Synthetic dimensions alter one of the most fundamental properties in nature, the dimension of space. They allow, for example, a real three-dimensional system to act as effectively four-dimensional. Driven by such possibilities, synthetic dimensions have been engineered in ongoing experiments with ultracold matter. We show that rotational states of ultracold molecules can be used as synthetic dimensions extending to many - potentially hundreds of - synthetic lattice sites. Microwaves coupling rotational states drive fully controllable synthetic inter-site tunnelings, enabling, for example, topological band structures. Interactions leads to even richer behavior: when molecules are frozen in a real space lattice with uniform synthetic tunnelings, dipole interactions cause the molecules to aggregate to a narrow strip in the synthetic direction beyond a critical interaction strength, resulting in a quantum string or a membrane, with an emergent condensate that lives on this string or membrane. All these phases can be detected using local measurements of rotational state populations.
Synthetic dimensions alter one of the most fundamental properties in nature, the dimension of space. They allow, for example, a real three-dimensional system to act as effectively four-dimensional. Driven by such possibilities, synthetic dimensions have been engineered in ongoing experiments with ultracold matter. We show that rotational states of ultracold molecules can be used as synthetic dimensions extending to many - potentially hundreds of - synthetic lattice sites. Microwaves coupling rotational states drive fully controllable synthetic inter-site tunnelings, enabling, for example, topological band structures. Interactions leads to even richer behavior: when molecules are frozen in a real space lattice with uniform synthetic tunnelings, dipole interactions cause the molecules to aggregate to a narrow strip in the synthetic direction beyond a critical interaction strength, resulting in a quantum string or a membrane, with an emergent condensate that lives on this string or membrane. All these phases can be detected using local measurements of rotational state populations.
Engineering synthetic dimensions, where the physics of additional spatial dimensions is simulated within the internal states of a quantum system, allows the realisation of phenomena not otherwise accessible in experiments. Ultracold ground-state polar molecules are an ideal platform to encode synthetic dimensions, offering access to large Hilbert spaces of long-lived internal states associated with the rotational and hyperfine degrees of freedom, that can be coupled together with microwave fields to simulate tunnelling. Here, to benchmark the advantages of ultracold molecules, we encode a 1D synthetic lattice in the rotational states of ultracold RbCs molecules and use it to investigate the well-known Su-Schrieffer-Heeger (SSH) model, a minimal model displaying topological properties. To probe the system, we perform spectroscopy using an auxiliary rotational state and study the time dynamics after deterministic state preparation. We demonstrate long coherence times, typically ~500 times the lattice tunnelling period, even for a synthetic lattice using 8 rotational states. Observations of dynamics at long times with full site-resolved readout of the synthetic dimension allow us to test the effects of chiral and non-chiral perturbations on the topologically protected edge states. Our work lays the foundation for further quantum simulations using the rich internal structure of molecules, including dipolar string phases in interacting samples of molecules, and adiabatic state preparation of many-body Hamiltonians.
We consider ultracold polar molecules trapped in a unit-filled one-dimensional chain in real space created with an optical lattice or a tweezer array and illuminated by microwaves that resonantly drive transitions within a chain of rotational states. We describe the system by a two-dimensional lattice model, with the first dimension being a lattice in real space and the second dimension being a lattice in a synthetic direction composed of rotational states. We calculate this system's ground-state phase diagram. We show that as the dipole interaction strength is increased, the molecules undergo a phase transition from a two-dimensional gas to a phase in which the molecules bind together and form a string that resembles a one-dimensional object living in the two-dimensional (i.e., one real and one synthetic dimensional) space. We demonstrate this with two complementary techniques: numerical calculations using matrix product state techniques and an analytic solution in the limit of infinitely strong dipole interaction. Our calculations reveal that the string phase at infinite interaction is effectively described by emergent particles living on the string and that this leads to a rich spectrum with excitations missed in earlier mean-field treatments.
Synthetic-dimension platforms offer unique pathways for engineering quantum matter. We compute the phase diagram of a many-body system of ultracold atoms (or polar molecules) with a set of Rydberg states (or rotational states) as a synthetic dimension, where the particles are arranged in real space in optical microtrap arrays and interact via dipole-dipole exchange interaction. Using mean-field theory, we find three ordered phases---two are localized in the synthetic dimension, predicted as zero-temperature ground states by Sundar et al. [Sci. Rep. 8, 3422 (2018); Phys. Rev. A 99, 013624 (2019)], and one is a delocalized phase. We characterize them by identifying the spontaneously broken discrete symmetries of the Hamiltonian. We also compute the phase diagram as a function of temperature and interaction strength for both signs of the interaction. For system sizes with more than six synthetic sites and attractive interactions, we find that the thermal phase transitions can be first or second order, which leads to a tricritical point on the phase boundary. By examining the dependence of the tricritical point and other special points of the phase boundary on the synthetic dimension size, we shed light on the physics for thermodynamically large synthetic dimension.
Synthetic dimensions are powerful tools for quantum simulation and computation. They are realized by harnessing internal or external degrees of freedom of an atom or molecule, which can mimic the motion of an electron in a real-space lattice potential. Such degrees of freedom are highly tunable and can be engineered to create configurations difficult to access or realize in real space. Some of the exciting possibilities include realizing higher dimensions systems[1, 2, 3], nontrivial real space[4, 5] and band structure[6, 7] topologies and artificial gauge fields[8, 9]. Experiments have utilized various degrees of freedom to create synthetic dimensions, such as motional[10, 11], spin[8, 12, 13, 14] and rotational[15] levels of atoms and molecules, and frequency modes, spatial modes, and arrival times in photonic systems[16]. Atomic synthetic dimensions have demonstrated artificial gauge fields, spin-orbit coupling, chiral edge states using Raman-coupled ground magnetic sublevels[8, 12, 17] of atoms, and phenomena such as Anderson localization using two-photon Bragg transitions by coupling free-particle momentum states[18]. Here, we harness the Rydberg levels of 84Sr to realize a synthetic lattice for studying quantum matter. Resonant millimeter-wave (mm-wave) radiation coupling Rydberg levels |i⟩ and |j⟩ with amplitude Ωij (Rabi frequency) are described by the same Hamiltonian as a particle tunneling between lattice sites |i⟩ and |j⟩ with tunneling amplitude Jij = Ωij /2. The mathematical equivalence to particles moving in a real-space lattice enables Rydberg levels to function as a synthetic spatial dimension. Rydberg-atom synthetic dimensions offer control over connectivity, tunneling rates and on-site potentials, which allows for the creation of a broad range of synthetic dimensional system. The capabilities of such a system are demonstrated by realizing the famous Su-Schrieffer-Heeger (SSH) model[19] and studying its topologically protected edge states(TPS).
We present a technique for engineering quantum magnets via ultracold polar molecules in optical lattices and explore exotic interplay between its spin superfluidity and solidity. The molecular ground and first excited rotational states are resonantly coupled by a linearly polarized microwave field. The spin-up (spin-down) states are presented by molecular rotational states of electric dipole moment along (against) the coupling field. By controlling the angle between the lattice direction and the coupling field, the inter-site interaction can be tuned from antiferromagnetic to ferromagnetic. Furthermore, the dipole-dipole interaction induces an exotic interplay between spin superfluidity and solidity, and spin supersolid phases may appear in mediate regions.
We calculate properties of dipolar interacting ultracold molecules or Rydberg atoms in a semisynthetic three-dimensional configuration---one synthetic dimension plus a two-dimensional real-space optical lattice or periodic microtrap array---using the stochastic Green's function quantum Monte Carlo method. Through a calculation of thermodynamic quantities and appropriate correlation functions, along with their finite-size scalings, we show that there is a second-order transition to a low-temperature phase in which two-dimensional ``sheets'' form in the synthetic dimension of internal rotational or electronic states of the molecules or Rydberg atoms, respectively. Simulations for different values of the interaction V, which acts between atoms or molecules that are adjacent both in real and synthetic space, allow us to compute a phase diagram. We find a finite-temperature transition at sufficiently large V as well as a quantum phase transition---a critical value Vc below which the transition temperature vanishes.