Many strongly correlated systems exhibit strange metallic behavior in certain parameter regimes characterized by anomalous transport properties that are irreconcilable with a Fermi-liquid-like description in terms of quasiparticles. The Hubbard model is a standard theoretical starting point to examine the properties of such systems and also exhibits non-Fermi-liquid behavior in simulations. Here we analytically study the two-dimensional hole-doped Hubbard model in the large
U limit, first identifying a doping-induced percolation transition in the low-energy sector occurring at a definite critical doping
pc depending on lattice structure. Using the critical properties near this transition we rewrite the Hubbard Hamiltonian and motivate a low-energy lattice-independent large-
N model with distinct non-Fermi-liquid properties. We show that this model has linear-in-
T resistivity with doping-dependent slope maximized at
p=pc and power-law optical conductivity ${\ensuremath{\sim}|\ensuremath{\omega}|}^{\ensuremath{-}2/3}$. Though the parameters used in developing this theory mean it cannot be directly applied to the cuprate superconductors, we nevertheless reproduce several important phenomena observed in their strange metal phase and also predict these same qualitative behaviors to manifest in other lattices near concrete hole dopings.
Strange metal behavior is traditionally associated with an underlying putative quantum critical point at zero temperature. However, in many correlated metals, e.g., high-
Tc cuprate superconductors, strange metallicity persists at low temperatures over an extended range of microscopic parameters, suggesting the existence of an underlying quantum critical phase, whose possible physical origins remain poorly understood. Systematic investigations of physical scenarios giving rise to such a critical, non-Fermi liquid (NFL) phase are therefore crucial to better understand this puzzling behavior. In a previous study [Bashan et al., Phys. Rev. Lett. 132, 236501 (2024)], we considered a solvable large-
N model consisting of itinerant electrons coupled to local two-level systems (TLSs) via spatially random interactions, inspired by the possibility of emergent metallic glassiness due to frustrated competing orders, and found that the system hosts an NFL phase with tunable exponents at intermediate couplings. In this paper, we expand our investigation to the following: (i) We study the extent to which this NFL phase is generic by considering various deformations of our theory, including coupling of electrons to multiple operators of the TLSs and arbitrarily directed TLS fields. We find that the physical picture obtained in Bashan et al. [Phys. Rev. Lett. 132, 236501 (2024)] qualitatively persist in a wide region of parameter space, showcasing the robustness of the NFL phase. (ii) We analyze the superconducting instability caused by the coupling of TLSs to electrons, and find a rich structure, including quantum critical pairing associated with the NFL phase and conventional BCS-like pairing in the weak and strong coupling limits. (iii) We elaborate on the analysis of Bashan et al. [Phys. Rev. Lett. 132, 236501 (2024)], including single-particle, transport, and thermodynamic properties.
Abstract. The normal state metallic behavior above the superconducting transition temperature (Tsc) remains one of the least understood properties since its discovery in cuprates by Bednorz and Müller [1]. Apart from the pseudogap (T ∗) phenomenon above Tsc, there is this T-linear resistivity that was first recognized by Anderson [2] as strange simply because it does not obey the low-temperature T 2 electron-electron scattering rate predicted from the Fermi liquid theory. Here, we prove that the finite temperature continu-ous quantum phase transition (CTQPT) is responsible for the transition from a strange metal to a Fermi liquid for a given chemical composition. Our proof follows the Green function formalism and the energy-level spacing renormal-ization group method. Interestingly, the CTQPT stated above can be related to the proof derived by Parameswaran, Shankar and Sondhi [3], in which, the one-to-one correspondence between the Fermi gas and Fermi liquid is indeed a special case. The theory is further exploited to give unambiguous explanations as to why and how doping gives rise to spectral weight transfer observed in the soft X-ray absorption spectroscopic measurements for the La-Sr-Cu-O system. PACS: 74.72.-h, 71.10.Hf, 74.25.F-, 74.25.Jb 1.
The strange metal is an enigma within the field of many-body quantum physics, as it defies the standard Fermi liquid theory of metals due to the absence of well-defined, electron-like quasiparticles. It has been presumed that strange metal behavior arises due to strong correlations between electrons that are not present in ordinary Fermi liquids, but the exact nature of these correlations is unknown. To this end, this thesis aims to address the fundamental question: What, precisely, is so strongly correlated about charge in the strange metal? This question is tackled by experimentally measuring the dynamic charge response function, which directly encodes charge correlations in momentum and energy, using the technique of Momentum-resolved Electron Energy-loss Spectroscopy (M-EELS). In particular, two prototypical members of the cuprate and ruthenate strange metal families are studied: Bi-2212 and Sr
2RuO
4. By studying Bi-2212 at optimal doping, it is found that the charge response of the strange metal is characterized by a broad continuum of fluctuations that are momentum and energy independent over a large range of parameter space, unlike Fermi liquid charge correlations which exhibit propagating density waves of charge with well defined energy and momentum (i.e. plasmons). We argue that, in essence, the charge correlations of the strange metal are highly localized in both space and time, unlike the Fermi Liquid where they are localized in momentum and energy instead. To understand how charge correlations change as one leaves the strange metal regime, the M-EELS response of Bi-2212 is mapped out as a function of doping and temperature. At high temperature, it is found that the continuum is largely doping independent. However, upon cooling, very large changes in spectral weight are observed over a range of energy scales nearly two orders of magnitude larger than the thermal scale
kBT. Moreover, this change in spectral weight undergoes a sign reversal as a function of doping, with spectral weight enhancement on the underdoped side, suppression in the overdoped regime, and no change at optimal doping. These changes in spectral weight are completely unlike the case of the Fermi liquid, where doping only acts to rigidly shift the plasmon energy and no significant changes occur as a function of temperature. Finally, we venture further and ask whether strange metal and Fermi liquid charge correlations can simultaneously coexist in a material. To explore this possibility, we measured the M-EELS response of Sr
2RuO
4, a material which exhibits strange and bad metal behavior at high temperature, but transitions to a well-defined Fermi liquid at low temperature. Surprisingly, in the strange metal regime, Sr
2RuO
4 exhibits both a broad continuum similar to Bi-2212 and a propagating Fermi liquid collective mode at low-energies and momentum. Upon cooling, low-energy spectral weight is suppressed in the strange metal continuum and the Fermi liquid collective mode velocity is strongly renormalized. These findings confirm the strange metal and Fermi liquid can coexist and demonstrate that Sr
2RuO
4 exhibits charge correlations with strange metal character at high energies and short length scales and Fermi liquid character at low energies and long wavelengths.
We propose that the nonequilibrium current measured in the
a-
b plane of an underdoped cuprate (in either the strange metal or pseudogap regime) in contact with either an overdoped cuprate or a standard Fermi liquid can be used to diagnose how different the pseudogap and strange metals are from a Fermi liquid. Naively, one expects the strange metal to be more different from a Fermi liquid than the pseudogap is. We compute the expected nonequilibrium transport signal with the three Green's functions that are available in the literature: (1) marginal Fermi-liquid theory, (2) the phenomenological ansatz for the pseudogap regime, and (3) the Wilsonian reduction of the Hubbard model which contains both the strange metal and pseudogap. All three give linear
I-
V curves at low bias voltages. Significant deviations from linearity at higher voltages obtain only in the marginal Fermi-liquid approach. The key finding, however, is that
I-
V curves for the strange metal/Fermi-liquid contact exceed that of the pseudogap/Fermi-liquid system. If this is borne out experimentally, this implies that the strange metal is less orthogonal to a Fermi liquid than the pseudogap is. Within the Wilsonian reduction of the Hubbard model, this result is explained in terms of a composite-particle picture. Namely, the pseudogap corresponds to a confinement transition of the charge degrees of freedom present in the strange metal. In the strange metal the composite excitations break up and electron quasiparticles scatter off bosons. The bosons here, however, do not arise from phonons but from the charge degrees of freedom responsible for dynamical spectral weight transfer.
A systematic study of optical and transport properties of the Hubbard model, based on the Metzner-Vollhardt dynamical mean-field approximation, is reviewed. This model shows interesting anomalous properties that are, in our opinion, ubiquitous to single-band strongly correlated systems (for all spatial dimensions greater than one) and also compare qualitatively with many anomalous transport features of the high-T c cuprates. This anomalous behaviour of the normal-state properties is traced to a ‘collective single-band Kondo effect’, in which a quasiparticle resonance forms at the Fermi level as the temperature is lowered, ultimately yielding a strongly renormalized Fermi liquid at zero temperature.