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arXiv:2212.11445 · Science Advances

Critical fluctuations in a confined driven-dissipative quantum condensate

Hassan Alnatah, P. Comaron, Shouvik Mukherjee, Jonathan Beaumariage, Loren N. Pfeiffer, K. W. West, Kirk Baldwin, Marzena Hanna Szymańska, David W. Snoke

Published Mar 22, 2024• 14 citations
arXivHTMLPDF

Abstract

Phase fluctuations determine the low-energy properties of quantum condensates. However, at the condensation threshold, both density and phase fluctuations are relevant. While strong emphasis has been given to the investigation of phase fluctuations, which dominate the physics of the quantum system away from the critical point, number fluctuations have been much less explored even in thermal equilibrium. In this work, we report experimental observation and theoretical description of fluctuations in a circularly confined nonequilibrium Bose-Einstein condensate of polaritons near the condensation threshold. We observe critical fluctuations, which combine the number fluctuations of a single-mode condensate state and competition between different states. The latter is analogous to mode hopping in photon lasers. Our theoretical analysis indicates that this phenomenon is of a quantum character, while classical noise of the pump is not sufficient to explain the experiments. The manifestation of a critical quantum state competition unlocks possibilities for the study of condensate formation while linking to practical realizations in photonic lasers.

DOI
10.1126/sciadv.adi6762

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Phase fluctuations determine the low-energy properties of quantum condensates. However, at the condensation threshold, both density and phase fluctuations are relevant. While strong emphasis has been given to the investigation of phase fluctuations, which dominate the physics of the quantum system away from the critical point, number fluctuations have been much less explored even in thermal equilibrium. In this work, we report experimental observation and theoretical description of fluctuations in a circularly confined nonequilibrium Bose-Einstein condensate of polaritons near the condensation threshold. We observe critical fluctuations, which combine the number fluctuations of a single-mode condensate state and competition between different states. The latter is analogous to mode hopping in photon lasers. Our theoretical analysis indicates that this phenomenon is of a quantum character, while classical noise of the pump is not sufficient to explain the experiments. The manifestation of a critical quantum state competition unlocks possibilities for the study of condensate formation while linking to practical realizations in photonic lasers.
Polariton condensates provide a versatile platform for exploring non-equilibrium phase transitions and collective phenomena in open quantum systems. Near the condensation threshold, these systems are particularly sensitive to fluctuations and instabilities, yet how these dynamics govern the initial formation of the condensate remains poorly understood. To address this, we directly access the photon statistics and second-order correlation function g (2) (0) of the condensate by using optical trapping and homodyne detection. We show that polariton condensation near the threshold is not a purely static transition, but instead undergoes a dynamical regime characterized by stochastic hopping between condensed and non-condensed states. These intermittent dynamics are accompanied by a gradual reduction of g (2) (0) toward unity, revealing the progressive build-up of coherence even in the presence of strong temporal fluctuations. Numerical simulations, based on a stochastic truncated Wigner description of the driven-dissipative polariton field, reproduce these dynamics and capture the essential role of noise and reservoir interactions. This work demonstrates that the observed temporal hopping is an intrinsic feature of polariton condensation, challenging traditional static descriptions of phase transitions and offering a framework for controlling noise and coherence in driven-dissipative quantum technologies.
Polariton condensates provide a versatile platform for exploring non-equilibrium phase transitions and collective phenomena in open quantum systems. Near the condensation threshold, these systems are particularly sensitive to fluctuations and instabilities, which can strongly influence the condensate formation. Using optical trapping and homodyne detection, we directly access the photon statistics and second-order correlation function g(2)(0)g^{(2)}(0)g(2)(0) of the condensate. We show that polariton condensation near the threshold is not a purely static transition, but instead undergoes a dynamical regime characterized by stochastic hopping between condensed and non-condensed states. These intermittent dynamics are accompanied by a gradual reduction of g(2)(0)g^{(2)}(0)g(2)(0) towards unity, revealing the progressive build-up of coherence even in the presence of strong temporal fluctuations. Numerical simulations, based on a stochastic Truncated Wigner description of the driven-dissipative polariton field, reproduce these dynamics and capture the essential role of noise and reservoir interactions. This work demonstrates that the observed temporal hopping is an intrinsic feature of polariton condensation, providing a dynamical perspective that goes beyond static descriptions of the condensation phase transition.
We investigate the near-critical dynamics of atomic density fluctuations in the nonequilibrium self-organization transition of an optically driven quantum gas coupled to a single mode of a cavity. In this system cavity-mediated long-range interactions between atoms, tunable by the drive strength, lead to softening of an excitation mode recently observed in experiments. This phenomenon has previously been studied within a two-mode approximation for the collective motional degrees of freedom of the atomic condensate, which results in an effective open-system Dicke model. Here, including the full spectrum of atomic modes we find a finite lifetime for a rotonlike mode in the Bogoliubov excitation spectrum that is strongly pump dependent. The corresponding decay rate and critical exponents for the phase transition are calculated explaining the nonmonotonic pump-dependent atomic damping rate observed in recent experiments. We compute the near-critical behavior of the intracavity field fluctuations that has been previously shown to be enhanced with respect to the equilibrium Dicke model in a two-mode approximation. We highlight the role of the finite size of the system in the suppression of it below the expectations of the open Dicke model.
Systems close to a phase transition turn weak perturbations into large responses. At equilibrium, this amplification is closely linked to criticality: fluctuations grow, dynamics slow, and a common soft mode controls the response. Whether this correspondence survives in driven-dissipative quantum systems, sustained by continuous pumping and loss away from thermal equilibrium, remains an open question. Here we show experimentally that it does. In a room-temperature semiconductor photon Bose-Einstein condensate, the critical slowing of spontaneous intensity fluctuations and the amplification of weak pump perturbations are measured independently. Both peak at the same condensate population, nˉc=1250\bar{n}_c = 1250nˉc​=1250, where the dimensionless slowing factor and susceptibility reach the same value, nˉc/2=625\bar{n}_c/2 = 625nˉc​/2=625. A single weakly damped collective photon-reservoir mode governs both effects. This fluctuation-response correspondence in a finite open quantum gas establishes critical susceptibility as a measurable dynamical signature of condensation, with peak gain set by system size.
After reviewing the interpretation of laser operation as a nonequilibrium Bose-Einstein condensation phase transition, we illustrate the novel features arising from the nonequilibrium nature of photon and polariton Bose-Einstein condensates recently observed in experiments. We then propose a quantitative criterion to experimentally assess the equilibrium versus nonequilibrium nature of a specific condensation process, based on fluctuation-dissipation relations. The power of this criterion is illustrated on two models which show very different behaviors. Historical and Conceptual Introduction The first introduction of concepts of nonequilibrium statistical mechanics into the realm of optics dates back to the early 1970s with pioneering works by Graham and Haken [1] and by DeGiorgio and Scully [2], who proposed a very insightful interpretation of the laser threshold in terms of a spontaneous breaking of the U( 1 ) symmetry associated with the phase of the emitted light. Similar to what happens to the order parameter at a second-order phase transition, such an optical phase is randomly chosen every time the device is switched on and remains constant for macroscopic times. Moreover, a long-range spatial order is established, as light emitted by a laser device above threshold is phase-coherent on macroscopic distances. While textbooks typically discuss this interpretation of laser operation in terms of a phase transition for the simplest case of a single-mode laser cavity, rigorously speaking this is valid only in spatially infinite systems. In fact, only in this case one can observe nonanalytic behaviors of the physical quantities at the transition point. In particular, the long-range order is typically assessed by looking at the long-distance behavior of the correlation function of the order parameter, which, for a laser, corresponds to the first-order spatial coherence of the emitted electric field, the spontaneous symmetry breaking is signaled by this quantity becoming nonzero (see Chapter 5). The average is taken on the stationary density matrix of the system. In order to be able to probe this long-distance behavior, experimental studies need devices with a spatially extended active region.
Many bosons can occupy a single quantum state without a limit. This state is described by quantum-mechanical Bose-Einstein statistics, which allows the formation of a Bose-Einstein condensate at low temperatures and high particle densities. Photons, historically the first considered bosonic gas, were late to show this phenomenon, which was observed in rhodamine-filled microlaser cavities and doped fiber cavities. These more recent findings have raised the natural question as to whether condensation is common in laser systems, with potential technological applications. Here, we show the Bose-Einstein condensation of photons in a broad-area vertical-cavity surface-emitting laser with positive cavity mode-gain peak energy detuning. We observed a Bose-Einstein condensate in the fundamental transversal optical mode at the critical phase-space density. The experimental results follow the equation of state for a two-dimensional gas of bosons in thermal equilibrium, although the extracted spectral temperatures were lower than those of the device. This is interpreted as originating from the driven-dissipative nature of the device and the stimulated cooling effect. In contrast, non-equilibrium lasing action is observed in the higher-order modes in a negatively detuned device. Our work opens the way for the potential exploration of superfluid physics of interacting photons mediated by semiconductor optical non-linearities. It also shows great promise for enabling single-mode high-power emission from a large aperture device.