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arXiv:2305.05831 · Physical Review Letters

Quartet Superfluid in Two-Dimensional Mass-Imbalanced Fermi Mixtures

Ruijin Liu, Wei Wang, Xiaoling Cui

Published Nov 9, 2023• 19 citations
arXivHTMLPDF

Abstract

Quartet superfluid (QSF) is a distinct type of fermion superfluidity that exhibits high-order correlation beyond the conventional BCS pairing paradigm. In this Letter, we report the emergent QSF in 2D mass-imbalanced Fermi mixtures with two-body contact interactions. This is facilitated by the formation of a quartet bound state in vacuum that consists of a light atom and three heavy fermions. For an optimized heavy-light number ratio 3:1, we identify QSF as the ground state in a considerable parameter regime of mass imbalance and 2D coupling strength. Its unique high-order correlation can be manifested in the momentum-space crystallization of a pairing field and density distribution of heavy fermions. Our results can be readily detected in Fermi-Fermi mixtures nowadays realized in cold atoms laboratories, and meanwhile shed light on exotic superfluidity in a broad context of mass-imbalanced fermion mixtures.

DOI
10.1103/physrevlett.131.193401

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Quartet superfluid (QSF) is a distinct type of fermion superfluidity that exhibits high-order correlation beyond the conventional BCS pairing paradigm. In this Letter, we report the emergent QSF in 2D mass-imbalanced Fermi mixtures with two-body contact interactions. This is facilitated by the formation of a quartet bound state in vacuum that consists of a light atom and three heavy fermions. For an optimized heavy-light number ratio 3:1, we identify QSF as the ground state in a considerable parameter regime of mass imbalance and 2D coupling strength. Its unique high-order correlation can be manifested in the momentum-space crystallization of a pairing field and density distribution of heavy fermions. Our results can be readily detected in Fermi-Fermi mixtures nowadays realized in cold atoms laboratories, and meanwhile shed light on exotic superfluidity in a broad context of mass-imbalanced fermion mixtures.
We study quantum fluctuations in a quartet superfluid (QSF) of two-dimensional (2D) fermion mixtures with mass imbalance. Here QSF is a high-order superfluid that corresponds to the condensation of (1+31+31+3) clusters, each consisting of a light fermion and three heavy ones. By incorporating the Gaussian fluctuations respecting dominant four-body correlations in this system, our theory successfully recovers the leading universal logarithmic contribution to the 2D equation of state in the deep binding regime, thereby offering a correct physical picture of quartet clusters behaving as composite bosons. By extending the Gaussian fluctuation theory from pairing to quartet superfluids, our results shed light on quantum fluctuations in general fermion superfluids with arbitrarily high-order correlations.
We consider a superfluid state in a two-component gas of fermionic atoms with equal densities and unequal masses in the BCS limit. We develop a perturbation theory along the lines proposed by Gorkov and Melik-Barkhudarov and find that for a large difference in the masses of heavy (M)(M)(M) and light (m)(m)(m) atoms one has to take into account both the second-order and third-order contributions. The result for the critical temperature and order parameter is then quite different from the prediction of the simple BCS approach. Moreover, the small parameter of the theory turns out to be $({p}_{F}\ensuremath{\mid}a\ensuremath{\mid}∕\ensuremath{\hbar})\sqrt{M∕m}⪡1$, where pF{p}_{F}pF​ is the Fermi momentum and aaa the scattering length. Thus, for a large mass ratio M∕mM∕mM∕m the conventional perturbation theory requires significantly smaller Fermi momenta (densities) or scattering lengths than in the case of $M\ensuremath{\sim}m$, where the small parameter is ${p}_{F}\ensuremath{\mid}a\ensuremath{\mid}∕\ensuremath{\hbar}⪡1$. We show that three-body scattering resonances appearing at a large mass ratio due to the presence of three-body bound Efimov states do not influence the result, which in this sense becomes universal.
We study the ground-state phase diagram of population balanced and imbalanced ultracold atomic Fermi gases with a short-range attractive interaction throughout the crossover from BCS to Bose-Einstein condensation (BEC), in a two-dimensional (2D) optical lattice comprised of a 2D array of 1D lines. We find that the mixing of lattice and continuum dimensions, together with population imbalance, has an extraordinary effect on pairing and the superfluidity of atomic Fermi gases. In the balanced case, the superfluid ground state prevails over the majority of the phase space. However, for relatively small lattice hopping integral ttt and large lattice constant ddd, a pair density wave (PDW) emerges unexpectedly at intermediate coupling strength, and the nature of the in-plane and overall pairing changes from particlelike to holelike in the BCS and unitary regimes, associated with an abnormal increase in the Fermi volume with the pairing strength. In the imbalanced case, the stable polarized superfluid phase shrinks to only a small portion of the entire phase space spanned by t,dt, dt,d, imbalance ppp, and interaction strength UUU, mainly in the bosonic regime of low ppp, moderately strong pairing, relatively large ttt, and small ddd. Due to the Pauli exclusion between paired and excessive fermions within the confined momentum space, a PDW phase emerges and the overall pairing evolves from particlelike into holelike, as the pairing strength grows stronger in the BEC regime. In both cases, the ground-state property is largely governed by the Fermi surface topology. These findings are very different from the cases of a pure 3D continuum, a 3D lattice, or a 1D optical lattice.
We consider ultracold imbalanced Fermi gases with strong attractive interactions, for which Cooper-pair formation plays an important role. The two-component mixtures consist either of identical fermionic atoms in two different hyperfine states, or of two different atomic species. In both cases, the number of atoms for each component is allowed to be different, leading to a spin imbalance or a polarization. In the second case, the two different species also give rise to a mass imbalance for the particles. Imbalanced Fermi mixtures play a fundamental role in condensed-matter, nuclear and astroparticle physics. Experimentally, the atomic mixtures are made strongly interacting with the use of two-channel Feshbach resonances. We start out by treating these in more detail. We review the relevant scattering theory, and apply it to the well-studied case of resonant s-wave collisions with zero angular momentum. Furthermore, we discuss the less-studied case of p-wave collisions with nonzero angular momentum, and the inhomogeneous case due to a trapping potential. Having discussed the two-body physics, we turn to the many-body physics. The pioneering experimental studies of Cooper pairing in lithium-6 mixtures with a spin imbalance were performed by Zwierlein et al. [Science 311, 492 (2006)] and Partridge et al. [Science 311, 503 (2006)]. We study the mean-field theory for the polarized Fermi mixture to obtain a qualitative understanding of these experiments. In the unitarity limit, where the scattering length of the interatomic interaction diverges, the theory gives rise to two exotic superfluid phases that are absent in the balanced mixture. These are the gapless superfluid Sarma phase and the phase-separated phase. By using renormalization group techniques to account for the effects of strong interactions, we obtain also quantitative agreement with Monte-Carlo calculations and experiments. We then generalize our knowledge of the solely spin-imbalanced mixture to the mass-imbalanced case, where in particular the mixture consisting of lithium-6 and potassium-40 is experimentally promising. We study the mean-field phase diagram for this mixture in the unitarity limit, where we not only find phase separation and Sarma superfluidity, but also a Lifshitz point. The latter signals an instability towards a supersolid phase. We also include the effects of fluctuations, which do not alter the topology of the phase diagram. However, fluctuation effects lower the critical temperatures with an experimentally relevant factor of three. Finally, we study superfluidity in a fully polarized gas of potassium-40 atoms near a p-wave Feshbach resonance. In particular, we consider coherent Josephson oscillations between the superfluid components in the two channels of the resonance, whose frequencies contain a clear signature of the quantum phase transition that occurs as a function of applied magnetic field.
Polarons can serve as an ideal platform to identify few-body correlations in tackling complex many-body problems. In this work, we reveal various crystalline few-body correlations smoothly emergent from the mass-imbalanced Fermi polarons in two dimensions. A unified variational approach up to three particle-hole excitations allows us to extract the dominant dimer, trimer, or tetramer correlation in a single framework. When the fermion-impurity mass ratio is beyond certain critical value, the Fermi polaron is found to undergo a smooth crossover, instead of a sharp transition, from the polaronic to trimer and tetramer regimes as the fermion-impurity attraction is increased. The emergent trimer and tetramer correlations result in the momentum-space crystallization of particle-hole excitations featuring a stable diagonal or triangular structure, as can be directly probed through the density-density correlation of majority fermions. Our results shed light on the intriguing quantum phases in the mass-imbalanced Fermi-Fermi mixtures beyond the pairing superfluid paradigm.
We study universal clusters in quasi-two-dimensions (q2D) that consist of a light (L) atom interacting with two or three heavy (H) identical fermions, forming the trimer or tetramer bound state. The axial confinement in q2D is shown to lift the threefold degeneracy of three-dimensional trimer (tetramer) in p -wave channel and uniquely select the ground state with magnetic angular momentum | m | = 1 ( m = 0 ). By varying the interaction or confinement strength, we explore the dimensional crossover of these clusters from 3D to 2D, characterized by a gradual change of critical H-L mass ratio for their emergence and momentum-space distribution. Importantly, we find that a finite effective range will not alter their critical mass ratios in the weak coupling regime. There, we establish an effective 2D model to quantitatively reproduce the properties of q2D clusters, and further identify the optimal interaction strengths for their detections in experiments. Our results suggest a promising prospect for observing universal clusters and associated high-order correlation effects in realistic q2D ultracold Fermi mixtures. Published by the American Physical Society 2024