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Charge fluctuations of the strange metal in space and time

Ali Husain

Published Jun 25, 2020• 0 citations
OpenAlex

Abstract

The strange metal is an enigma within the field of many-body quantum physics, as it defies the standard Fermi liquid theory of metals due to the absence of well-defined, electron-like quasiparticles. It has been presumed that strange metal behavior arises due to strong correlations between electrons that are not present in ordinary Fermi liquids, but the exact nature of these correlations is unknown. To this end, this thesis aims to address the fundamental question: What, precisely, is so strongly correlated about charge in the strange metal? This question is tackled by experimentally measuring the dynamic charge response function, which directly encodes charge correlations in momentum and energy, using the technique of Momentum-resolved Electron Energy-loss Spectroscopy (M-EELS). In particular, two prototypical members of the cuprate and ruthenate strange metal families are studied: Bi-2212 and Sr$_2$RuO$_4$. By studying Bi-2212 at optimal doping, it is found that the charge response of the strange metal is characterized by a broad continuum of fluctuations that are momentum and energy independent over a large range of parameter space, unlike Fermi liquid charge correlations which exhibit propagating density waves of charge with well defined energy and momentum (i.e. plasmons). We argue that, in essence, the charge correlations of the strange metal are highly localized in both space and time, unlike the Fermi Liquid where they are localized in momentum and energy instead. To understand how charge correlations change as one leaves the strange metal regime, the M-EELS response of Bi-2212 is mapped out as a function of doping and temperature. At high temperature, it is found that the continuum is largely doping independent. However, upon cooling, very large changes in spectral weight are observed over a range of energy scales nearly two orders of magnitude larger than the thermal scale $k_B T$. Moreover, this change in spectral weight undergoes a sign reversal as a function of doping, with spectral weight enhancement on the underdoped side, suppression in the overdoped regime, and no change at optimal doping. These changes in spectral weight are completely unlike the case of the Fermi liquid, where doping only acts to rigidly shift the plasmon energy and no significant changes occur as a function of temperature. Finally, we venture further and ask whether strange metal and Fermi liquid charge correlations can simultaneously coexist in a material. To explore this possibility, we measured the M-EELS response of Sr$_2$RuO$_4$, a material which exhibits strange and bad metal behavior at high temperature, but transitions to a well-defined Fermi liquid at low temperature. Surprisingly, in the strange metal regime, Sr$_2$RuO$_4$ exhibits both a broad continuum similar to Bi-2212 and a propagating Fermi liquid collective mode at low-energies and momentum. Upon cooling, low-energy spectral weight is suppressed in the strange metal continuum and the Fermi liquid collective mode velocity is strongly renormalized. These findings confirm the strange metal and Fermi liquid can coexist and demonstrate that Sr$_2$RuO$_4$ exhibits charge correlations with strange metal character at high energies and short length scales and Fermi liquid character at low energies and long wavelengths.

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Reports on Progress in Physics•Mar 20, 2025•5 citations
The strange metal is an enigma within the field of many-body quantum physics, as it defies the standard Fermi liquid theory of metals due to the absence of well-defined, electron-like quasiparticles. It has been presumed that strange metal behavior arises due to strong correlations between electrons that are not present in ordinary Fermi liquids, but the exact nature of these correlations is unknown. To this end, this thesis aims to address the fundamental question: What, precisely, is so strongly correlated about charge in the strange metal? This question is tackled by experimentally measuring the dynamic charge response function, which directly encodes charge correlations in momentum and energy, using the technique of Momentum-resolved Electron Energy-loss Spectroscopy (M-EELS). In particular, two prototypical members of the cuprate and ruthenate strange metal families are studied: Bi-2212 and Sr2_22​RuO4_44​. By studying Bi-2212 at optimal doping, it is found that the charge response of the strange metal is characterized by a broad continuum of fluctuations that are momentum and energy independent over a large range of parameter space, unlike Fermi liquid charge correlations which exhibit propagating density waves of charge with well defined energy and momentum (i.e. plasmons). We argue that, in essence, the charge correlations of the strange metal are highly localized in both space and time, unlike the Fermi Liquid where they are localized in momentum and energy instead. To understand how charge correlations change as one leaves the strange metal regime, the M-EELS response of Bi-2212 is mapped out as a function of doping and temperature. At high temperature, it is found that the continuum is largely doping independent. However, upon cooling, very large changes in spectral weight are observed over a range of energy scales nearly two orders of magnitude larger than the thermal scale kBTk_B TkB​T. Moreover, this change in spectral weight undergoes a sign reversal as a function of doping, with spectral weight enhancement on the underdoped side, suppression in the overdoped regime, and no change at optimal doping. These changes in spectral weight are completely unlike the case of the Fermi liquid, where doping only acts to rigidly shift the plasmon energy and no significant changes occur as a function of temperature. Finally, we venture further and ask whether strange metal and Fermi liquid charge correlations can simultaneously coexist in a material. To explore this possibility, we measured the M-EELS response of Sr2_22​RuO4_44​, a material which exhibits strange and bad metal behavior at high temperature, but transitions to a well-defined Fermi liquid at low temperature. Surprisingly, in the strange metal regime, Sr2_22​RuO4_44​ exhibits both a broad continuum similar to Bi-2212 and a propagating Fermi liquid collective mode at low-energies and momentum. Upon cooling, low-energy spectral weight is suppressed in the strange metal continuum and the Fermi liquid collective mode velocity is strongly renormalized. These findings confirm the strange metal and Fermi liquid can coexist and demonstrate that Sr2_22​RuO4_44​ exhibits charge correlations with strange metal character at high energies and short length scales and Fermi liquid character at low energies and long wavelengths.
The strange metallic regime across a number of high-temperature superconducting materials presents numerous challenges to the classic theory of Fermi liquid metals. Recent measurements of the dynamical charge response of strange metals, including optimally doped cuprates, have revealed a broad, featureless continuum of excitations, extending over much of the Brillouin zone. The collective density oscillations of this strange metal decay into the continuum in a manner that is at odds with the expectations of Fermi liquid theory. Inspired by these observations, we investigate the phenomenology of bosonic collective modes and the particle-hole excitations in a class of strange metals by making an analogy to the phonons of classical lattices falling apart across an unconventional jamming-like transition associated with the onset of rigidity. By making comparisons to the experimentally measured dynamical response functions, we reproduce many of the qualitative features using the above framework. We conjecture that the dynamics of electronic charge density over an intermediate range of energy scales in a class of strongly correlated metals can be at the brink of a jamming-like transition.
The anomalous strange metal phase found in high-T c cuprates does not follow the conventional condensed-matter principles enshrined in the Fermi liquid and presents a great challenge for theory.Highly precise experimental determination of the electronic self-energy can provide a test bed for theoretical models of strange metals, and angle-resolved photoemission can provide this as a function of frequency, momentum, temperature and doping.Here we show that constant energy cuts through the nodal spectral function in (Pb,Bi) 2 Sr 2-x La x CuO 6+δ have a non-Lorentzian lineshape, consistent with a selfenergy that is k dependent.This provides a new test for aspiring theories.Here we show that the experimental data are captured remarkably well by a power law with a k-dependent scaling exponent smoothly evolving with doping, a description that emerges naturally from anti-de Sitter/conformal-field-theory based semi-holography.This puts a spotlight on holographic methods for the quantitative modelling of strongly interacting quantum materials like the cuprate strange metals.The rich temperature versus doping diagram of the cuprate high-T c superconductors presents a cornucopia of non-conformity 1 .The superconductivity does not follow BCS theory anywhere in the phase diagram 2,3 , and in their normal state these unusual metals display qualitatively different experimental behaviour compared to the Fermi liquid, with the linear-in-T resistivity and quadratic-in-T Hall angle being among the most strange.One intriguing possible explanation of strange metal phenomenology is that it is controlled by a strongly interacting quantum critical phase.If so, the question follows whether their properties can be
Momentum-resolved electron energy-loss spectroscopy (EELS) on strange-metal BiSrCaCuO(Bi-2212) observes a broad charge continuum that is nearly momentum independent over an extended finite-momentum regime, whereas optical spectroscopy determines a metallic local conductivity. We analyze the long-wavelength response function that connects these regimes: the proper homogeneous bulk charge-density polarization. For any homogeneous-conserving metal whose longitudinal matter conductivity remains finite in thelimit at fixed nonzero frequency, the Ward identity gives. We then prove that any nonnegative normalized momentum-resolution kernel with a self-similar-scaled profile, uniformly bounded second moment, and tight second-moment tails preserves thisasymptotic behavior, changing only the prefactor. Consequently, a nearly local finite-continuum in Bi-2212, if continuously connected to a regular metallic optical limit of the same proper bulk response, is naturally described by a crossover surface. The theorem is a constraint on the proper bulk density response, or on a positive-scaled convolution of it; screened loss functions and surface EELS observables require the corresponding electrodynamic conversion before the constraint is applied.
We propose that the nonequilibrium current measured in the aaa-bbb plane of an underdoped cuprate (in either the strange metal or pseudogap regime) in contact with either an overdoped cuprate or a standard Fermi liquid can be used to diagnose how different the pseudogap and strange metals are from a Fermi liquid. Naively, one expects the strange metal to be more different from a Fermi liquid than the pseudogap is. We compute the expected nonequilibrium transport signal with the three Green's functions that are available in the literature: (1) marginal Fermi-liquid theory, (2) the phenomenological ansatz for the pseudogap regime, and (3) the Wilsonian reduction of the Hubbard model which contains both the strange metal and pseudogap. All three give linear III-VVV curves at low bias voltages. Significant deviations from linearity at higher voltages obtain only in the marginal Fermi-liquid approach. The key finding, however, is that III-VVV curves for the strange metal/Fermi-liquid contact exceed that of the pseudogap/Fermi-liquid system. If this is borne out experimentally, this implies that the strange metal is less orthogonal to a Fermi liquid than the pseudogap is. Within the Wilsonian reduction of the Hubbard model, this result is explained in terms of a composite-particle picture. Namely, the pseudogap corresponds to a confinement transition of the charge degrees of freedom present in the strange metal. In the strange metal the composite excitations break up and electron quasiparticles scatter off bosons. The bosons here, however, do not arise from phonons but from the charge degrees of freedom responsible for dynamical spectral weight transfer.
Recent progress in extremely correlated Fermi liquid theory (ECFL) and the dynamical mean field theory (DMFT) enables us to accurately compute in the $d\ensuremath{\rightarrow}\ensuremath{\infty}$ limit the resistivity of the $t\ensuremath{-}J$ model after setting $J\ensuremath{\rightarrow}0$. This is also the $U=\ensuremath{\infty}$ Hubbard model. Since JJJ is set to zero, our study isolates the dynamical effects of the single occupation constraint enforced by the projection operator originally introduced by Gutzwiller. We study three densities n=.75,.8,.85n=.75,.8,.85n=.75,.8,.85 that correspond to a range between the overdoped and optimally doped Mott insulating state. We delineate four distinct regimes separated by three crossovers, which are characterized by different behaviors of the resistivity $\ensuremath{\rho}$. We find at the lowest temperature TTT a Gutzwiller correlated Fermi liquid regime with $\ensuremath{\rho}\ensuremath{\propto}{T}^{2}$ extending up to an effective Fermi temperature that is dramatically suppressed from the noninteracting value by the proximity to half filling, $n\ensuremath{\sim}1$. This is followed by a Gutzwiller correlated strange metal regime with $\ensuremath{\rho}\ensuremath{\propto}(T\ensuremath{-}{T}_{0})$, i.e., a linear resistivity extrapolating back to $\ensuremath{\rho}=0$ at a positive T0{T}_{0}T0​. At a higher temperature scale this crosses over into the bad metal regime with $\ensuremath{\rho}\ensuremath{\propto}(T+{T}_{1})$, i.e., a linear resistivity extrapolating back to a finite resistivity at T=0T=0T=0 and passing through the Ioffe-Regel-Mott value where the mean free path is a few lattice constants. This regime finally gives way to the high TTT metal regime, where we find $\ensuremath{\rho}\ensuremath{\propto}T$, i.e., a linear resistivity extrapolating back to zero at T=0T=0T=0. The present work emphasizes the first two, i.e., the two lowest temperature regimes, where the availability of an analytical ECFL theory is of help in identifying the changes in related variables entering the resistivity formula that accompanies the onset of linear resistivity, and the numerically exact DMFT helps to validate the results. We also examine thermodynamical variables such as the magnetic susceptibility, compressibility, heat capacity, and entropy and correlate changes in these with the change in resistivity. This exercise casts valuable light on the nature of charge and spin correlations in the Gutzwiller correlated strange metal regime, which has features in common with the physically relevant strange metal phase seen in strongly correlated matter.
Abstract The mysterious metallic phase showing T-linear resistivity and a universal scattering rate 1 / τ = α P k B T / ℏ with a universal prefactor α P ∼ 1 and logarithmic-in-temperature singular specific heat coefficient, the so-called ‘Planckian metal phase’ was observed in various overdoped high- T c cuprate superconductors over a finite range in doping. Revealing the mystery of the Planckian metal state is believed to be the key to understanding the mechanism for high- T c superconductivity. Here, we propose a generic microscopic mechanism for this state based on quantum-critical local bosonic charge Kondo fluctuations coupled to both spinon and a heavy conduction-electron Fermi surface within the heavy-fermion formulation of the slave-boson t–J model. By a controlled perturbative renormalization group analysis, we examine the competition between the pseudogap phase, characterized by Anderson’s Resonating-Valence-Bond spin-liquid, and the Fermi-liquid state, modeled by the electron hopping (effective charge Kondo effect). We find a quantum-critical metallic phase with a universal Planckian ℏ ω / k B T scaling in scattering rate near an extended localized-delocalized (pseudogap-to-Fermi liquid) charge-Kondo breakdown transition. The d-wave superconducting ground state emerges near the transition. Unprecedented qualitative and quantitative agreements are reached between our theoretical predictions and various experiments, including optical conductivity, universal doping-independent field-to-temperature scaling in magnetoresistance, specific heat coefficient, marginal Fermi-liquid spectral function observed in ARPES, and Fermi surface reconstruction observed in Hall coefficients in various overdoped cuprates. Our mechanism offers a microscopic understanding of the quantum-critical Planckian metal phase observed in cuprates and its link to the pseudogap, d-wave superconducting, and Fermi liquid phases. It offers a promising route for understanding how d-wave superconductivity emerges from such a strange metal phase in cuprates–one of the long-standing open problems in condensed matter physics since 1990s–as well as shows a broader implication for the Planckian strange metal states observed in other correlated unconventional superconductors.