This work explores the possibility of creating and controlling unconventional nonlinearities by periodic driving, in a broad class of systems described by the nonlinear Schrödinger equation (NLSE).By means of a parent quantum many-body description, we demonstrate that such driven systems are well captured by an effective NLSE with emergent nonlinearities, which can be finely controlled by tuning the driving sequence.We first consider a general class of two-mode nonlinear systems-relevant to optical Kerr cavities, waveguides, and Bose-Einstein condensates-where we find an emergent four-wave mixing nonlinearity, which originates from pair-hopping processes in the parent quantum picture.Tuning this drive-induced nonlinearity is shown to modify the phase-space topology, which can be detected through relative population and phase measurements, and also leads to enhanced quantum properties such as spin squeezing.We then couple individual (two-mode) dimers in view of designing extended lattice models with unconventional nonlinearities and controllable pair-hopping processes.Following this general dimerization construction, we obtain an effective lattice model with drive-induced interactions, whose ground state exhibits orbital order, chiral currents, and emergent magnetic fluxes through the spontaneous breaking of time-reversal symmetry.We analyze these intriguing properties both in the weakly interacting (mean-field) regime, captured by the effective NLSE, and in the strongly correlated quantum regime.Our general approach opens a route for the engineering of unconventional optical nonlinearities in photonic devices and controllable drive-induced interactions in ultracold quantum matter.
This work explores the possibility of creating and controlling unconventional nonlinearities by periodic driving, in a broad class of systems described by the nonlinear Schrödinger equation (NLSE).By means of a parent quantum many-body description, we demonstrate that such driven systems are well captured by an effective NLSE with emergent nonlinearities, which can be finely controlled by tuning the driving sequence.We first consider a general class of two-mode nonlinear systems-relevant to optical Kerr cavities, waveguides, and Bose-Einstein condensates-where we find an emergent four-wave mixing nonlinearity, which originates from pair-hopping processes in the parent quantum picture.Tuning this drive-induced nonlinearity is shown to modify the phase-space topology, which can be detected through relative population and phase measurements, and also leads to enhanced quantum properties such as spin squeezing.We then couple individual (two-mode) dimers in view of designing extended lattice models with unconventional nonlinearities and controllable pair-hopping processes.Following this general dimerization construction, we obtain an effective lattice model with drive-induced interactions, whose ground state exhibits orbital order, chiral currents, and emergent magnetic fluxes through the spontaneous breaking of time-reversal symmetry.We analyze these intriguing properties both in the weakly interacting (mean-field) regime, captured by the effective NLSE, and in the strongly correlated quantum regime.Our general approach opens a route for the engineering of unconventional optical nonlinearities in photonic devices and controllable drive-induced interactions in ultracold quantum matter.
Subjecting a physical system to a time-periodic drive can substantially modify its properties and applications. This Floquet-engineering approach has been extensively applied to a wide range of classical and quantum settings in view of designing synthetic systems with exotic properties. Considering a general class of two-mode nonlinear optical devices, we show that effective optical nonlinearities can be created by subjecting the light field to a repeated pulse sequence, which couples the two modes in a fast and time-periodic manner. The strength of these drive-induced optical nonlinearities, which include an emerging four-wave mixing, can be varied by simply adjusting the pulse sequence. This leads to topological changes in the system's phase space, which can be detected through light intensity and phase measurements. Our proposal builds on an effective-Hamiltonian approach, which derives from a parent quantum many-body Hamiltonian describing driven interacting bosons. As a corollary, our results equally apply to Bose-Einstein condensates in driven double-well potentials, where pair tunneling effectively arises from the periodic pulse sequence. Our scheme offers a practical route to engineer and finely tune exotic nonlinearities and interactions in photonics and ultracold quantum gases.
Controlling and stabilising collective phases of many-body quantum systems is a problem of deep fundamental and technological interest. In this thesis, we perform a theoretical investigation on how useful quantum phases may be engineered in strongly correlated fermionic lattice systems, especially through periodic driving. We first compute the phase diagram of the one-dimensional t–J model with the addition of non-standard pair hopping terms. We show that at dilute fillings these terms enhance superconductivity while, counter- intuitively, suppressing it at large fillings. We argue that this is due to dynamical constraints originating from the fact that local pairs cannot overlap. We conjecture that these constraints may play a more significant role in the physics of two-dimensional systems where the t–J model is studied as a candidate model of high-Tc superconductivity. We begin to investigate these dynamical constraints on a ladder geometry. We then study the fermionic Hubbard model under periodic driving. We show that the driving induces a strong and robust singlet-pairing effect consistent with a superconducting state. This could provide a new mechanism for light-induced superconductivity in some classes of strongly cor- related materials. We show using Floquet theory that the dynamics of the driven Hubbard model are described precisely by the t–J model studied in the previous section. As the driven Hubbard model is also implementable with ultracold fermions in an optical lattice, our results could lead to their use as a quantum simulator for a broad class of candidate models for high-Tc superconductivity.
In this thesis, we theoretically investigate exotic quantum phenomena underlying periodically-driven systems.We discuss three distinct systems, noninteracting Dirac systems, lattice systems with a strong repulsive interaction, and lattice systems with a strong attractive interaction.We reveal various novel phenomena underlying these systems, and provide clear understanding of them.Periodically-driven systems, i.e., systems with a discrete time-translational symmetry, are described by the Floquet formalism, which maps the time-dependent Hamiltonian to a static "photon-dressed Hamiltonian".While a perturbative expansion of this Hamiltonian from the limit of high driving frequency has clarified various novel phenomena peculiar to periodically-driven systems, such an approach suffers from serious heating or damage when it is applied to realistic condensed matters.In this thesis, we focus on a lower-frequency regime, especially when the heating should be suppressed due to the small driving amplitude or an energy gap larger than the driving frequency.There, the high-frequency expansion cannot capture the relevant physics, so that we first formulate various perturbative expansions for three distinct regimes, i.e., high-frequency, small-amplitude, and strong-coupling regimes.We apply the small-amplitude expansion to two-and three-dimensional Dirac electrons driven by a circularly-polarized light to explore their behavior in the lowfrequency regime.We find an emergence of infinite numbers of topological gaps for the former and Weyl nodes for the latter.We also discuss how a regularization of the model affects this topological structure.We then introduce a strong repulsive interaction, and discuss behaviors of spins using the strong-coupling expansion.We predict an emergence of scalar spin chirality when a circularly-polarized light is illuminated, and discuss possible applications to photo-induced chiral spin liquids, and optical probing of spin chirality.Finally we turn to a strong attractive interaction to discuss the fate of the ordinary s-wave superconductivity under the periodic driving.We demonstrate an emergence of long sought-after η-pairing superconductivity, first as a ground state of the photon-dressed Hamiltonian, and then as a consequence of a dynamical phase transition in an isolated system such as an optical lattice system.
This thesis reports on the realization of Floquet topological systems with ultracold atoms in an optical honeycomb lattice. Using periodically driven quantum systems, topological phases of matter can be simulated by an effective, static Hamiltonian related to the time-evolution at integer multiples of the driving period, which is known as Floquet engineering. However, periodic driving can also give rise to genuinely time-dependent settings without static counterparts. One example is the anomalous Floquet phase in two dimensions, in which all bulk bands have a Chern number of zero but nevertheless robust chiral edge modes appear, which would be precluded by the bulk-edge correspondence in a static system. In an optical honeycomb lattice, anomalous Floquet systems can be created by continuous, periodic modulation of the laser intensities. This driving scheme results in different topological regimes, three of which are investigated, including the anomalous Floquet phase and a Haldane-like phase. Periodically driven systems feature periodic quasienergies and can be characterized in terms of winding numbers, which count the number of chiral edge modes in each quasienergy gap. By interferometric measurements of the quasienergy gaps between the first two Floquet bands, the topological phase transitions, emerging as gap closings, are located. For periodically driven systems, a modified bulk-edge correspondence can be formulated. In particular, the change of the winding number at a phase transition is related to the sign change of the local Berry curvature. The Berry curvature at the gap closing points is probed by Hall deflection measurements to obtain the winding numbers in each of the topological regimes, revealing the existence of chiral edge modes also in a setting with smooth boundaries as used in the experiments. The measured quasienergy gaps and transverse deflections are quantitatively well described by a numerical calculation of the Floquet bandstructure that includes coupling to higher bands during the driving period. To derive the spectrum of the modulated lattice in a geometry with edges, a tight-binding description of the system is discussed. Circular phase modulation of the honeycomb lattice can also give rise to an anomalous Floquet system when inversion symmetry is broken. The topological phase diagrams and the experimental feasibility are compared for both modulation schemes. Due to the vanishing Chern numbers, the bulk states in the anomalous Floquet regime can be fully localized by a disorder potential. This could prevent heating in interacting, periodically driven systems, resulting in a many-body localized bulk coexisting with thermalizing edge states. The experimental realization of disorder and strong interactions, as well as independent probes of the edge states are investigated. Bloch band geometry can be extended to multiband systems, using Wilson lines. The possible symmetry protection of their eigenvalues is discussed, along with measurements in the optical honeycomb lattice. Moreover, the onset of heating in weakly-interacting, periodically driven systems, triggered by parametric instabilities, is studied experimentally in a one-dimensional lattice.
Controlling and manipulating complex many-body quantum systems will be a key ingredient \nfor the development of next-generation technologies. While the realisation of a \nuniversal quantum machine is still out of reach, in recent years experimental systems of \nultracold atoms have already evolved into a vivid field of research for quantum simulation. \nCrucially, such systems even allow for the successful quantum engineering of targeted \nmany-body systems by means of coherent periodic driving. The essential properties of \nthese Floquet systems encompass two main aspects: fast driving facilitates the simulation \nof effective static systems, and interactions lead to unique heating effects as energy is only \nconserved modulo the driving frequency. Within this thesis we theoretically study both \nof these aspects in respective model systems. \nIn part I of this thesis, we investigate the dynamics of excitations of a bosonic Mott \ninsulator in a designed one-dimensional Floquet system. Here, periodic driving in combination \nwith breaking all mirror symmetries of the system can induce directed motion of \nparticles. In the limit of small excitation densities, the effectively non-interacting quantum \nratchet determines the motion of holes and doublons in the Mott insulator and can in fact \nbe used to manipulate the dynamics of such. This little quantum machine can also be \nused to drive particles against an external force, where transport is possible but requires \nthe fulfilment of a commensurability condition for long times. \nIn part II, we discuss the role of interactions for periodically driven systems by means \nof a Floquet version of the Boltzmann equation. Starting from the Keldysh approach, \nwe develop this semiclassical formalism based on a clear separation of time scales. The \nresult is a description of the dynamics and the scattering of Floquet quasiparticles in \nsuch systems. Here, the property of discrete energy violation is naturally encoded in our \nformalism predicting the heating of interacting Floquet systems to infinite temperatures in \nthe long-time limit. As a first application of this approach, we investigate a cold atom setup \nrealising the Haldane model by means of periodic shaking. While homogeneous systems \nheat up globally, a confining potential evokes thermoelectric transport effects resulting \nfrom spatially dependent heating characteristics. Moreover, we show that the interplay \nof intrinsic heating, macroscopic diffusion and non-trivial topological properties of the \nHaldane model lead to an anomalous Floquet-Nernst effect, which describes anomalous \nparticle transport as the result of developing temperature gradients. \nIn part III, we elaborate on the quantum simulator aspect of ultracold atoms by providing \na theoretical framework for a possible simulation of a topological edge state in a \none-dimensional optical lattice. In this case, the one-dimensional Dirac equation with \nspatially varying mass is important, which captures the topological properties of a corresponding \nsystem of the BDI symmetry class. We analytically discuss such system and \ninvestigate the role of mean-field interaction effects. We also identify the emergence of \ndynamical instabilities in a realisation with bosonic atoms.
The non-equilibrium control of electronic properties has emerged as a transformative paradigm for engineering novel quantum phases. The most intriguing example of such a phase is light-induced superconductivity (SC) in non-superconducting materials. However, realizing unconventional SC at commensurate half-filling remains a formidable challenge even in non-equilibrium, as the regime is typically dominated by the robust stability of the antiferromagnetic (AFM) Mott insulating (MI) state. Here, we provide a novel non-equilibrium route to realize unconventional d-wave SC in a half-filled system through Floquet engineering. We analyze the periodically driven Fermi-Hubbard model on a bipartite lattice and demonstrate that a high-frequency drive can transform a weakly interacting insulator into a regime of strong correlations by the drive-induced renormalization of nearest-neighbor hopping. Furthermore, the drive induces staggered higher range hoppings that can frustrate the AFM order while simultaneously generate staggered potential that lifts the kinetic constraints inherent to the half-filled system, fostering the charge dynamics required to stabilize d-wave pairing against the competing AFM state. The resulting SC phase is protected by high-frequency prethermalization, maintaining stability over timescales exponentially large in the drive frequency. This protocol circumvents the need for chemical doping, offering a 'disorder-free' alternative for realizing unconventional pairing with direct applications in optimizing the performance of superconducting quantum computers, qubit arrays and other upcoming quantum technologies.