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arXiv:2302.14774 · Physical Review A

Quantum simulation of the central spin model with a Rydberg atom and polar molecules in optical tweezers

Jacek Dobrzyniecki, Michał Tomza

Published Nov 28, 2023• 13 citations
arXivHTMLPDF

Abstract

Central spin models, where a single spinful particle interacts with a spin environment, find wide application in quantum information technology and can be used to describe, e.g., the decoherence of a qubit over time. We propose a method of realizing an ultracold quantum simulator of a central spin model with $XX$ (spin-exchanging) interactions. The proposed system consists of a single Rydberg atom (central spin) and surrounding polar molecules (bath spins), coupled to each other via dipole-dipole interactions. By mapping internal particle states to spin states, spin-exchanging interactions can be simulated. As an example system geometry, we consider a ring-shaped arrangement of bath spins and show how it allows us to exact precise control over the interaction strengths. We numerically analyze two example dynamical scenarios which can be simulated in this setup: a decay of central spin polarization, which can represent qubit decoherence in a disordered environment, and a transfer of an input spin state to a specific output spin, which can represent the transmission of a single bit across a quantum network. We demonstrate that this setup allows us to realize a central spin model with highly tunable parameters and geometry for applications in quantum science and technology.

DOI
10.1103/physreva.108.052618

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We propose a scheme for constructing versatile quantum simulators using ultracold Rydberg atoms in long-lived circular and elliptical states. By exciting different subspaces of internal atomic states, the atoms can be used to simulate two effective spin species with different spin-spin interactions. The strengths of transverse and longitudinal spin-spin interactions, both intra- and interspecies, can be controlled within a wide range of values. This setup can be used to simulate two-species spin models or lattice models with two sublattices. We show examples of specific models which can be realized.
Single atoms in dipole microtraps or optical tweezers have recently become a promising platform for quantum computing and simulation. Here we report a detailed theoretical analysis of the physics underlying an implementation of a Rydberg two-qubit gate in such a system---a cornerstone protocol in quantum computing with single atoms. We focus on a blockade-type entangling gate and consider various decoherence processes limiting its performance in a real system. We provide numerical estimates for the limits on fidelity of the maximally entangled states and predict the full process matrix corresponding to the noisy two-qubit gate. We consider different excitation geometries and show certain advantages for the gate realization with linearly polarized driving beams. Our methods and results may find implementation in numerical models for simulation and optimization of neutral atom based quantum processors.
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Ultracold molecules are attractive candidates for various applications including ultracold chemistry, quantum information processing, quantum simulation and searches for physics beyond the standard model. Combined with optical tweezer techniques, an optical tweezer array of ultracold polar molecules holds promise for versatile quantum applications. Their long-lived molecular rotational states form robust qubits, while the long-range dipolar interaction between molecules provides quantum entanglement. In this thesis, we build a new generation experiment of optical tweezer array of ultracold CaF molecules. We optically transport the laser cooled and optically trapped molecules into a science glass cell using a hybrid method, where high numerical aperture optical access allows for tighter optical tweezers. In an array of these tight optical tweezers, we demonstrate dipolar spin-exchange interactions between single CaF molecules for the first time. We realize the spin-12\frac{1}{2}21​ quantum XY model by encoding an effective spin-12\frac{1}{2}21​ system into the rotational states of the molecules, and use it to generate a Bell state through an iSWAP operation. Conditioned on the verified existence of molecules in both tweezers at the end of the measurement, we obtain a Bell state fidelity of 0.89(6). Employing interleaved tweezer arrays, we demonstrate single site molecular addressability. To further improve the platform, cooling of the molecules to near the motional ground state is crucial for reducing various dephasings. We demonstrate Raman sideband cooling (RSC) of CaF molecules in optical tweezers to near their 3-D motional ground state, with a 3-D motional ground state probability of 54±18%54\pm18\%54±18% of the molecules that survive the RSC. This paves the way to increase molecular coherence times in optical tweezers for robust quantum information processing and simulation applications in the near future.
We consider dynamics of a Rydberg impurity in a cloud of ultracold bosonic atoms in which the Rydberg electron undergoes spin-changing collisions with surrounding atoms. This system realizes a new type of quantum impurity problems that compounds essential features of the Kondo model, the Bose polaron, and the central spin model. To capture the interplay of the Rydberg-electron spin dynamics and the orbital motion of atoms, we employ a new variational method that combines an impurity-decoupling transformation with a Gaussian ansatz for the bath particles. We find several unexpected features of this model that are not present in traditional impurity problems, including interaction-induced renormalization of the absorption spectrum that eludes simple explanations from molecular bound states, and long-lasting oscillations of the Rydberg-electron spin. We discuss generalizations of our analysis to other systems in atomic physics and quantum chemistry, where an electron excitation of high orbital quantum number interacts with a spinful quantum bath.