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arXiv:2210.03835 · Physical Review A

Micromotion-synchronized pulsed Doppler cooling of trapped ions

Alexander Kato, ANDREI NOMEROTSKI, B. B. Blinov

Published Feb 27, 2023• 4 citations
arXivHTMLPDF

Abstract

We propose and demonstrate a method for Doppler cooling trapped-ion crystals where the distribution of micromotion amplitudes may be large and uneven. The technique uses pulses of Doppler cooling light synchronized with the trap rf that selectively target ions when their velocity is near a node, leading to more uniform cooling across a crystal by a single tone of cooling light. We lay out a theoretical framework that describes where this technique is practical and provides a simple experimental demonstration.

DOI
10.1103/physreva.107.023116

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We propose and demonstrate a method for Doppler cooling trapped-ion crystals where the distribution of micromotion amplitudes may be large and uneven. The technique uses pulses of Doppler cooling light synchronized with the trap rf that selectively target ions when their velocity is near a node, leading to more uniform cooling across a crystal by a single tone of cooling light. We lay out a theoretical framework that describes where this technique is practical and provides a simple experimental demonstration.
We study the Doppler-cooling of radial two-dimensional (2D) Coulomb crystals of trapped barium ions in a radiofrequency trap. Ions in radial 2D crystals experience micromotion of an amplitude that increases linearly with the distance from the trap center, leading to a position-dependent frequency modulation of laser light in each ion's rest frame. We use two tones of Doppler-cooling laser light separated by approximately 100 MHz to efficiently cool distinct regions in the crystals with differing amplitudes of micromotion. This technique allows us to trap and cool more than 50 ions populating four shells in a radial 2D crystal, where with a single tone of Doppler cooling light we are limited to 30 ions in three shells. We also individually characterize the micromotion of all ions within the crystals and use this information to locate the center of the trap and to determine the Matthieu parameters qx{q}_{x}qx​ and qy{q}_{y}qy​.
Several groups have recently used laser cooling to produce ordered arrays of ions, ion crystals, in rf quadrupole ion traps (Paul traps). Laser cooling has been understood using previous theories which ignore ion micromotion and replace the oscillating rf trap potential with a static pseudopotential. We show that in recent experiments, ion micromotion can exceed one wavelength of the cooling radiation and that the resulting Doppler shifts can transform laser cooling into laser heating. Changes in trap voltage, ion position, and laser intensity can all reverse the sign of laser cooling. This, together with ideas of deterministic chaos, can lead to a reinterpretation of experiments on ion crystals. The recognition that effects previously attributed to an experimental artifact, rf heating, may actually be due to a failure of laser cooling opens the door, on the one hand, to precise theories of phase transitions and, on the other, to improved cooling techniques that can permit the creation of larger ion crystals.
We propose a sub-Doppler cooling scheme for trapped-ion crystals in Paul traps. The combination of a hollow tweezer and microwave drive creates an effective two-level system which is cooled through attractive Sisyphus cooling. For 171Yb+{}^{171}\rm{Yb}^+171Yb+ ions, we numerically identify optimal parameters for one- and two-ion crystals, and investigate the cooling rate in ion crystals with up to three ions. Our cooling scheme utilizes a single ion addressed with a tweezer to achieve sub-Doppler cooling of the NNN axial motional modes perpendicular to the tweezer propagation direction, does not rely on the Lamb-Dicke regime and uses off-resonant light. We reach 1/e1/e1/e cooling times for the center of mass mode of τcom<2τ_{\rm com}<2τcom​<2 ms, and a steady-state excitation number of nˉcom≈0.7\bar{n}_{\rm{com}}\approx 0.7nˉcom​≈0.7. Our scheme is well-suited as an intermediate stage between Doppler cooling and ground-state sideband cooling, and can be readily realized in trapped-ion platforms.
Laser cooling typically requires one or more repump lasers to clear dark states and enable recycling transitions. Here, we have achieved cooling of Be+ ions using a single laser beam, facilitated by one-dimensional heating through micromotion. By manipulating the displacement from the trap's nodal line, we precisely controlled the ion micromotion direction and speed, reaching up to 3144 m/s, which corresponds to a 7.1 GHz Doppler frequency shift in our experiment. This approach eliminates the necessity of a 1.25 GHz offset repump laser while keeping the Be+ ions cold in the perpendicular direction. Measurements were taken using cooling laser detuning and imaging of ion trajectories. Molecular dynamics simulations, based on machine learned time-dependent electric field E(X, Y, Z, t) inside the trap, accurately reproduced the experimental observation, illuminating the relationship between the direction of micromotion and the trapping electric filed vector. This work not only provides a robust method for managing the micromotion velocity of ions but also sheds light on laser cooling complex systems that require multiple repumping lasers. Additionally, it offers a method for controlling energy in the context of ion-molecule collision investigations.
In this paper, direct observation of micromotion for multiple ions in a laser-cooled trapped ion crystal is discussed along with a measurement technique for micromotion amplitude. Micromotion is directly observed using a time-resolving, single-photon-sensitive camera that provides both fluorescence and position data for each ion on the nanosecond time scale. Micromotion amplitude and phase for each ion in the crystal are measured, allowing this method to be sensitive to tilts and shifts of the ion chain from the null of the radio-frequency quadrupole potential in the linear trap. Spatial resolution makes this micromotion detection technique suitable for complex ion configurations, including two-dimensional geometries. It does not require any additional equipment or laser beams, and the modulation of the cooling lasers or trap voltages is not necessary for detection as it is in other methods.