The ultrastrong coupling between the elementary excitations of matter and microcavity modes is studied in a fully analytical quantum-mechanical theoretical framework. The elementary excitation could be phonons, excitons, plasmons, etc. From the diagonalization of the Hamiltonian, we obtain the ground state of the polariton Hamiltonian. The ground state belongs to the Gaussian class. Using the Gaussian property, we calculate the quantum entanglement in the ground state. We use two different measures for quantum entanglement---entanglement entropy and the logarithmic negativity parameter---and obtain rather simple analytical expressions for the entanglement measures. Our findings show that the amount of quantum entanglement in the ground state is quite significant in the ultrastrong-coupling regime. It can be obtained from the measurement of the polariton frequencies.
The ultrastrong coupling between the elementary excitations of matter and microcavity modes is studied in a fully analytical quantum-mechanical theoretical framework. The elementary excitation could be phonons, excitons, plasmons, etc. From the diagonalization of the Hamiltonian, we obtain the ground state of the polariton Hamiltonian. The ground state belongs to the Gaussian class. Using the Gaussian property, we calculate the quantum entanglement in the ground state. We use two different measures for quantum entanglement---entanglement entropy and the logarithmic negativity parameter---and obtain rather simple analytical expressions for the entanglement measures. Our findings show that the amount of quantum entanglement in the ground state is quite significant in the ultrastrong-coupling regime. It can be obtained from the measurement of the polariton frequencies.
We have investigated theoretically a dissipative polariton system in the ultrastrong light-matter coupling regime without using the rotating-wave approximation on system-reservoir coupling. Photons in a cavity and excitations in matter respectively couple two large ensembles of harmonic oscillators (photonic and excitonic reservoirs). Inheriting the quantum statistics of polaritons in the ultrastrong coupling regime, in the ground state of the whole system, the two reservoirs are not in the vacuum states but they are squeezed and correlated. We presume the reservoirs to be in this nonvacuum state in the master equation and in the input-output formalism with Langevin equations. Both approaches consistently guarantee the decay of the polariton system to its ground state; no photon detection is also obtained when the polariton system is in the ground state.
We develop a microscopic quantum theory of surface plasmon polaritons valid for arbitrary metal-dielectric geometries. Our framework is based on the Power-Zienau-Woolley representation of quantum electrodynamics, which provides an optimal separation between electronic and photonic degrees of freedom and is therefore particularly well suited for constructing quantum descriptions of polaritonic excitations in strongly dispersive media. Within this formulation, the fundamental electronic oscillator is identified as the bulk plasmon mode, which is nonperturbatively coupled to the radiative continuum of free photon modes. This coupling induces a geometry-dependent renormalization of the bulk plasma frequency, giving rise to confined plasmonic resonances. As specific applications, we recover the localized surface plasmon modes of metallic nanoparticles, including radiative frequency shifts and decay, as well as the exact dispersion relation of propagating surface plasmon polaritons at planar interfaces. Our quantum treatment further reveals that light-matter interactions at metal-dielectric interfaces are inherently in the ultrastrong coupling regime. As a result, in the quasistatic limit, the system exhibits unconventional ground-state quantum fluctuations that can be controlled through the refractive index. These results open new intriguing perspectives in the field of quantum plasmonics.
We study theoretically the entanglement of two-photon states in the ground state of the intersubband cavity system, i.e., the so-called polariton vacuum. The system consists of a sequence of doped quantum wells located inside a microcavity and the photons can interact with intersubband excitations inside the quantum wells. Using an explicit solution for the ground state of the system, operated in the ultrastrong-coupling regime, a postselection is introduced, where only certain two-photon states are considered and analyzed for mode entanglement. We find that a fast quench of the coupling creates entangled photons and that the degree of entanglement depends on the absolute values of the in-plane wave vectors of the photons. Maximally entangled states can be generated by choosing the appropriate modes in the postselection.
Ultrastrong coupling between light and matter has, in the past decade, transitioned from a theoretical idea to an experimental reality. It is a new regime of quantum light–matter interaction, which goes beyond weak and strong coupling to make the coupling strength comparable to the transition frequencies in the system. The achievement of weak and strong coupling has led to increased control of quantum systems and to applications such as lasers, quantum sensing, and quantum information processing. Here we review the theory of quantum systems with ultrastrong coupling, discussing entangled ground states with virtual excitations, new avenues for nonlinear optics, and connections to several important physical models. We also overview the multitude of experimental setups, including superconducting circuits, organic molecules, semiconductor polaritons, and optomechanical systems, that have now achieved ultrastrong coupling. We conclude by discussing the many potential applications that these achievements enable in physics and chemistry.
We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultrastrong light-matter coupling regime, in which the vacuum Rabi frequency is a significant fraction of the active electronic transition frequency and the antiresonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. In the case of a time-independent vacuum Rabi frequency, exact analytical expressions for the operators are obtained, which allows us to characterize the quantum dissipative response of the cavity to an arbitrary initial condition (vacuum, coherent field, thermal excitation). For a vacuum input in both the photonic and electronic polarization modes, the ground state of the cavity system is a two-mode squeezed vacuum state with a finite population in both photonic and electronic modes. These excitations are, however, virtual and cannot escape from the cavity: for a vacuum input, a vacuum output is found, without any trace of the intracavity squeezing. For a coherent photonic input the linear optical response spectra (reflectivity, absorption, transmission) have been studied, and signatures of the ultrastrong coupling have been identified in the asymmetric and peculiar anticrossing of the polaritonic eigenmodes. Finally, we have calculated the electroluminescence spectra in the case of an incoherent electronic input: the emission intensity in the ultrastrong coupling regime results in being significantly enhanced as compared to the case of an isolated quantum well without a surrounding cavity.
In recent years, the study of entanglement properties of quantum field theories has led to deep insights in fields as diverse as quantum gravity and condensed matter physics. Originating as effective field theories for certain quantum dimer models, the Quantum Lifshitz Model (QLM) and its generalizations are bosonic quantum field theories with anisotropic scaling symmetry between space and time. Being closely related to conformal field theories, they provide a fruitful playground, where diverse entanglement calculations can be performed analytically. \n \nIn this thesis, we concentrate on two entanglement measures, the entanglement entropy and logarithmic negativity. Motivated to extract sub-leading universal behavior, we perform analytic calculations in two and higher even dimensions. In order to make the calculations tractable, we put the QLM on compact manifolds, such as spheres and tori, where the spectrum of a certain operator appearing in the ground state of the theory is explicitly known. Mostly by means of the replica method, we then find analytic expressions for the finite sub-leading terms of the entanglement entropy and logarithmic negativity of the ground state, as well as the entanglement entropy of the excited states of the QLM. In the case of the ground state entanglement entropy, we provide analytic expressions for the sub-leading terms as functions of the dimension and the dynamical critical exponent. For the excited states we provide analytic formulae of the sub-leading coefficients as functions of the excitation numbers.