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arXiv:2301.10589 · Journal of Experimental and Theoretical Physics Letters

Hubbard Bands, Mott Transition and Deconfinement in Strongly Correlated Systems

V. Yu. Irkhin

Published Dec 26, 2022• 4 citations
arXivHTMLPDF

Abstract

The problem of deconfinement phases in strongly correlated systems is discussed. In space–time dimension $$d = 3 + 1$$ , a competition of confinement and Coulomb phases occurs, but in $$d = 2 + 1$$ the confining phase dominates owing to monopole proliferation, but Dirac points can change the situation. Combining the Kotliar–Ruckenstein representation and fractionalized spin-liquid deconfinement picture, the Mott transition and Hubbard subbands are treated, general expressions in the case of an arbitrary bare band spectrum being obtained. The transition into a metallic state is determined by condensation of a gapless boson mode. The spectrum picture in the insulating state is considerably influenced by the spinon spin-liquid spectrum and hidden Fermi surface.

DOI
10.1134/s002136402260269x

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The problem of deconfinement phases in strongly correlated systems is discussed. In space–time dimension d=3+1d = 3 + 1d=3+1 , a competition of confinement and Coulomb phases occurs, but in d=2+1d = 2 + 1d=2+1 the confining phase dominates owing to monopole proliferation, but Dirac points can change the situation. Combining the Kotliar–Ruckenstein representation and fractionalized spin-liquid deconfinement picture, the Mott transition and Hubbard subbands are treated, general expressions in the case of an arbitrary bare band spectrum being obtained. The transition into a metallic state is determined by condensation of a gapless boson mode. The spectrum picture in the insulating state is considerably influenced by the spinon spin-liquid spectrum and hidden Fermi surface.
I present a pedagogical survey of a variety of quantum phases of the Hubbard model. The honeycomb lattice model has a conformal field theory connecting the semi-metal to the insulator with Neel order. States with fractionalized excitations are linked to the deconfined phases of gauge theories. I also consider the confining phases of such gauge theories, and show how Berry phases of monopoles induce valence bond solid order. The triangular lattice model can display a metal-insulator transition from a Fermi liquid to a deconfined spin liquid, and I describe the theory of this transition. The bilayer triangular lattice is used to illustrate another compressible metallic phase, the `fractionalized Fermi liquid'. I make numerous connections of these phases and critical points to the AdS/CFT correspondence. In particular, I argue that two recent holographic constructions connect respectively to the Fermi liquid and fractionalized Fermi liquid phases.
An analytical solution of the Mott transition is obtained for the Hubbard model on the Bethe lattice in the large coordination number (zzz) limit. The excitonic binding of doublons (doubly occupied sites) and holons (empty sites) is shown to be the origin of a continuous Mott transition between a metal and an emergent quantum spin liquid insulator. The doublon-holon binding theory enables a different large-zzz limit and a different phase structure than the dynamical meanfield theory by allowing intersite spinon correlations to lift the 2N2^N2N-fold degeneracy of the local moments in the insulating phase. We show that the spinons are coupled to doublons/holons by a dissipative compact U(1) gauge field that is in the deconfined phase, stabilizing the spin-charge separated gapless spin liquid Mott insulator.
Abstract: The metal–insulator transition (MIT) constitutes one of the most profound and persistent problems in condensed matter physics, sitting at the intersection of electronic structure theory, many-body physics, and emergent quantum phenomena. Conventional band theory, which successfully classifies materials as metals or insulators according to the filling of their electronic bands, fails dramatically when confronted with a class of compounds transition metal oxides chief among them that ought to be metallic by band-counting arguments yet are robustly insulating in the laboratory. The resolution of this paradox required abandoning the independent-electron picture entirely and recognizing that strong Coulomb repulsion between electrons can, by itself, drive localization. This insight, formalized by Mott and later distilled into the Hubbard model, established correlation-driven insulation as a phenomenon distinct from band insulation. The present paper offers a theoretical exploration of the MIT problem, tracing its conceptual development from the Mott criterion through the Hubbard Hamiltonian, the Brinkman–Rice scenario of quasiparticle mass divergence, and the watershed development of dynamical mean-field theory (DMFT), which rendered the Mott transition quantitatively tractable for the first time. We argue that the competition between the electronic bandwidth and the on-site interaction encoded in the ratio U/W provides the unifying organizing principle for the field. Building toward the modern frontier, we examine how the Mott transition connects to quantum phase transitions and quantum criticality, where zero-temperature instabilities governed by quantum rather than thermal fluctuations produce non-Fermi-liquid behavior and anomalous scaling. Case studies of vanadium oxides, rare-earth nickelates, and doped cuprates illustrate the diversity and subtlety of real correlated materials. We conclude that the MIT remains a central and unresolved problem whose continued study is increasingly entangled with the development of quantum materials and quantum technologies. Keywords: Metal–Insulator Transition; Mott Insulator; Strongly Correlated Electrons; Hubbard Model; DMFT; Quantum Criticality; Quantum Materials; Condensed Matter Physics
We argue that the binding between doubly occupied (doublon) and empty (holon) sites governs incoherent excitations and plays a key role in the Mott transition in strongly correlated Mott-Hubbard systems. We construct a new saddle-point solution with doublon-holon binding in the Kotliar-Ruckenstein slave-boson functional integral formulation of the Hubbard model. On a half-filled honeycomb lattice and square lattice, the ground state is found to exhibit a continuous transition from a paramagnetic semimetal/metal to an antiferromagnetic-ordered Slater insulator with coherent quasiparticles at Uc1{U}_{c1}Uc1​, followed by a Mott transition into an electron-fractionalized AF∗{}^{*}∗ phase without coherent excitations at Uc2{U}_{c2}Uc2​. Such a phase structure appears to be generic for bipartite lattices without frustration. We show that doublon-holon binding unites the three important ideas of strong correlation: coherent quasiparticles, incoherent Hubbard bands, and deconfined Mott insulator.
Introduction In this chapter we study metal–insulator transitions which occur due to correlations between the charge carriers. This quantum phase transitions results from the competition between kinetic energy and Coulomb repulsion where the latter has the tendency to localise the electrons. The simplest model which describes this competition is the one-band Hubbard model with its two energy scales, the bandwidth W and the Coulomb repulsion U between electrons of opposite spins on the same site. For a fixed density of electrons, n = 1; as the ratio U/W increases, we expect to find a zero-temperature phase transition from a metallic state to an insulator where the electrons are frozen at the lattice sites. The method employed here to investigate this transition is the Gutzwiller approach (Gutzwiller, 1965). This is a variational method which played an important role in providing a framework for the ideas of Mott on the problem of the metal–insulator transition (Mott, 1974). On the metallic side of the transition, this approach describes a metal with renormalised Fermi liquid parameters, essentially with enhanced effective mass and uniform susceptibility. This is the so-called highly correlated electron gas (Brinkman and Rice, 1970) for which the metal oxide V 2 O 3 is the prototype system. In the insulating side, Gutzwiller's approximation yields a noninteracting system of localised electrons. This insulating phase is incompressible , i.e. has zero compressibility and infinite zero temperature susceptibility. The latter is not a consequence of interactions but simply due to the divergence of the Curie susceptibility, χ ∝ 1 /T , of non-interacting moments at T = 0. Then, in Gutzwiller's approach the transition is from a paramagnetic metal to a paramagnetic insulator. We will continue using the designation Mott transition to describe this type of phase transition where the insulating phase has no long-range magnetic order. In real systems, most frequently, localisation due to interactions is accompanied by the appearance of antiferromagnetic order.
We reinvestigate the bandwidth-control and doping-control Mott transitions (BCMT and DCMT) from a spin liquid Mott insulator to a Fermi liquid metal based on the slave-rotor representation of the Hubbard model [Florens and Georges, Phys. Rev. B 66, 165111 (2002); 70, 035114 (2004)] where the Mott transitions are described by softening of bosonic collective excitations. We find that the nature of the insulating phase away from half filling is different from that of half filling in the respect that a charge density wave coexists with a topological order (spin liquid) away from half filling because the condensation of vortices generically breaks translational symmetry in the presence of ``dual magnetic fields'' resulting from hole doping while the topological order remains stable owing to gapless excitations near the Fermi surface. Performing a renormalization group analysis, we discuss the role of dissipative gauge fluctuations due to the Fermi surface in both the BCMT and the DCMT.