We introduce a classical analog of quantum matter in ultracold molecule -- or Rydberg atom -- synthetic dimensions, extending the Potts model to include interactions J1 between atoms adjacent in both real and synthetic space and studying its finite temperature properties. For intermediate values of J1, the resulting phases and phase diagrams are similar to those of the clock and Villain models, in which three phases emerge. There exists a sheet phase analogous to that found in quantum synthetic dimension models between the high temperature disordered phase and the low temperature ferromagnetic phase. We also employ machine learning to uncover non-trivial features of the phase diagram using the learning by confusion approach. The key result there is that the method is able to discern several successive phase transitions.
We introduce a classical analog of quantum matter in ultracold molecule -- or Rydberg atom -- synthetic dimensions, extending the Potts model to include interactions J1 between atoms adjacent in both real and synthetic space and studying its finite temperature properties. For intermediate values of J1, the resulting phases and phase diagrams are similar to those of the clock and Villain models, in which three phases emerge. There exists a sheet phase analogous to that found in quantum synthetic dimension models between the high temperature disordered phase and the low temperature ferromagnetic phase. We also employ machine learning to uncover non-trivial features of the phase diagram using the learning by confusion approach. The key result there is that the method is able to discern several successive phase transitions.
We calculate properties of dipolar interacting ultracold molecules or Rydberg atoms in a semisynthetic three-dimensional configuration---one synthetic dimension plus a two-dimensional real-space optical lattice or periodic microtrap array---using the stochastic Green's function quantum Monte Carlo method. Through a calculation of thermodynamic quantities and appropriate correlation functions, along with their finite-size scalings, we show that there is a second-order transition to a low-temperature phase in which two-dimensional ``sheets'' form in the synthetic dimension of internal rotational or electronic states of the molecules or Rydberg atoms, respectively. Simulations for different values of the interaction V, which acts between atoms or molecules that are adjacent both in real and synthetic space, allow us to compute a phase diagram. We find a finite-temperature transition at sufficiently large V as well as a quantum phase transition---a critical value Vc below which the transition temperature vanishes.
Synthetic-dimension platforms offer unique pathways for engineering quantum matter. We compute the phase diagram of a many-body system of ultracold atoms (or polar molecules) with a set of Rydberg states (or rotational states) as a synthetic dimension, where the particles are arranged in real space in optical microtrap arrays and interact via dipole-dipole exchange interaction. Using mean-field theory, we find three ordered phases---two are localized in the synthetic dimension, predicted as zero-temperature ground states by Sundar et al. [Sci. Rep. 8, 3422 (2018); Phys. Rev. A 99, 013624 (2019)], and one is a delocalized phase. We characterize them by identifying the spontaneously broken discrete symmetries of the Hamiltonian. We also compute the phase diagram as a function of temperature and interaction strength for both signs of the interaction. For system sizes with more than six synthetic sites and attractive interactions, we find that the thermal phase transitions can be first or second order, which leads to a tricritical point on the phase boundary. By examining the dependence of the tricritical point and other special points of the phase boundary on the synthetic dimension size, we shed light on the physics for thermodynamically large synthetic dimension.
Synthetic dimensions alter one of the most fundamental properties in nature, the dimension of space. They allow, for example, a real three-dimensional system to act as effectively four-dimensional. Driven by such possibilities, synthetic dimensions have been engineered in ongoing experiments with ultracold matter. We show that rotational states of ultracold molecules can be used as synthetic dimensions extending to many - potentially hundreds of - synthetic lattice sites. Microwaves coupling rotational states drive fully controllable synthetic inter-site tunnelings, enabling, for example, topological band structures. Interactions leads to even richer behavior: when molecules are frozen in a real space lattice with uniform synthetic tunnelings, dipole interactions cause the molecules to aggregate to a narrow strip in the synthetic direction beyond a critical interaction strength, resulting in a quantum string or a membrane, with an emergent condensate that lives on this string or membrane. All these phases can be detected using local measurements of rotational state populations.
In this dissertation, I theoretically investigate the equilibrium properties of three strongly correlated multi-level quantum platforms -- synthetic dimension using ultracold Rydberg atoms, multi-flavor Fermi-Hubbard simulators with ultracold atoms, and magnon-spin coupled rare-earth orthoferrites -- using various numerical and analytical methods. After the broad research motivation in the first chapter, Chapter 2 introduces the general principles of quantum simulation using synthetic dimension platforms. Chapter 3 discusses the first realization with Rydberg atom platform to simulate the topological Su-Schrieffer-Heeger (SSH) model, and how environmental noise affects it. Chapter 4 shows the mean-field phase diagram of dipole-coupled ultracold Rydberg atom arrays exhibiting quantum strings and other ordered states. The connection of the thermal phase transition to that of a classical extended Potts model is also discussed from a renormalization (RG) and generalized duality perspective. These examples illustrate the versatility of synthetic dimension in simulating and engineering quantum phenomena. Chapters 5-6 explore the properties of multi-flavor Fermi-Hubbard models on square optical lattices using numerical linked-cluster expansions (NLCE). First, I show universal thermodynamics of SU(N) Fermi-Hubbard models above superexchange temperatures. Then, I discuss the agreement between numerical simulated equations of state and correlation functions to optical lattice experiments using 173Yb [SU(N)-symmetric interactions] and three spin-flavors of 6Li [spin-dependent interactions] at intermediate temperatures. Thermometry performed with this method agrees well with the model-independent thermometry. Lastly, I propose a method of computing observables at low temperatures in bipartite ordered states by adding a suitable boundary field to the NLCE. NLCE agreeing to quantum simulations at temperatures above the superexchange temperatures and a possibility to make accurate predictions at low temperatures for certain states make it a powerful algorithm to be used side-by-side with quantum simulations. Chapter 7 is based on the observation of magnonic superradiance in ErFeO3. The spin Hamiltonian reveals a simultaneous kink and mode-softening of two of the lower polaritons, strongly suggesting a superradiant phase transition. Its mapping to an extended Dicke model is also discussed. This is the first evidence towards a macroscopically squeezed spin state. Finally, I conclude with a broad discussion and an outlook in Chapter 8.
Synthetic dimensions are powerful tools for quantum simulation and computation. They are realized by harnessing internal or external degrees of freedom of an atom or molecule, which can mimic the motion of an electron in a real-space lattice potential. Such degrees of freedom are highly tunable and can be engineered to create configurations difficult to access or realize in real space. Some of the exciting possibilities include realizing higher dimensions systems[1, 2, 3], nontrivial real space[4, 5] and band structure[6, 7] topologies and artificial gauge fields[8, 9]. Experiments have utilized various degrees of freedom to create synthetic dimensions, such as motional[10, 11], spin[8, 12, 13, 14] and rotational[15] levels of atoms and molecules, and frequency modes, spatial modes, and arrival times in photonic systems[16]. Atomic synthetic dimensions have demonstrated artificial gauge fields, spin-orbit coupling, chiral edge states using Raman-coupled ground magnetic sublevels[8, 12, 17] of atoms, and phenomena such as Anderson localization using two-photon Bragg transitions by coupling free-particle momentum states[18]. Here, we harness the Rydberg levels of 84Sr to realize a synthetic lattice for studying quantum matter. Resonant millimeter-wave (mm-wave) radiation coupling Rydberg levels |i⟩ and |j⟩ with amplitude Ωij (Rabi frequency) are described by the same Hamiltonian as a particle tunneling between lattice sites |i⟩ and |j⟩ with tunneling amplitude Jij = Ωij /2. The mathematical equivalence to particles moving in a real-space lattice enables Rydberg levels to function as a synthetic spatial dimension. Rydberg-atom synthetic dimensions offer control over connectivity, tunneling rates and on-site potentials, which allows for the creation of a broad range of synthetic dimensional system. The capabilities of such a system are demonstrated by realizing the famous Su-Schrieffer-Heeger (SSH) model[19] and studying its topologically protected edge states(TPS).