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arXiv:2210.08719 · Frontiers of Physics

A multi-band atomic candle with microwave-dressed Rydberg atoms

Yafen Cai, Shuai Shi, Yijia Zhou, Jianhao Yu, Yali Tian, Yitong Li, Kuan Zhang, Chenhao Du, Weibin Li, Lin Li

Published Nov 23, 2022• 4 citations
arXivHTMLPDF

Abstract

Stabilizing important physical quantities to atom-based standards lies at the heart of modern atomic, molecular and optical physics, and is widely applied to the field of precision metrology. Of particular importance is the atom-based microwave field amplitude stabilizer, the so-called atomic candle. Previous atomic candles are realized with atoms in their ground state, and hence suffer from the lack of frequency band tunability and small stabilization bandwidth, severely limiting their development and potential applications. To tackle these limitations, we employ microwave-dressed Rydberg atoms to realize a novel atomic candle that features multi-band frequency tunability and large stabilization bandwidth. We demonstrate amplitude stabilization of microwave field from C-band to Ka-band, which could be extended to quasi-DC and terahertz fields by exploring abundant Rydberg levels. Our atomic candle achieves stabilization bandwidth of 100 Hz, outperforming previous ones by more than two orders of magnitude. Our simulation indicates the stabilization bandwidth can be further increased up to 100 kHz. Our work paves a route to develop novel electric field control and applications with a noise-resilient, miniaturized, sensitive and broadband atomic candle.

DOI
10.1007/s11467-022-1218-6

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Stabilizing important physical quantities to atom-based standards lies at the heart of modern atomic, molecular and optical physics, and is widely applied to the field of precision metrology. Of particular importance is the atom-based microwave field amplitude stabilizer, the so-called atomic candle. Previous atomic candles are realized with atoms in their ground state, and hence suffer from the lack of frequency band tunability and small stabilization bandwidth, severely limiting their development and potential applications. To tackle these limitations, we employ microwave-dressed Rydberg atoms to realize a novel atomic candle that features multi-band frequency tunability and large stabilization bandwidth. We demonstrate amplitude stabilization of microwave field from C-band to Ka-band, which could be extended to quasi-DC and terahertz fields by exploring abundant Rydberg levels. Our atomic candle achieves stabilization bandwidth of 100 Hz, outperforming previous ones by more than two orders of magnitude. Our simulation indicates the stabilization bandwidth can be further increased up to 100 kHz. Our work paves a route to develop novel electric field control and applications with a noise-resilient, miniaturized, sensitive and broadband atomic candle.
Rydberg atoms, with their giant transition electric dipole moments and abundant energy-level transitions, offer exceptional potential for microwave (MW) electric field sensing, combining high sensitivity and broad frequency coverage. However, simultaneously achieving high sensitivity and broad instantaneous bandwidth in a Rydberg-based MW sensor remains a critical challenge. Here, we propose a multi-dressed-state engineered superheterodyne detection scheme for Rydberg electrometry to overcome this challenge. It is found that the key to simultaneously achieving large instantaneous bandwidth and high sensitivity lies in the coherence of dressed states and the interference between transition channels of dressed states. By strategically engineering the multiple dressed states of Rydberg atoms, we demonstrate a thermal 87Rb\mathrm{^{87}Rb}87Rb vapor-based sensor with a sensitivity of 222.6 \,nV \,cm−1 ^{-1}\,−1Hz−1/2^{-1/2}−1/2 and a record instantaneous bandwidth of 76.8 \,MHz with the local microwave frequency 16.03 \,GHz. This advancement paves the way for Rydberg-atom technologies in radar, wireless communication, and spectrum monitoring.
Just as it is possible to stabilize the frequency of an electromagnetic field to an atomic resonance between energy eigenstates, so too is it possible to stabilize the amplitude (or 'brightness') of a field to atomic parametric resonances, the so-called Rabi-resonances. For ease of reference, and by analogy to the atomic clock, we have coined the term 'atomic candle' for this quantum-mechanical, amplitude-stabilization system. Though the atomic candle was originally developed to stabilize microwave power in gas-cell atomic clocks, thereby eliminating a source of timekeeping instability in these devices, the atomic candle's applications extend well beyond the area of precise timekeeping. Basically, the atomic-candle provides a means for detecting and controlling subtle amplitude changes in electromagnetic fields at very low Fourier frequencies (i.e., f < 0.1 Hz). In the present work, we discuss a number of atomic candle applications: laser stabilization, absorption/refractive-index measurements, observations of cavity mode stability over very long time scales (i.e., 50 days), and measurements of low-frequency absorption/scattering fluctuations along a propagation path.
Broadband Rydberg Atomic Microwave Sensing with 44.6 \,MHz Instantaneous Bandwidth
Rydberg atoms have become a promising novel type of microwave sensor due to their excellent physical properties -- broad frequency coverage and large electric dipole moments. High sensitivity and broad instantaneous bandwidth are two indispensable requirements for deployable Rydberg microwave sensors. However, enabling broadband operation while retaining high sensitivity has been a longstanding barrier limiting their applications. We propose and experimentally demonstrate a Rydberg microwave sensor whose instantaneous bandwidth is significantly enhanced via an auxiliary microwave field. By finely modulating the Rydberg energy levels with this field, we broaden the bandwidth substantially while retaining the sensor's inherent high sensitivity. An instantaneous bandwidth of 44.6 \,MHz ($\pm22.322.322.3\,MHz)withasensitivityof225.7MHz) with a sensitivity of 225.7MHz)withasensitivityof225.7\,nVnVnV\,cmcmcm^{-1}\,HzHzHz^{-1/2}$ is realized in a thermal 87^{87}87Rb vapor with the local microwave frequency of 16.03 \,GHz. Our work delivers concurrent broad instantaneous bandwidth and high sensitivity for Rydberg microwave sensors, paving a technically viable path for their practical deployment in broadband microwave metrology, radar, and wireless communication.
Atomic heterodyne dressed by a local oscillator resonant with Rydberg transitions allows high sensitivity and robust phase measurement of a microwave electric field, but it is typically limited to detection of discrete frequencies within the narrow bandwidth of Rydberg transitions. Here we demonstrate an atomic heterodyne scheme for continuous-frequency electric field measurement based on multilevel Rydberg atoms in a room-temperature vapor cell. Driven by two off-resonant microwaves acting as a tunable local oscillator field, the heterodyne receiver can retrieve the amplitude, phase, and frequency information of signal microwave in a continuous frequency band. In our experiment, the receiver achieves an electric field sensitivity of up to $1.5\phantom{\rule{0.2em}{0ex}}\ensuremath{\mu}\mathrm{V}\phantom{\rule{0.2em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}1}\phantom{\rule{0.2em}{0ex}}{\mathrm{Hz}}^{\ensuremath{-}1/2}$, 80-dB linear dynamic range, and over 1 GHz of continuous frequency range. We also demonstrate the reliable reception of continuously tunable phase-modulated carriers in the digital communication. This work will facilitate the application of atomic heterodyne in the areas such as radar technique, radio monitoring, and radio astronomy.
Rydberg atoms are atoms in their highly excited energy states. The physical properties of Rydberg atoms in the presence of external fields play an important role in quantum precision measurement. In recent years, radio-frequency electric field sensing based on Rydberg atoms has attracted significant interest. It is widely recognized as an electromagnetic sensing system fundamentally different from traditional ones. As a quantum sensor, it is expected to surpass several foundational limitations of traditional receivers, such as sensitivity, dynamic range and frequency bandwidth. It was reported that Rydberg sensing systems can sense microwaves of frequencies from DC up to 1THz. Its quantum nature would possibly avoid internal thermal (Johnson) noise, even at room temperature. Recent demonstrations have also observed high precision for terahertz imaging, strong fields sensing, proof-of-principle communication. However, limitations of this novel system have not been addressed, especially for a practical radar, communication or electronic warfare system. Here in this work, we first compare the architectures of different microwave receivers and then analyze the metrics of Rydberg microwave receivers, such as instantaneous bandwidth and dynamic range based on experimental results. We concluded by pointing out several main obstacles to overcome for realizing a practical state-of-the-art microwave receiver.
Rydberg atoms are neutral atoms excited to high principal quantum number states, which endows them with exaggerated properties such as large electric dipole moments, long lifetimes, and extreme sensitivity to external electromagnetic fields. These characteristics form the foundation of Rydberg atom-based sensors, an emerging class of quantum devices capable of optically detecting electric fields across frequencies from DC to the terahertz regime. Rydberg-based electrometry operates through both Autler–Townes (AT) splitting of resonant Rydberg transitions and Stark-shift measurements for high-frequency or far-detuned fields, enabling broadband field sensing from DC to the THz regime. Using ladder-type electromagnetically induced transparency (EIT) and AT splitting, these sensors enable non-invasive, SI-traceable measurements of field amplitude, frequency, phase, and polarization. Recent developments have demonstrated broadband electric field probes, voltage calibration standards, and compact RF receivers based on thermal vapor cells and integrated photonic architectures. Furthermore, innovations in multi-photon EIT, superheterodyne readout, and multi wave mixing have expanded the dynamic range and bandwidth of Rydberg-based electrometry. Despite challenges related to environmental perturbations, linewidth broadening, and laser stabilization, ongoing advances in atomic control, hybrid photonic integration, and EIT-based readout promise scalable, chip-compatible sensors. This review summarizes the physical principles, experimental progress, and emerging applications of Rydberg atom-based sensing, emphasizing their potential for next generation quantum metrology, wireless communication, and precision field mapping.