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arXiv:2209.10403 · Physical Review A

Probing dressed states and quantum nonlinearities in a strongly coupled three-qubit waveguide system under optical pumping

Sofia Arranz Regidor, Stephen Hughes

Published Sep 27, 2023• 5 citations
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Abstract

We study a three-qubit waveguide system in the presence of optical pumping, when the side qubits act as atomlike mirrors, manifesting in a strong light-matter coupling regime. The qubits are modeled as two-level systems, where we account for important saturation effects and quantum nonlinearities. Optically pumping this system into a nonlinear regime is shown to lead to a rich manifold of dressed states that can be seen in the emitted spectrum, and we show two different theoretical solutions using a medium-dependent master-equation model in the Markovian limit, as well as using matrix product states without invoking any Markov approximations. We demonstrate how a rich nonlinear spectrum is obtained by varying the relative decay rates of the mirror qubits as well as their spatial separation and show the limitations of using a Markovian master equation. Our model allows one to directly model giant-atom phenomena, while including important retardation effects and multiphoton nonlinearities. We also show how the excited three-qubit system, in a strong-coupling regime, deviates significantly from a Jaynes-Cummings model when entering the nonlinear regime.

DOI
10.1103/physreva.108.033719

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We study a three-qubit waveguide system in the presence of optical pumping, when the side qubits act as atomlike mirrors, manifesting in a strong light-matter coupling regime. The qubits are modeled as two-level systems, where we account for important saturation effects and quantum nonlinearities. Optically pumping this system into a nonlinear regime is shown to lead to a rich manifold of dressed states that can be seen in the emitted spectrum, and we show two different theoretical solutions using a medium-dependent master-equation model in the Markovian limit, as well as using matrix product states without invoking any Markov approximations. We demonstrate how a rich nonlinear spectrum is obtained by varying the relative decay rates of the mirror qubits as well as their spatial separation and show the limitations of using a Markovian master equation. Our model allows one to directly model giant-atom phenomena, while including important retardation effects and multiphoton nonlinearities. We also show how the excited three-qubit system, in a strong-coupling regime, deviates significantly from a Jaynes-Cummings model when entering the nonlinear regime.
We introduce a three-qubit waveguide-QED system to achieve a cavity-QED strong-coupling regime for a probe qubit embedded in atomlike mirrors, which was realized in recent experiments. We then extend this system into the deep non-Markovian regime and demonstrate the profound role that retardation plays on the dressed resonances, allowing one to significantly improve the polariton lifetimes (by several orders of magnitude), tune the resonances, as well as realize Fano-like resonances and simultaneous coupling to multiple cavity modes. Exact Green's function solutions are presented for the classical spectral resonances, and the full quantum dynamics are simulated using matrix product states, where we demonstrate additional control of the cavity-QED system using chiral probe qubits. We show example qubit dynamics with both one and two quantum excitations.
We study a two-level system (atom, superconducting qubit, or quantum dot) strongly coupled to a single photonic mode of a cavity, in the presence of incoherent pumping and including detuning and dephasing. This system displays a striking quantum-to-classical transition. On the grounds of several approximations that reproduce to various degrees exact results obtained numerically, we separate five regimes of operations, that we term ``linear,'' ``quantum,'' ``lasing,'' ``quenching,'' and ``thermal.'' In the fully quantized picture, the lasing regime arises as a condensation of dressed states and manifests itself as a Mollow triplet structure in the direct emitter photoluminescence spectrum, which embeds fundamental features of the full-field quantization description of light-matter interaction.
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We theoretically investigate quantum Rabi oscillations in a system consisting of a two-level atom (qubit) strongly coupled to a one-dimensional open waveguide. In contrast to conventional cavity quantum electrodynamics, the qubit interacts with a continuum of propagating modes, which gives rise to fundamentally different dynamical behavior. Within the rotating-wave approximation, we express the multimode Jaynes-Cummings Hamiltonian in terms of collective bosonic operators and show that the system possesses two integrals of motion, enabling an exact diagonalization of the Hamiltonian in the single-excitation subspace. We show that for a strongly interacting qubit-photon system, the dynamics are captured by a reduced two-level model. In this framework, each level is defined as the product of the atomic excited state and a specific field mode, which takes the form of a multiphoton Fock-like state. In this picture, the Rabi oscillations represent a collective phenomenon corresponding to oscillations between multiphoton states differing by a single photon. We then extend our analysis to multiphoton processes in which the initial field is a coherent state with a continuous spectrum. In this case, the Rabi frequency is shown to be sensitive to the spectral profile of the function that generates the coherent state.
Light and matter can be unified under the strong coupling regime, creating superpositions of both, called dressed states or polaritons. After initially being demonstrated in bulk semiconductors and atomic systems ,strong coupling phenomena have been realized in solid state optical microcavities. They form an essential ingredient in the exciting physics spanning from many-body quantum coherence phenomena, like Bose-Einstein condensation and superfluidity, to cavity quantum electrodynamics (cQED). A widely used approach within cQED is the Jaynes-Cummings (JC) model that describes the interaction of a single fermionic two-level system with a single bosonic photon mode. For a photon number larger than one, known as quantum strong coupling (QSC), a significant anharmonicity is predicted for the ladder-like spectrum of dressed states. For optical transitions in semiconductor nanostructures, first signatures of the quantum strong coupling were recently published. In our latest report we applied advanced coherent nonlinear spectroscopy to explore a strongly coupled exciton-cavity system. Specifically, we measured and simulated its four-wave mixing (FWM) response, granting direct access to the first two rungs of the JC ladder. This paper summarizes the main results of Ref. 15 and adds FWM experiments obtained on a micropillar cavity in which a doublet of quantum dot (QD) excitons interacts with the cavity mode in the limit of weak to strong coupling.
We study the quantum nonlinear dynamics of multiple two-level atoms (qubits) in a waveguide quantum electrodynamics system, with a focus on modified superradiance effects between two or four atoms with finite delay times. Using a numerically exact matrix-product-states approach, we explore both Markovian and non-Markovian regimes and highlight the significant influence of time-delayed feedback effects and the clear breakdown of assuming instantaneous coupling dynamics. We first show a system composed of two spatially separated qubits, prepared in a doubly excited state (both fully excited), and provide a comprehensive study of how delayed feedback influences the collective system decay rates, as well as the quantum correlations between waveguide photons, atoms, and between atoms and photons. The system is then extended to include two additional qubits located next to the initial ones (four qubits in total), and we demonstrate, by manipulating the initial excitations and the time-delay effects, how long-term quantum correlations and light-matter entangled states can be established.