corresponding to correlated tunneling of kkk Cooper pairs. The parity of the dominant tunneling process, i.e.~whether an odd or even number of Cooper pairs tunnel, results in qualitatively different properties, and controlling this opens up a wide range of applications in superconducting technology. However, access to even-dominated regimes has remained challenging and has so far relied on complex multi-junction or all-hybrid architectures. Here, we demonstrate a simple "harmonic parity qubit" (HPQ); an element that combines two aluminum-oxide tunnel junctions in parallel to a gate-tunable InAs/Al nanowire junction forming a SQUID, and use spectroscopy versus flux to reconstruct its energy-phase relation at 85 gate voltage points. At half flux quantum, the odd harmonics of the Josephson potential can be suppressed by up to two orders of magnitude relative to the even harmonics, producing a double-well potential dominated by even harmonics with minima near ±π/2\pmπ/2±π/2. The ability to control harmonic parity enables supercurrent carried by pairs of Cooper pairs and provides a new building block for Fourier engineering in superconducting circuits.
Hybrid semiconductor-superconductor qubits have recently emerged as a promising alternative to traditional platforms, combining material advantages with device-level tunability. A defining feature is their gate-tunable Josephson coupling, enabling superconducting qubit architectures with full electric-field control and offering a path toward scalable, low-crosstalk quantum processors. This approach seeks to merge benefits of superconducting and semiconductor qubits, for instance by encoding quantum information in the spin of a quasiparticle occupying an Andreev bound state, thus combining long coherence times with fast, flexible control. Progress has accelerated through bottom-up engineering of Andreev states in coupled quantum dot arrays, leading to architectures such as minimal Kitaev chains hosting Majorana zero modes. In parallel, Hamiltonian-protected designs aim to enhance resilience against local noise and decoherence by exploiting superconducting phase dynamics and discrete charge or flux degrees of freedom. This article reviews recent theoretical and experimental advances in hybrid qubits, providing an overview of physical mechanisms, device implementations, and emerging architectures, with emphasis on their potential for (topologically) protected quantum information processing. While many designs remain at proof-of-concept stage, rapid progress suggests practical demonstrations may soon be achievable.
Coherence of superconducting qubits can be improved by implementing designs that protect the parity of Cooper pairs on superconducting islands. Here, we introduce a parity-protected qubit based on voltage-controlled semiconductor nanowire Josephson junctions, taking advantage of the higher harmonic content in the energy-phase relation of few-channel junctions. A symmetric interferometer formed by two such junctions, gate-tuned into balance and frustrated by a half-quantum of applied flux, yields a cos(2φ) Josephson element, reflecting coherent transport of pairs of Cooper pairs. We demonstrate that relaxation of the qubit can be suppressed tenfold by tuning into the protected regime.
Hybrid superconductor(S)-semiconductor(Sm) devices bring a range of functionalities into superconducting circuits by introducing Josephson field-effect transistors (JoFETs): Josephson junctions with a gate-tunable critical current. In particular, hybrid parity-protected qubits and Josephson diodes were recently proposed and experimentally demonstrated. Such devices leverage the multiharmonicity of the Josephson current-phase relation (CPR) in highly transparent S-Sm-S junctions, a so-far underutilized property. In this work we report an experimental study of superconducting quantum-interference devices (SQUIDs) embedding JoFETs fabricated from a SiGe/Ge/SiGe heterostructure grown at CEA-Grenoble. The single junction CPRs shows multiple harmonics with gate tunable amplitudes. In the presence of microwave irradiation, the appearance of integer and half integer Shapiro steps confirms this observation. A combination of magnetic-flux and gate-voltage control enables tuning the SQUID functionality from a nonreciprocal Josephson-diode regime with 27 % asymmetry to a π-periodic Josephson regime. Within a double SQUID device, we are able to quantitatively characterize a regime where the sin(2φ) component accounts for more than 95 % of the total supercurrent. Finally, this result is placed into perspective through a discussion of the implementation of a cos(2φ) parity-protected qubit within the Al-Ge/SiGe hybrid platform