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arXiv:2002.04686 · Physical Review Letters

Topological Superconductivity in the Doped Chiral Spin Liquid on the Triangular Lattice

Yi‐Fan Jiang, Hong‐Chen Jiang

Published Oct 9, 2020• 47 citations
arXivHTMLPDF

Abstract

It has long been proposed that doping a chiral spin liquid (CSL) or fractional quantum Hall state can give rise to topological superconductivity. Despite intensive effort, definitive evidences still remain lacking. We address this problem by studying the t-J model supplemented by time-reversal symmetry breaking chiral interaction J_{χ} on the triangular lattice using density-matrix renormalization group with a finite concentration δ of doped holes. It has been established that the undoped, i.e., δ=0, system has a CSL ground state in the parameter region 0.32≤J_{χ}/J≤0.56. Upon light doping, we find that the ground state of the system is consistent with a Luther-Emery liquid with power-law superconducting and charge-density-wave correlations but short-range spin-spin correlations. In particular, the superconducting correlations, whose pairing symmetry is consistent with d±id wave, are dominant at all hole doping concentrations. Our results provide direct evidences that doping the CSL on the triangular lattice can naturally give rise to topological superconductivity.

DOI
10.1103/physrevlett.125.157002

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It has long been proposed that doping a chiral spin liquid (CSL) or fractional quantum Hall state can give rise to topological superconductivity. Despite intensive effort, definitive evidences still remain lacking. We address this problem by studying the t-J model supplemented by time-reversal symmetry breaking chiral interaction J_{χ} on the triangular lattice using density-matrix renormalization group with a finite concentration δ of doped holes. It has been established that the undoped, i.e., δ=0, system has a CSL ground state in the parameter region 0.32≤J_{χ}/J≤0.56. Upon light doping, we find that the ground state of the system is consistent with a Luther-Emery liquid with power-law superconducting and charge-density-wave correlations but short-range spin-spin correlations. In particular, the superconducting correlations, whose pairing symmetry is consistent with d±id wave, are dominant at all hole doping concentrations. Our results provide direct evidences that doping the CSL on the triangular lattice can naturally give rise to topological superconductivity.
Abstract Broad interest in quantum spin liquid (QSL) phases was triggered by the notion that they can be viewed as insulating phases with preexisting electron pairs, such that upon light doping they might automatically yield high temperature superconductivity. Yet despite intense experimental and numerical efforts, definitive evidence showing that doping QSLs leads to superconductivity has been lacking. We address the problem of a lightly doped QSL through a large-scale density-matrix renormalization group study of the t-J model on finite-circumference triangular cylinders with a small but nonzero concentration of doped holes. We provide direct evidences that doping QSL can naturally give rise to d-wave superconductivity. Specifically, we find power-law superconducting correlations with a Luttinger exponent, Ksc ≈ 1, which is consistent with a strongly diverging superconducting susceptibility, χsc ∼ T−(2 − Ksc){\chi }_{sc} \,\sim\, {T}^{-(2\,-\,{K}_{sc})}χsc​∼T−(2−Ksc​) χ s c ~ T − ( 2 − K s c ) as the temperature T → 0. The spin–spin correlations—as in the undoped QSL state—fall exponentially which suggests that the superconducting pair-pair correlations evolve smoothly from the insulating parent state.
The emergence of superconductivity from doping strongly correlated chiral topological phases in purely repulsive two-dimensional fermionic systems is a problem of broad and fundamental interest. However, existing numerical evidence has been limited to finite-size studies, and direct thermodynamic-limit evidence for superconducting long-range order has remained lacking. Here we provide such evidence for chiral superconductivity in the triangular Hofstadter-Hubbard model by advancing a simplex tensor-network approach that simultaneously captures superconducting long-range order and chiral topological order in the presence of intrinsic charge fluctuations, a capability that has remained challenging for previous two-dimensional approaches. We show that a broad intermediate-UUU chiral spin liquid is separated from the weak-UUU Chern insulator by a Mott transition, together forming undoped parent chiral topological states. Upon hole doping, we identify a uniform chiral superconducting state in the infinite system, characterized by a finite complex pairing order parameter. The pairing field exhibits an almost universal phase winding over a broad interaction-doping regime, with a distinct pocket of opposite winding near the Mott criticality. In addition, the entanglement spectrum retains the chiral structure of the parent topological phases while developing additional low-energy branches upon doping. These results establish that chiral superconductivity emerges robustly from doped chiral topological phases.
Demonstrating superconductivity in purely repulsive Hubbard models is a compelling goal which underscores the counter-intuitive ability of Coulomb interactions to mediate superconductivity. Here, we present numerical evidence for robust superconductivity in a triangular Hubbard-Hofstadter model at π/2π/2π/2 flux per plaquette. Employing infinite density matrix renormalization group calculations on infinite cylinders of finite circumference, we observe superconducting ground states for a wide range of dopings, whose pair-correlations strengthen as the 2D limit is approached. At a density of one electron per site, Hubbard interactions have been reported to drive the insulating parent state of the superconductor from an integer quantum Hall (IQH) state to a chiral spin liquid (CSL). Our findings give credence to a recent proposal that proximity to the IQH-CSL transition serves to make chiral superconductivity energetically favorable on doping, and also correctly predicts the nature of the edge modes in the superconductor. On the CSL side, this suggests the superconductor can be thought of as arising from Laughlin's `anyon superconductivity' mechanism. Thus the Hubbard-Hofstadter model studied here offers a clean and experimentally accessible setup, potentially realizable in moiré heterostructures, for exploring the properties of anyonic matter at finite density and the interplay of topological order, quantum criticality and superconductivity.
We address the problem of a lightly doped spin liquid through a large-scale density-matrix renormalization group study of the t-J model on a kagome lattice with a small but nonzero concentration δ of doped holes. It is now widely accepted that the undoped (δ=0) spin-1/2 Heisenberg antiferromagnet has a spin-liquid ground state. Theoretical arguments have been presented that light doping of such a spin liquid could give rise to a high temperature superconductor or an exotic topological Fermi liquid metal. Instead, we infer that the doped holes form an insulating charge-density wave state with one doped hole per unit cell, i.e., a Wigner crystal. Spin correlations remain short ranged, as in the spin-liquid parent state, from which we infer that the state is a crystal of spinless holons, rather than of holes. Our results may be relevant to kagome lattice herbertsmithite upon doping.
We report a density-matrix renormalization group study of the lightly doped $t\text{\ensuremath{-}}J$ model on a four-leg cylinder with doped hole concentrations per site $\ensuremath{\delta}=5%\text{--}12.5%$. By keeping an unusually large number of states and long system sizes, we are able to accurately document the interplay between superconductivity, spin, and charge-density-wave orders. The long-distance behavior is consistent with that of a Luther-Emery liquid with a spin gap and power-law charge-density-wave and superconducting correlations. This is the widest $t\text{\ensuremath{-}}J$ or Hubbard system in which power-law superconducting correlations have been established.
Abstract We study the ground state properties of the Hubbard model on three-leg triangular cylinders using large-scale density-matrix renormalization group simulations. At half-filling, we identify an intermediate gapless spin liquid phase, which has one gapless spin mode and algebraic spin–spin correlations but exponential decay scalar chiral–chiral correlations, between a metallic phase at weak coupling and Mott insulating dimer phase at strong interaction. Upon light doping the gapless spin liquid, the system exhibits power-law charge-density-wave (CDW) correlations but short-range single-particle, spin–spin, and chiral–chiral correlations. Similar to CDW correlations, the superconducting correlations also decay in power-law but oscillate in sign as a function of distance, which is consistent with the striped pair-density wave. When further doping the gapless spin liquid phase or doping the dimer order phase, another phase takes over, which has similar CDW correlations but all other correlations decay exponentially.