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arXiv:2210.13551 · Quantum

Chiral superconductivity in the doped triangular-lattice Fermi-Hubbard model in two dimensions

Vinicius Zampronio, Tommaso Macrì

Published Jul 20, 2023• 8 citations
arXivHTMLPDF

Abstract

The triangular-lattice Fermi-Hubbard model has been extensively investigated in the literature due to its connection to chiral spin states and unconventional superconductivity. Previous simulations of the ground state of the doped system rely on quasi-one-dimensional lattices where true long-range order is forbidden. Here we simulate two-dimensional and quasi-one-dimensional triangular lattices using state-of-the-art Auxiliary-Field Quantum Monte Carlo. Upon doping a non-magnetic chiral spin state, we observe evidence of chiral superconductivity supported by long-range order in Cooper-pair correlation and a finite value of the chiral order parameter. With this aim, we first locate the transition from the metallic to the non-magnetic insulating phase and the onset of magnetic order. Our results pave the way towards a better understanding of strongly correlated lattice systems with magnetic frustration.

DOI
10.22331/q-2023-07-20-1061

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The triangular-lattice Fermi-Hubbard model has been extensively investigated in the literature due to its connection to chiral spin states and unconventional superconductivity. Previous simulations of the ground state of the doped system rely on quasi-one-dimensional lattices where true long-range order is forbidden. Here we simulate two-dimensional and quasi-one-dimensional triangular lattices using state-of-the-art Auxiliary-Field Quantum Monte Carlo. Upon doping a non-magnetic chiral spin state, we observe evidence of chiral superconductivity supported by long-range order in Cooper-pair correlation and a finite value of the chiral order parameter. With this aim, we first locate the transition from the metallic to the non-magnetic insulating phase and the onset of magnetic order. Our results pave the way towards a better understanding of strongly correlated lattice systems with magnetic frustration.
We investigate the evolution of the Mott insulators in the triangular lattice Hubbard Model, as a function of hole doping $\ensuremath{\delta}$ in both the strong and intermediate coupling limits. Using the advanced density matrix renormalization group (DMRG) method, at light hole doping $\ensuremath{\delta}\ensuremath{\lesssim}10%$, we find a significant difference between strong and intermediate couplings. Notably, at intermediate coupling an unusual metallic state emerges, with short ranged spin correlations but long ranged spin-chirality order. Moreover, no clear Fermi surface or wave vector is observed, this chiral metal also exhibits staggered loop current, which breaks the translational symmetry. These features disappear on increasing interaction strength or on further doping. At strong coupling, the 120 degree magnetic order of the insulating magnet persists for light doping, and produces hole pockets with a well-defined Fermi surface. On further doping, $\ensuremath{\delta}\ensuremath{\approx}10%\ensuremath{\sim}20%$ SDW order and coherent hole Fermi pockets are found at both strong and intermediate couplings. At even higher doping $\ensuremath{\delta}\ensuremath{\gtrsim}20%$, the SDW order is suppressed and the spin-singlet Cooper pair correlations are simultaneously enhanced. We also briefly comment on the strong particle-hole asymmetry of the model.
The emergence of superconductivity from doping strongly correlated chiral topological phases in purely repulsive two-dimensional fermionic systems is a problem of broad and fundamental interest. However, existing numerical evidence has been limited to finite-size studies, and direct thermodynamic-limit evidence for superconducting long-range order has remained lacking. Here we provide such evidence for chiral superconductivity in the triangular Hofstadter-Hubbard model by advancing a simplex tensor-network approach that simultaneously captures superconducting long-range order and chiral topological order in the presence of intrinsic charge fluctuations, a capability that has remained challenging for previous two-dimensional approaches. We show that a broad intermediate-UUU chiral spin liquid is separated from the weak-UUU Chern insulator by a Mott transition, together forming undoped parent chiral topological states. Upon hole doping, we identify a uniform chiral superconducting state in the infinite system, characterized by a finite complex pairing order parameter. The pairing field exhibits an almost universal phase winding over a broad interaction-doping regime, with a distinct pocket of opposite winding near the Mott criticality. In addition, the entanglement spectrum retains the chiral structure of the parent topological phases while developing additional low-energy branches upon doping. These results establish that chiral superconductivity emerges robustly from doped chiral topological phases.
The interplay of strong interactions and magnetic fields gives rise to unusual forms of superconductivity and magnetism in quantum many-body systems. Here, we present an experimental study of the two-dimensional Fermi-Hubbard model-a paradigm for strongly correlated fermions on a lattice-in the presence of a Zeeman field and varying doping. Using site-resolved measurements, we revealed anisotropic antiferromagnetic correlations, a precursor to long-range canted order. We observed nonmonotonic behavior of the local polarization with doping for strong interactions, which we attribute to the evolution from an antiferromagnetic insulator to a metallic phase. Our results pave the way to experimentally mapping the low-temperature phase diagram of the Fermi-Hubbard model as a function of both doping and spin polarization, for which many open questions remain.
The suppression of antiferromagnetic ordering in geometrically frustrated Hubbard models leads to a variety of exotic quantum phases including quantum spin liquids and chiral states. Here, we focus on the Hubbard model on one of the simplest frustrated lattice geometries, a triangular lattice. Motivated by the recent realization of ultracold fermionic atoms in triangular optical lattices, we study the properties of the triangular-lattice Hubbard model through a numerical linked-cluster expansion algorithm. We investigate the Mott insulator transition finding a critical interaction Uc/t=7.0(2){U}_{c}/t=7.0(2)Uc​/t=7.0(2) and use spatial two- and three-point correlation functions to explore doped and imbalanced systems. Our results demonstrate that many interesting features occur at temperatures previously obtained for ultracold fermions in optical lattices and are accessible by upcoming experiments. Our calculations will be helpful for thermometry in ultracold atom quantum simulators and can guide experimental searches for exotic quantum phases in atomic triangular Hubbard quantum simulators.
The existence of a gapped chiral spin liquid has been recently suggested in the vicinity of the metal-insulator transition of the Hubbard model on the triangular lattice, by intensive density-matrix renormalization group (DMRG) simulations [A. Szasz, J. Motruk, M. P. Zaletel, and J. E. Moore, Phys. Rev. X 10, 021042 (2020)]. Here, we report the results obtained within the variational Monte Carlo technique based upon Jastrow-Slater wave functions, implemented with backflow correlations. As in DMRG calculations, we consider NNN-leg cylinders. For N=4N=4N=4 and in the presence of a next-nearest-neighbor hopping, a chiral spin liquid emerges between the metal and the insulator with magnetic quasi-long-range order. Within our approach, the chiral state is gapped and breaks the reflection symmetry. By contrast, for both N=5N=5N=5 and 6, the chiral spin liquid is not the state with the lowest variational energy: in the former case, a nematic spin liquid is found in the entire insulating regime, while for the less frustrated case with N=6N=6N=6 the results are very similar to that obtained on two-dimensional clusters [L. F. Tocchio, A. Montorsi, and F. Becca, Phys. Rev. B 102, 115150 (2020)], with an antiferromagnetic phase close to the metal-insulator transition and a nematic spin liquid in the strong-coupling regime.
It has long been proposed that doping a chiral spin liquid (CSL) or fractional quantum Hall state can give rise to topological superconductivity. Despite intensive effort, definitive evidences still remain lacking. We address this problem by studying the t-J model supplemented by time-reversal symmetry breaking chiral interaction J_{χ} on the triangular lattice using density-matrix renormalization group with a finite concentration δ of doped holes. It has been established that the undoped, i.e., δ=0, system has a CSL ground state in the parameter region 0.32≤J_{χ}/J≤0.56. Upon light doping, we find that the ground state of the system is consistent with a Luther-Emery liquid with power-law superconducting and charge-density-wave correlations but short-range spin-spin correlations. In particular, the superconducting correlations, whose pairing symmetry is consistent with d±id wave, are dominant at all hole doping concentrations. Our results provide direct evidences that doping the CSL on the triangular lattice can naturally give rise to topological superconductivity.