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arXiv:2303.11458 · Nature Communications

A chip-scale atomic beam clock

Gabriela D. Martinez, Chao Li, Alexander L. Staron, John E. Kitching, Chandra Raman, William McGehee

Published Jun 13, 2023• 68 citations
arXivHTMLPDF

Abstract

Abstract Atomic beams are a longstanding technology for atom-based sensors and clocks with widespread use in commercial frequency standards. Here, we report the demonstration a chip-scale microwave atomic beam clock using coherent population trapping (CPT) interrogation in a passively pumped atomic beam device. The beam device consists of a hermetically sealed vacuum cell fabricated from an anodically bonded stack of glass and Si wafers. Atomic beams are created using a lithographically defined microcapillary array connected to a Rb reservoir1 and propagate in a 15 mm long drift cavity. We present a detailed characterization of the atomic beam performance (total Rb flux ≈ 7.7 × 1011 s-1 at 363 K device temperature) and of the vacuum environment in the device (pressure < 1 Pa), which is sustained using getter materials which pump residual gases and Rb vapor. A chip-scale beam clock is realized using Ramsey CPT spectroscopy of the 87Rb ground state hyperfine transition over a 10 mm Ramsey distance in the atomic beam device. The prototype atomic beam clock demonstrates a fractional frequency stability of ≈ 1.2 × 10-9/√τ for integration times τ from 1 s to 250 s, limited by detection noise. Optimized atomic beam clocks based on this approach may exceed the long-term stability of existing chip-scale clocks, and leading long-term systematics are predicted to limit the ultimate fractional frequency stability below 10-12.

DOI
10.1038/s41467-023-39166-1

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•Apr 14, 2019•0 citations
Abstract Atomic beams are a longstanding technology for atom-based sensors and clocks with widespread use in commercial frequency standards. Here, we report the demonstration a chip-scale microwave atomic beam clock using coherent population trapping (CPT) interrogation in a passively pumped atomic beam device. The beam device consists of a hermetically sealed vacuum cell fabricated from an anodically bonded stack of glass and Si wafers. Atomic beams are created using a lithographically defined microcapillary array connected to a Rb reservoir1 and propagate in a 15 mm long drift cavity. We present a detailed characterization of the atomic beam performance (total Rb flux ≈ 7.7 × 1011 s-1 at 363 K device temperature) and of the vacuum environment in the device (pressure < 1 Pa), which is sustained using getter materials which pump residual gases and Rb vapor. A chip-scale beam clock is realized using Ramsey CPT spectroscopy of the 87Rb ground state hyperfine transition over a 10 mm Ramsey distance in the atomic beam device. The prototype atomic beam clock demonstrates a fractional frequency stability of ≈ 1.2 × 10-9/√τ for integration times τ from 1 s to 250 s, limited by detection noise. Optimized atomic beam clocks based on this approach may exceed the long-term stability of existing chip-scale clocks, and leading long-term systematics are predicted to limit the ultimate fractional frequency stability below 10-12.
We report on progress in the characterization of systematic shifts in chip-scale atomic beam clocks, which offer the potential for improved long-term stability relative to existing chip-scale atomic clocks. Previous work has demonstrated the key features of chip-scale atomic beam devices including the use of a microfabricated Si/glass atomic beam cell, passively maintained vacuum environment, and an integrated Rb atomic beam source. A beam clock has been realized using Ramsey coherent population trapping interrogation with a demonstrated short-term fractional frequency stability of ≈ 1.2 × 10^(-9)at 1 s of integration. In this talk, we discuss the path toward long-term stabilty in chip-scale atomic beam clocks and leading clock systematics. Chip-scale atomic beams are a new platform for quantum sensing which offer the potential for long-term stability in compact, low-power applications.
We present a coherent population trapping clock system based on laser-cooled 87Rb atoms. The clock consists of a frequency-stabilized CPT interrogation laser and a cooling laser as well as a compact magneto-optical trap, a high-performance microwave synthesizer, and a signal detection system. The resonance signal in the continuous wave regime exhibits an absorption contrast of ∼ 50%. In the Ramsey interrogation method, the linewidth of the central fringe is 31.25 Hz. The system achieves fractional frequency stability of 2.4 × 10 − 11 / τ , which goes down to 1.8 × 10−13 at 20000 s. The results validate that cold atom interrogation can improve the long-term frequency stability of coherent population trapping clocks and holds the potential for developing compact/miniature cold atoms clocks.
We investigate the application of Ramsey spectroscopy for the development of a microcell atomic clock based on coherent population trapping (CPT). The dependence of the central Ramsey-CPT fringe properties on key experimental parameters is first studied for optimization of the clock’s short-term frequency stability. The sensitivity of the clock frequency to light-shift effects is then studied. In comparison with the continuous-wave (CW) regime case, the sensitivity of the clock frequency to laser power variations is reduced by a factor up to 14 and 40.3 for dark times of 150 and450 μs450~\mu \text{s}450 μs, respectively, at the expense of intensity 3.75 times higher for short-term stability optimization. The dependence of the clock frequency on the microwave power is also reduced in the Ramsey case. We demonstrate that the Ramsey-CPT interrogation improves the clock Allan deviation for averaging times higher than 100 s. With a dark time of450 μs450~\mu \text{s}450 μs, a clock fractional frequency stability of3.8×10−123.8 \times 10^{-12}3.8×10−12at 104s is obtained, in comparison with the level of8×10−118\times 10^{-11}8×10−11obtained in the standard CW case, in similar environmental conditions. These results demonstrate that Ramsey-based interrogation protocols might be an attractive approach for the development of chip-scale atomic clocks (CSACs) with enhanced mid- and long-term stability.
We demonstrate a microfabricated atomic clock physics package based on coherent population trapping (CPT) on the D1 line of 87Rb atoms. The package occupies a volume of 12 mm3 and requires 195 mW of power to operate at an ambient temperature of 200 degrees C. Compared to a previous microfabricated clock exciting the D2 transition in Cs [1], this 87Rb clock shows significantly improved short- and long-term stability. The instability at short times is 4 x?10-11 / tau?/2 and the improvement over the Cs device is due mainly to an increase in resonance amplitude. At longer times (tau?> 50 s), the improvement results from the reduction of a slow drift to ?5 x 10-9 / day. The drift is most likely caused by a chemical reaction of nitrogen and barium inside the cell. When probing the atoms on the D1 line, spin-exchange collisions between Rb atoms and optical pumping appear to have increased importance compared to the D2 line.
We demonstrate a vapor-cell atomic-clock prototype based on a continuous-wave interrogation and double-modulation coherent population trapping (DM-CPT) technique. The DM-CPT technique uses a synchronous modulation of polarization and the relative phase of a bichromatic laser beam in order to increase the number of atoms trapped in a dark state, i.e., a nonabsorbing state. The narrow resonance, observed in the transmission of a Cs vapor cell, is used as a narrow frequency discriminator in an atomic clock. A detailed characterization of the CPT resonance versus numerous parameters is reported. A short-term fractional-frequency stability of 3.2×10−13τ−1/2 up to a 100-s averaging time is measured. These performances are more than one order of magnitude better than industrial Rb clocks and are comparable to those of the best laboratory-prototype vapor-cell clocks. The noise-budget analysis shows that the short- and midterm frequency stability is mainly limited by the power fluctuations of the microwave used to generate the bichromatic laser. These preliminary results demonstrate that the DM-CPT technique is well suited for the development of a high-performance atomic clock, with the potential compact and robust setup due to its linear architecture. This clock could find future applications in industry, telecommunications, instrumentation, or global navigation satellite systems.