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arXiv:1905.08523 · Physical Review Letters

Quantum Rydberg Central Spin Model

Yuto Ashida, Tao Shi, Richard Schmidt, H. R. Sadeghpour, J. I. Cirac, Eugene Demler

Published Oct 31, 2019• 37 citations
arXivHTMLPDF

Abstract

We consider dynamics of a Rydberg impurity in a cloud of ultracold bosonic atoms in which the Rydberg electron undergoes spin-changing collisions with surrounding atoms. This system realizes a new type of quantum impurity problems that compounds essential features of the Kondo model, the Bose polaron, and the central spin model. To capture the interplay of the Rydberg-electron spin dynamics and the orbital motion of atoms, we employ a new variational method that combines an impurity-decoupling transformation with a Gaussian ansatz for the bath particles. We find several unexpected features of this model that are not present in traditional impurity problems, including interaction-induced renormalization of the absorption spectrum that eludes simple explanations from molecular bound states, and long-lasting oscillations of the Rydberg-electron spin. We discuss generalizations of our analysis to other systems in atomic physics and quantum chemistry, where an electron excitation of high orbital quantum number interacts with a spinful quantum bath.

DOI
10.1103/physrevlett.123.183001

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We consider dynamics of a Rydberg impurity in a cloud of ultracold bosonic atoms in which the Rydberg electron undergoes spin-changing collisions with surrounding atoms. This system realizes a new type of quantum impurity problems that compounds essential features of the Kondo model, the Bose polaron, and the central spin model. To capture the interplay of the Rydberg-electron spin dynamics and the orbital motion of atoms, we employ a new variational method that combines an impurity-decoupling transformation with a Gaussian ansatz for the bath particles. We find several unexpected features of this model that are not present in traditional impurity problems, including interaction-induced renormalization of the absorption spectrum that eludes simple explanations from molecular bound states, and long-lasting oscillations of the Rydberg-electron spin. We discuss generalizations of our analysis to other systems in atomic physics and quantum chemistry, where an electron excitation of high orbital quantum number interacts with a spinful quantum bath.
We investigate the absorption spectrum of a Rydberg impurity immersed in and interacting with an ideal Bose-Einstein condensate. Here, the impurity-bath interaction range can greatly exceed the mean interparticle distance; this discrepancy in length scales challenges the assumptions underlying the universal aspects of impurity atoms in dilute bosonic environments. Our analysis finds three distinct parameter regimes, each characterized by a unique spectral response. In the low-density regime, we find that the Rydberg impurity is dressed by the surrounding bath similarly to the known Bose polaron. Transitioning to intermediate densities, the impurity response, given by sharp quasiparticle peaks, fragments into an intricate pattern bearing the hallmarks of a diverse molecular structure. Finally, at high density, a universal Gaussian response emerges as the statistical nature of the bath dominates its quantum dynamics. We complement this analysis with a study of an ionic impurity, which behaves equivalently. Our exploration offers insights into the interplay between interaction range, density, and many-body behavior in impurity systems. Published by the American Physical Society 2024
Central spin models, where a single spinful particle interacts with a spin environment, find wide application in quantum information technology and can be used to describe, e.g., the decoherence of a qubit over time. We propose a method of realizing an ultracold quantum simulator of a central spin model with XXXXXX (spin-exchanging) interactions. The proposed system consists of a single Rydberg atom (central spin) and surrounding polar molecules (bath spins), coupled to each other via dipole-dipole interactions. By mapping internal particle states to spin states, spin-exchanging interactions can be simulated. As an example system geometry, we consider a ring-shaped arrangement of bath spins and show how it allows us to exact precise control over the interaction strengths. We numerically analyze two example dynamical scenarios which can be simulated in this setup: a decay of central spin polarization, which can represent qubit decoherence in a disordered environment, and a transfer of an input spin state to a specific output spin, which can represent the transmission of a single bit across a quantum network. We demonstrate that this setup allows us to realize a central spin model with highly tunable parameters and geometry for applications in quantum science and technology.
A versatile and efficient variational approach is developed to solve in- and out-of-equilibrium problems of generic quantum spin-impurity systems. Employing the discrete symmetry hidden in spin-impurity models, we present a new canonical transformation that completely decouples the impurity and bath degrees of freedom. Combining it with Gaussian states, we present a family of many-body states to efficiently encode nontrivial impurity-bath correlations. We demonstrate its successful application to the anisotropic and two-lead Kondo models by studying their spatiotemporal dynamics and universal behavior in the correlations, relaxation times, and the differential conductance. We compare them to previous analytical and numerical results. In particular, we apply our method to study new types of nonequilibrium phenomena that have not been studied by other methods, such as long-time crossover in the ferromagnetic easy-plane Kondo model. The present approach will be applicable to a variety of unsolved problems in solid-state and ultracold-atomic systems.
Recent work is reviewed on continuous quantum phase transitions in impurity models, both with fermionic and bosonic baths – these transitions are interesting realizations of boundary critical phenomena at zero temperature. The models with fermion bath are generalizations of the standard Kondo model, with the common feature that Kondo screening of the localized spin can be suppressed due to competing processes. The models with boson bath are related to the spin–boson model of dissipative two-level systems, where the interplay between tunneling and friction results in multiple phases. The competition inherent to all models can generate unstable fixed points associated with quantum phase transitions, where the impurity properties undergo qualitative changes. Interestingly, certain impurity transitions feature both lower-critical and upper-critical “dimensions” and allow for epsilon-type expansions. Results are presented for a number of observables, obtained by both analytical and numerical renormalization group techniques, and connections made to experiments.
We analyze the dynamics of Bose polarons in the vicinity of a Feshbach resonance between the impurity and host atoms. We compute the radio-frequency absorption spectra for the case when the initial state of the impurity is noninteracting and the final state is strongly interacting with the host atoms. We compare results of different theoretical approaches including a single excitation expansion, a self-consistent T-matrix method, and a time-dependent coherent state approach. Our analysis reveals sharp spectral features arising from metastable states with several Bogoliubov excitations bound to the impurity atom. This surprising result of the interplay of many-body and few-body Efimov type bound state physics can only be obtained by going beyond the commonly used Fröhlich model and including quasiparticle scattering processes. Close to the resonance we find that strong fluctuations lead to a broad, incoherent absorption spectrum where no quasiparticle peak can be assigned.