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arXiv:2305.06406 · Physical Review Letters

Fluctuation-Dissipation Relation in a Nonequilibrium Quantum Fluid

T. R. Kirkpatrick, D. Belitz

Published Dec 13, 2023• 4 citations
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Abstract

There is no simple fluctuation-dissipation theorem (FDT) for nonequilibrium systems. We show that for a fluid in a nonequilibrium steady state (NESS) characterized by a constant temperature gradient there is a generalized FDT that relates commutator correlation functions to the bilinear response of products of observables. This allows for experimental probes of the long-range correlations in such a system, quantum or classical, via response experiments. We also show that the correlations are not tied to thermal fluctuations but are intrinsic to the NESS and reflect a generalized rigidity.

DOI
10.1103/physrevlett.131.244001

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There is no simple fluctuation-dissipation theorem (FDT) for nonequilibrium systems. We show that for a fluid in a nonequilibrium steady state (NESS) characterized by a constant temperature gradient there is a generalized FDT that relates commutator correlation functions to the bilinear response of products of observables. This allows for experimental probes of the long-range correlations in such a system, quantum or classical, via response experiments. We also show that the correlations are not tied to thermal fluctuations but are intrinsic to the NESS and reflect a generalized rigidity.
The absence of a simple fluctuation-dissipation theorem is a major obstacle for studying systems that are not in thermodynamic equilibrium. We show that for a fluid in a nonequilibrium steady state characterized by a constant temperature gradient the commutator correlation functions are still related to response functions; however, the relation is to the bilinear response of products of two observables, rather than to a single linear response function as is the case in equilibrium. This modified fluctuation-response relation holds for both quantum and classical systems. It is both motivated and informed by the long-range correlations that exist in such a steady state and allows for probing them via response experiments. This is of particular interest in quantum fluids, where the direct observation of fluctuations by light scattering would be difficult. In classical fluids it is known that the coupling of the temperature gradient to the diffusive shear velocity leads to correlations of various observables, in particular temperature fluctuations, that do not decay as a function of distance, but rather extend over the entire system. We investigate the nature of these correlations in a fermionic quantum fluid and show that the crucial coupling between the temperature gradient and velocity fluctuations is the same as in the classical case. Accordingly, the nature of the long-ranged correlations in the hydrodynamic regime also is the same. However, as one enters the collisionless regime in the low-temperature limit the nature of the velocity fluctuations changes: they become ballistic rather than diffusive. As a result, correlations of the temperature and other observables are still singular in the long-wavelength limit, but the singularity is weaker than in the hydrodynamic regime.
The fluctuation-dissipation theorem (FDT) is a central result in statistical physics, both for classical and quantum systems. It establishes a relationship between the linear response of a system under a time-dependent perturbation and time correlations of certain observables in equilibrium. Here we derive a generalization of the theorem which can be applied to any Markov quantum system and makes use of the symmetric logarithmic derivative (SLD). There are several important benefits from our approach. First, such a formulation clarifies the relation between classical and quantum versions of the equilibrium FDT. Second, and more important, it facilitates the extension of the FDT to arbitrary quantum Markovian evolution, as given by quantum maps. Third, it clarifies the connection between the FDT and quantum metrology in systems with a non-equilibrium steady state.
We present a fluctuation-dissipation theorem (FDT) for nonequilibrium quantum systems with detailed-balance breaking, which deviates from the conventional form of the FDT for equilibrium systems preserving detailed balance. Using the phase space formulation of quantum mechanics and the potential-flux landscape framework, we find that the response function of nonequilibrium quantum systems to external perturbations contains a nontrivial contribution from the quantum curl flux quantifying detailed-balance breaking in the steady state, in addition to the correlation function of observables in the steady state representing the contribution of spontaneous fluctuations which is also present in the equilibrium FDT. We illustrate our general formalism with a harmonic oscillator coupled to two heat baths, and show that the nonequilibrium FDT reduces to the conventional expression at the equilibrium condition when the flux contribution vanishes.
The fluctuation-dissipation theorem (FDT) is a cornerstone of statistical mechanics, linking the linear response of a system to external perturbations with the equilibrium fluctuations of its constituent degrees of freedom. Traditionally formulated for Hermitian quantum systems in thermal equilibrium, its applicability to non-Hermitian quantum systems, which are increasingly relevant in areas such as open quantum systems, PT-symmetric quantum mechanics, and topological phases, remains a complex and largely unresolved challenge. This paper presents a theoretical framework for a universal fluctuation-dissipation theorem applicable to a broad class of non-Hermitian quantum systems. We demonstrate how the presence of non-Hermiticity, characterized by complex energy eigenvalues and non-orthogonal eigenstates, fundamentally modifies the relationship between correlation functions and response functions. Our derivation utilizes a generalized time-evolution operator and incorporates concepts from non-Hermitian spectral theory, revealing a modified FDT that accounts for energy gain or loss inherent in these systems. The resulting theorem provides insights into the interplay between quantum noise and dissipation in environments far from conventional thermal equilibrium, offering a crucial tool for understanding and engineering non-Hermitian quantum devices. We discuss the implications for non-equilibrium steady states and the breakdown of standard notions of temperature and entropy, proposing a path towards experimental verification in platforms like photonic lattices and cold atoms with controlled losses.
The fluctuation-dissipation theorem (FDT) is a central result in statistical physics, both for classical and quantum systems. It establishes a relationship between the linear response of a system under a time-dependent perturbation and time correlations of certain observables in equilibrium. Here we derive a generalization of the theorem which can be applied to any Markov quantum system and makes use of the symmetric logarithmic derivative (SLD). There are several important benefits from our approach. First, such a formulation clarifies the relation between classical and quantum versions of the equilibrium FDT. Second, and more important, it facilitates the extension of the FDT to arbitrary quantum Markovian evolutions, as given by quantum maps. Third, it brings out the full connection between the FDT and the Quantum Fisher information, the figure of merit in quantum metrology.
We derive a general set of fluctuation relations for a nonequilibrium open quantum system described by a Lindblad master equation. In the special case of conservative Hamiltonian dynamics, these identities allow us to retrieve quantum versions of Jarzynski and Crooks relations. In the linear response regime, these fluctuation relations yield a fluctuation-dissipation theorem (FDT) valid for a stationary state arbitrarily far from equilibrium. For a closed system, this FDT reduces to the celebrated Callen-Welton-Kubo formula.