We report on the development of an advanced ultracold dysprosium apparatus, which incorporates a cold atom microscope (CAM) with a design resolution of a quarter micrometer. The CAM and the cooling and trapping regions are within the same vacuum glass vessel ensuring simple atom transport between them. We demonstrate the essential experimental steps of laser and evaporative cooling, lattice loading, transporting, and precise positioning of a cloud of the bosonic isotope $^{164}\mathrm{Dy}$ at the CAM focal plane. Basic characterization of the CAM and future plans in enabling its full capacity are outlined. We also present a feasible platform for simulating complex spin models of quantum magnetism, such as the XYZ model, by exploiting a set of closely spaced opposite parity levels in Dy with a large magnetic and electric dipole moment. We isolate a degenerate isospin-1/2 system, which possesses both magnetic and electric dipole-dipole coupling, containing Ising, exchange, and spin-orbit terms. The last gives rise to a spin model with asymmetric tunable rates that depend on the lattice geometry.
We report on the development of an advanced ultracold dysprosium apparatus, which incorporates a cold atom microscope (CAM) with a design resolution of a quarter micrometer. The CAM and the cooling and trapping regions are within the same vacuum glass vessel ensuring simple atom transport between them. We demonstrate the essential experimental steps of laser and evaporative cooling, lattice loading, transporting, and precise positioning of a cloud of the bosonic isotope 164Dy at the CAM focal plane. Basic characterization of the CAM and future plans in enabling its full capacity are outlined. We also present a feasible platform for simulating complex spin models of quantum magnetism, such as the XYZ model, by exploiting a set of closely spaced opposite parity levels in Dy with a large magnetic and electric dipole moment. We isolate a degenerate isospin-1/2 system, which possesses both magnetic and electric dipole-dipole coupling, containing Ising, exchange, and spin-orbit terms. The last gives rise to a spin model with asymmetric tunable rates that depend on the lattice geometry.
Laser cooling and trapping of the most magnetic fermionic atom, dysprosium (Dy), may provide a framework to explore quantum liquid crystal (QLC) theory (Chapter 1). This thesis presents details of the Dy laser cooling and trapping apparatus including the laser systems at 421, 741, and 1064 nm, the ultra-high vacuum (UHV) chamber, and the computer control that has produced a magneto-optically (MOT) and magneto-statically (MT) trapped Dy gas (Chapters 3, 4, 5). Despite the fact that Dy has a complex energy level structure with nearly 140 metastable states (Chapter 2), Dy MOT at 421-nm transition with 32-MHz linewidth was realized without any rempumper, exploiting its large magnetic moment, which brought a strong magnetic confinement of metastable states of Dy. This unique MOT/MT dynamics is discussed and its quantitative measurements are shown in Chapter 6. When the Dy atoms dropped from the MOT were adsorptively imaged, it was observed that Dy MOT had a bimodal temperature distribution in contrast to the usual MOT described by a single temperature (Chapter 7). Such novel anisotropic sub-Doppler laser cooling of Dy, which breaks the symmetry in cooling, is due to Dy's large magnetic spin aligned along a strong axis of the quadrupole field of the MOT, and we further support this plausible conjecture with the velocity selective resonance (VSR) theory. The MOT at ~ 1 mK was cooled to ~ 10 uK by narrow-line cooling at 741 nm with a linewidth of 2 kHz, and we were able to load the optical dipole trap (ODT) at 1064 nm. By loading two isotopes of 164Dy and 163Dy in sequence to the MOT and narrow-line cooling them simultaneously, ultracold Bose-Fermi mixtures of Dy in the ODT were realized (Chapter 8). This thesis is concluded with a discussion of prospect on the Bose-Fermi mixtures of Dy.
Ultracold dysprosium gases, with a magnetic moment 10 times that of alkali atoms and equal only to terbium as the most magnetic atom, are expected to exhibit a multitude of fascinating collisional dynamics and quantum dipolar phases, including quantum liquid crystal physics. We report the first laser cooling and trapping of half a billion Dy atoms using a repumper-free magneto-optical trap (MOT) and continuously loaded magnetic confinement, and we characterize the trap recycling dynamics for bosonic and fermionic isotopes. The first inelastic collision measurements in the few partial wave, 100 microK-1 mK, regime are made in a system possessing a submerged open electronic f shell. In addition, we observe unusual stripes of intra-MOT <10 microK sub-Doppler cooled atoms.
This thesis describes and characterizes a setup to conduct experiments combining the fields of cold atoms and nanophotonics. Furthermore, a series of numerical simulations is employed to deepen of atom transport under experimentally realistic conditions. The study of cold atoms is usually fundamental in nature and a very clean approach to investigate the laws of physics. High purity samples of atoms are cooled down to millikelvins or microkelvins. The potential landscape for the atoms can be carefully controlled using lasers and/or magnetic fields. Since the atoms' responses to electric, magnetic or electromagnetic fields are known with very high fidelity, any deviations to the state the atoms are prepared in can be precisely measured. Nanophotonics is the study of light close to or beyond the diffraction limit. In this region the field-like nature of light starts to play a role. By confining light in sub-wavelength-sized structures, high peak intensities can be achieved, giving rise to exciting non-linear optics phenomena. The strong field gradient that can be created allows, for instance, precise spectroscopy measurements, phase-sensitive sub-wavelength microscopy, as well as producing highly receptive sensing devices. Combining cold atoms and nanophotonics creates strong synergy effects. It gives access to strong coupling of light and matter. The scalability of nanophotonics now extends to atomic physics. Atoms can be trapped, coupled and manipulated at very small length scales, and in large numbers. Moreover, the potential landscape for atoms is highly customizable. The rubidium isotope 87 is used in this setup. A cloud of rubidium atoms is gathered and cooled in a two dimensional magneto-optical trap (MOT). Since the atoms are only cooled in two dimensions, they are free to escape in the third dimension and load a following three dimensional MOT. The atoms are now cooled further, compressed and loaded into an optical dipole trap. This dipole trap transports the atoms close to a sample inside the vacuum chamber. A moving optical lattice, or optical conveyor belt, brings the atoms then close to the sample surface. Now experiments can be conducted, studying the interaction of cold atoms and strongly confined light. The atom transport down to the sample surface shows some unexpected behaviour: the atoms seem to spread through the optical lattice during transport. A combination of microscopic and macroscopic numerical simulations, including genetic algorithms, are used to deepen our understanding of the underlying physics. This also allows us to get access to experimental variables that cannot be directly obtained.
The laser cooling and trapping of ultracold neutral dysprosium has been demonstrated recently using the broad, open, 421-nm cycling transition. Narrow-line magneto-optical trapping of Dy on longer wavelength transitions would enable the preparation of ultracold Dy samples suitable for loading optical dipole traps and subsequent evaporative cooling. We have identified the closed 741-nm cycling transition as a candidate for the narrow-line cooling of Dy. We present experimental data on the isotope shifts, the hyperfine constants A and B, and the decay rate of the 741-nm transition. In addition, we report a measurement of the 421-nm transition's linewidth, which agrees with previous measurements. We summarize the laser-cooling characteristics of these transitions as well as other narrow cycling transitions that may prove useful for cooling Dy.
This thesis explores the development and application of laser-cooled mercury atoms for precision measurements relevant to fundamental physics. A primary motivation is the search for a permanent electric dipole moment in mercury, that could shed light on the baryon asymmetry of the universe. We present the design and construction of a custom experimental apparatus for producing and trapping cold mercury atoms, detailing challenges associated with working with mercury in an ultra-high vacuum environment and considering deep-ultraviolet optics. A magneto-optical trap operating on the 1S0-3P1 intercombination line at 254 nm is realized for all seven stable isotopes, achieving atom numbers up to 5x107 and phase-space densities up to 1x10-6 suitable for optical dipole trap loading. Cooling efficiency for all bosonic and fermionic isotopes are characterized over a wide parameter space, and we show sub-Doppler cooling in 199Hg and 201Hg. The successful loading of mercury into a high-power optical dipole trap is demonstrated, forming the basis for future electric dipole moment experiments of laser cooled mercury atoms. Prospects of evaporatively cooling mercury down to quantum degeneracy could allow for a quantum-enhanced metrology tool kit for the planned measurements. Apart from this, we are exploring the use of ultracold fermionic gases made of mercury as a quantum simulator for impurity physics. As a promising versatile and tunable platform for studying impurity-bath interactions, we are assessing the feasibility of observing Friedel oscillations in ultracold quantum gases.Further, we perform precision isotope shift spectroscopy on several dipole-allowed atomic transitions in mercury. Via King plot analysis this allows investigations of the mercury nuclear structure – also relevant for electric dipole moment bounds – and lays the foundation for probing a potential fifth force carrier coupling electrons to neutrons. We also propose upgrades to the machine for improvements in laser cooling, extensions of the spectroscopy search and a proposed experimental setup for probing the atomic electric dipole moment in an optical dipole trap of cold mercury atoms.
Ultracold mixture experiments hold the promise of providing new insights into many-body quantum systems as well as ultracold chemistry and few-body phenomena. The work presented in this thesis dealt with the construction of a new apparatus for the production and study of ultracold gases of fermionic lithium-6 and bosonic caesium-133. These isotopes offer a wide tunability in their interaction strength, both in inter-species and intra-species collisions, through magnetic Feshbach resonances. Additionally, the widely different resonance frequencies of lithium and caesium enables independent control of each of the species. With this apparatus, Bose-Einstein condensates (BEC) containing 10^4 lithium Feshbach molecules are routinely produced. The cooling system for caesium has been developed in parallel and important steps towards producing ultracold caesium gases have been made. An optical dipole trap has been loaded with 2x10^6 caesium atoms and evaporative cooling towards quantum degeneracy can now be pursued. Laser, vacuum, magnetic and control systems have been developed for the implementation of this experiment. Light produced with this laser system was used to laser cool atoms, create conservative dipole traps as well as to provide means of imaging atomic clouds. Additionally, a system to produce strong magnetic fields of up to 1400 G has been established in order to exploit the wide tunability in the atomic interactions. Software that was developed for the computerised control system facilitated the coordination of all the components involved in the experimental sequence. Measurements and calculations that showcase the functionality of relevant parts of the setup are presented in this thesis. In this experiment, lithium and caesium atoms are obtained from a novel type of Zeeman slower and are loaded into a magneto-optical trap (MOT). The system is capable of doing this independently for each of the atomic species as well as sequentially. After the MOT has been loaded with atoms, they are transferred into a conservative far-off-resonance optical dipole trap. By adjusting the interactions between atoms and lowering the depth of the dipole trap, efficient evaporative cooling of lithium was carried out from which a molecular BEC was obtained. Time-of-flight measurements were used to characterise the condensate and study its expansion dynamics.