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arXiv:2210.04691 · Frontiers in Quantum Science and Technology

Detection of infrared light through stimulated four-wave mixing process

Weihang Zhang, Jing-Yuan Peng, Enze Li, Ying-Hao Ye, Lei Zeng, Ming‐Xin Dong, Dong-Sheng Ding, Bao‐Sen Shi

Published Aug 25, 2022• 2 citations

Abstract

Infrared optical measurement has a wide range of applications in industry and science, but infrared light detectors suffer from high costs and inferior performance than visible light detectors. Four-wave mixing (FWM) process allows detection in the infrared range by detecting correlated visible light. We experimentally investigate the stimulated FWM process in a hot 85Rb atomic vapor cell, in which a weak infrared signal laser at 1,530 nm induces the FWM process and is amplified and converted into a strong FWM light at 780 nm, the latter can be detected more easily. We find the optimized single- and two-photon detunings by studying the dependence of the frequency of input laser on the generated FWM light. What’s more, the power gain increases rapidly as the signal intensity decreases, which is consistent with our theoretical analysis. As a result, the power gain can reach up to 500 at a signal laser power of 0.1 μW and the number of detected photons increased by a factor of 250. Finally, we experimentally prove that our amplification process can work in a broad band in the frequency domain by exploring the response rate of our stimulated FWM process.

DOI: 10.3389/frqst.2022.984638

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Abstract We demonstrate 1.37 µ m coherent near-infrared light generation via self-seeded parametric four-wave mixing (FWM) process in Rb atomic vapor. Two lasers (780 nm and 776 nm) in the co-propagating configuration, drive the Rb atoms from the 5S 1/2 ground state to the 5D 5/2 excited state. The parametric FWM around the 5P 3/2 –5D 5/2 –6P 3/2 –6S 1/2 –5P 3/2 transition loop is effectively established under phase matching conditions. The generated coherent light wavelength is confirmed using an optical spectrum analyzer, and the output power is investigated with the input laser frequency, power and atomic density. Consequently, a 1.37 µ m coherent light with the power of 27 µ W and the beam quality of M x 2 = 1.22 and M y 2 = 1.25 is obtained. An additional 795 nm laser is introduced to enhance the output power by 1.5 times through velocity-selective optical hyperfine repumping.

We have demonstrated experimentally that infrared light at 1529.4 nm can be converted into the visible at 780 nm with 54% efficiency through a ladder-type atomic configuration in 85Rb. Specifically we theoretically analyze that high efficiency is due to the large nonlinear dispersion of the index of refraction from the off-resonant enhancement in a four-wave mixing (FWM) process. By using two perpendicular polarized pump fields, the coherence of two FWM processes in this configuration is verified.

Diode-pumped alkali lasers, possessing high efficiency and narrow linewidth, can provide feasible solutions for wavelength ranges difficult to reach by commercial lasers. In this study, we investigate a generation of coherent blue light (CBL) via four-wave mixing (FWM)-based up-conversion processes in cesium (Cs) vapor. A bichromatic pumping scheme with 852- and 917-nm lasers drives the Cs atoms to the 6 D 5/2 excited level, followed by cascaded decay of 6 D 5/2 → 7 P 3/2 → 6 S 1/2 , producing 456-nm CBL under phase matching conditions. The fluorescence in multiple bands from blue to near- and far-infrared in the FWM process is demonstrated under different experimental conditions. To optimize the experimental parameters, we investigate the dependence of 456-nm CBL on the vapor temperature, frequency, and intensity of the two pump lasers. A maximum power of 2.94 mW is achieved with pump powers of 430 mW (for 852 nm) and 470 mW (for 917 nm). The corresponding conversion efficiency is 1.5%/W, three-fold higher than those in previous studies. Our results can contribute to fundamental research on atom—photon interactions and quantum metrology.

As an essential quantum resource, the intensity-difference squeezed state based on four-wave mixing (FWM) in atomic vapor is widely applied in quantum information processing. In particular, a high intensity-difference squeezing bandwidth is vital for the realization of high-speed information processing. However, limited by the bandwidth of photodetectors, broadband intensity-difference squeezed state based on this system has not yet been reported. Here, we developed a transimpedance broadband balanced homodyne detector at 895 nm, achieving a bandwidth greater than 100 MHz and a maximum signal-to-noise ratio of 15 dB with 4 mW optical power. Utilizing this detector in a nondegenerate FWM process based on cesium vapor, we experimentally achieved broadband intensity-difference squeezing with a bandwidth of 100 MHz, which yielded a maximum squeezing of −7.17 ± 0.8 dB between 20 and 40 MHz. Meanwhile, using this detector, we experimentally investigated the cavity-enhanced FWM process, achieving a squeezing level of −6.07 ± 0.5 dB within a 4 MHz frequency range, which is limited by the cavity bandwidth. This work provides a reliable detection tool and experimental foundation for the research and application of broadband squeezed light sources based on FWM.

Phase-sensitive nonlinear gain processes have been implemented as noise-reduced optical amplifiers, which have the potential to achieve signal-to-noise ratios beyond the classical limit. We experimentally demonstrate a novel phase-sensitive four-wave mixing amplification process in a single atomic vapor cell with only two input frequencies and two input vacuum modes. The amount of phase sensitivity depends on the power ratio between the inserted probes as well as on the input frequency of the probes. We find that, for certain phase values, the intensity noise of an output mode is lower than that of its phase-insensitive counterpart.