We study the quantum nonlinear dynamics of multiple two-level atoms (qubits) in a waveguide quantum electrodynamics system, with a focus on modified superradiance effects between two or four atoms with finite delay times. Using a numerically exact matrix-product-states approach, we explore both Markovian and non-Markovian regimes and highlight the significant influence of time-delayed feedback effects and the clear breakdown of assuming instantaneous coupling dynamics. We first show a system composed of two spatially separated qubits, prepared in a doubly excited state (both fully excited), and provide a comprehensive study of how delayed feedback influences the collective system decay rates, as well as the quantum correlations between waveguide photons, atoms, and between atoms and photons. The system is then extended to include two additional qubits located next to the initial ones (four qubits in total), and we demonstrate, by manipulating the initial excitations and the time-delay effects, how long-term quantum correlations and light-matter entangled states can be established.
We study the quantum nonlinear dynamics of multiple two-level atoms (qubits) in a waveguide quantum electrodynamics system, with a focus on modified superradiance effects between two or four atoms with finite delay times. Using a numerically exact matrix-product-states approach, we explore both Markovian and non-Markovian regimes and highlight the significant influence of time-delayed feedback effects and the clear breakdown of assuming instantaneous coupling dynamics. We first show a system composed of two spatially separated qubits, prepared in a doubly excited state (both fully excited), and provide a comprehensive study of how delayed feedback influences the collective system decay rates, as well as the quantum correlations between waveguide photons, atoms, and between atoms and photons. The system is then extended to include two additional qubits located next to the initial ones (four qubits in total), and we demonstrate, by manipulating the initial excitations and the time-delay effects, how long-term quantum correlations and light-matter entangled states can be established.
We study the quantum dynamics of multiple two-level atoms (qubits) in a waveguide quantum electrodynamics system, with a focus on modified superradiance effects between two or four atoms with finite delay times. Using a numerically exact matrix product approach, we explore both Markovian and non-Markovian regimes, and highlight the significant influence of time-delayed feedback effects and the clear breakdown of assuming instantaneous coupling dynamics. We first show a system composed of two spatially separated qubits, prepared in a doubly excited state (both fully excited), and provide a comprehensive study of how delayed feedback influences the collective system decay rates, as well as the quantum correlations between waveguide photons, atoms, and between atom and photons. The system is then extended to include two additional qubits located next to the initial ones (four qubits in total), and we demonstrate, by manipulating the initial excitations and the time-delay effects, how long-term quantum correlations and light-matter entangled states can be established.
The model of light-matter interaction in quantum electrodynamics typically relies on the Markovian approximation, which assumes that the system's future evolution depends solely on its current state, effectively treating it as a ``memoryless" process. However, this approximation is not valid in scenarios when retardation effects are significant. These memory and retardation effects have the potential to improve existing quantum technologies (e.g., large-scale quantum networks, quantum information processing) and unlock new phenomena for future applications. In this work, we show theory and experiments of a time-delayed coherent feedback system using a transmon artificial atom (treated as a qubit) embedded in a superconducting circuit waveguide, in both linear and nonlinear excitation regimes. By using a feedback loop with a delay time comparable to the qubit relaxation time, pronounced non-Markovian effects appear in the dynamics of the qubit evolution. We also show how the resonance fluorescence spectrum, including elastic and inelastic scattering (such as the well-known Mollow triplet), can be significantly modified through the interaction between the qubit and feedback loop to show genuine non-Markovian and quantum nonlinear phenomena that cannot be explained with instantaneous coupling parameters. This work presents the first experimental report of Mollow triplets in the non-Markovian regime.
An array of initially excited emitters coupled to a one-dimensional waveguide exhibits superradiant decay under the Born-Markov approximation, manifested as a coherent burst of photons in the output field. In this work, we employ tensor-network methods to investigate its non-Markovian dynamics induced by finite time delays in photon exchange among the emitters. We find that the superradiant burst breaks into a structured train of correlated photons, each intensity peak corresponding to a specific photon number. We quantify the emitter-photon and emitter-emitter entanglement generated during this process and show that the latter emerges in the long-time limit, as part of the excitation becomes trapped within the emitters' singlet subspace. We finally consider the decay of the system's most radiant state, the symmetric Dicke state, and show that time delay can lead to decay rates exceeding those predicted by the Markovian approximation.
To continue developing quantum technologies, such as quantum computing, quantum communication and quantum cryptography, we need reliable sources of quantum states of light. These quantum states of light can come in many forms; single photons, entangled pairs, bunched and anti-bunched light, all have uses in current quantum technologies, but for the best performance, this light must maintain its coherence. Time-delayed coherent feedback is a passive feedback method proposed for waveguide quantum electrodynamic systems to improve their performance and unlock new quantum optical phenomena. Additionally, due to its underlying non-Markovian dynamics, feedback is also an interesting theoretical problem to study. In this thesis, we use a quantum trajectory discretized waveguide (QTDW) model to simulate feedback dynamics and investigate its effects in a variety of applications. Originally proposed by Whalen in 2018, we develop the QTDW model beyond its initial implementation to now calculate quantum correlation functions, output spectra, waiting time distributions, and single photon source figures of merit. First, we present an explanation of quantum trajectory theory which is used to model the time dynamics in the QTDW approach, and discuss feedback in the linear regime to highlight the differences between Markovian and non-Markovian dynamics with coherent feedback. We next present nonlinear spectra and multi-photon effects from coherent feedback highlighting how the typical Mollow triplet is dressed by the feedback to create new resonances in the output field. This is followed by a collaborative theory and experiment work which observed our predicted non-Markovian signatures in the nonlinear output spectrum along with new non-Markovian phenomena in the linear regime. We then investigate how pulse-triggered single photon sources can be improved through the inclusion of a time-delayed coherent feedback, presenting the possible improvement to the performance figures of merit. Lastly, the modeling techniques developed for single photon sources with feedback are used to compare the performance of three new off-resonant driving techniques for on-demand single photon sources. These findings show time-delayed coherent feedback is an excellent degree of control to include in future waveguide quantum electrodynamic systems to unlock better performance and new phenomena in the system under investigation.
Abstract This work introduces a theoretical framework to model the collective dynamics of quantum emitters in highly non-Markovian environments, interacting through the exchange of photons with significant retardations. The formalism consists on a set of coupled delay differential equations for the emitter’s raising/lowering operators σ i ± , supplemented by input–output relations that describe the field mediating the interactions. These equations capture the dynamics of both linear (bosonic) and nonlinear (two-level) emitter arrays. It is exact in some limits—e.g. bosonic emitters or generic systems with up to one collective excitation—and can be integrated to provide accurate results for larger numbers of photons. These equations support a study of collective spontaneous emission of emitter arrays in open waveguide-QED environments. This study uncovers an effect we term cascaded super- and sub-radiance, characterized by light-cone-limited propagation and increasingly correlated photon emission across distant emitters. The collective nature of this dynamics for two-level systems is evident both in the enhancement of collective emission rates, as well as in a superradiant burst with a faster than linear growth. While these effects should be observable in existing circuit QED devices or slight generalizations thereof, the formalism put forward in this work can be extended to model other systems such as network of quantum emitters or the generation of correlated photon states.
We present two different methods for modeling non-Markovian quantum light-matter interactions in waveguide QED systems, using matrix product states (MPSs) and a space-discretized waveguide (SDW) model.After describing the general theory and implementation of both approaches, we compare and contrast these methods directly on three topical problems of interest in waveguide-QED, including (i) a two-level system (TLS) coupled to an infinite (one-dimensional) waveguide, (ii) a TLS coupled to a terminated waveguide with a time-delayed coherent feedback, and (iii) two spatially separated TLSs coupled within an infinite waveguide.Both approaches are shown to efficiently describe multiphoton nonlinear dynamics in highly non-Markovian regimes, and we highlight the advantages and disadvantages of these methods for modeling waveguide QED interactions, including their implementation in PYTHON, computational run times, and ease of conceptual understanding.We explore both vacuum dynamics as well as regimes of strong optical pumping, where a weak excitation approximation cannot be applied.The MPS approach scales better when modeling multiphoton dynamics and long delay times and explicitly includes non-Markovian memory effects.In contrast, the SDW model accounts for non-Markovian effects through space discretization and solves Markovian equations of motion, yet rigorously includes the effects of retardation.The SDW model, based on an extension of recent collisional pictures in quantum optics, is solved through quantum trajectory techniques and can more easily add in additional dissipation processes, including off-chip decay and TLS pure dephasing.The impact of these processes is shown directly on feedback-induced population trapping and TLS entanglement between spatially separated TLSs.