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arXiv:2209.05422 · Physical Review Letters

Quantification of Quantum Correlations in Two-Beam Gaussian States Using Photon-Number Measurements

Artur Barasiński, Jan Peřina, Antonín Černoch

Published Jan 24, 2023• 6 citations
arXivHTMLPDF

Abstract

Identification, and subsequent quantification of quantum correlations, is critical for understanding, controlling, and engineering quantum devices and processes. We derive and implement a general method to quantify various forms of quantum correlations using solely the experimental intensity moments up to the fourth order. This is possible as these moments allow for an exact determination of the global and marginal impurities of two-beam Gaussian fields. This leads to the determination of steering, tight lower and upper bounds for the negativity, and the Kullback-Leibler divergence used as a quantifier of state nonseparability. The principal squeezing variances are determined as well using the intensity moments. The approach is demonstrated on the experimental twin beams with increasing intensity and the squeezed super-Gaussian beams composed of photon pairs. Our method is readily applicable to multibeam Gaussian fields to characterize their quantum correlations.

DOI
10.1103/physrevlett.130.043603

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Identification, and subsequent quantification of quantum correlations, is critical for understanding, controlling, and engineering quantum devices and processes. We derive and implement a general method to quantify various forms of quantum correlations using solely the experimental intensity moments up to the fourth order. This is possible as these moments allow for an exact determination of the global and marginal impurities of two-beam Gaussian fields. This leads to the determination of steering, tight lower and upper bounds for the negativity, and the Kullback-Leibler divergence used as a quantifier of state nonseparability. The principal squeezing variances are determined as well using the intensity moments. The approach is demonstrated on the experimental twin beams with increasing intensity and the squeezed super-Gaussian beams composed of photon pairs. Our method is readily applicable to multibeam Gaussian fields to characterize their quantum correlations.
Quantum universal invariants of general N -beam Gaussian fields are investigated from the point of view of fields' intensity moments. A method that uniquely links these invariants, including the global and marginal fields' purities, to intensity moments is suggested. Determination of these invariants identifies the Gaussian states including their quantum correlations. In particular, the Peres-Horodecki separability criterion is reformulated in terms of quantum universal invariants, and consequently in terms of experimental intensity moments, offering a practical tool for determining the entanglement or separability of these states. The approach is experimentally demonstrated by determining the invariants of noisy symmetric three-beam Gaussian states using photon-number resolved measurements. Furthermore, their entanglement properties are analyzed and characterized.
Quantum correlations of symmetric three-beam Gaussian states are analyzed using their quantum universal invariants. These invariants, one-, two-, and three-beam purities, are expressed in terms of the beams’ intensity moments up to sixth order. The three-beam symmetric Gaussian states with varying amounts of the noise are experimentally generated using entangled photon pairs from down-conversion, their invariants are determined, and their quantum correlations are quantified. The coexistence of bipartite and tripartite entanglement and genuine tripartite entanglement is observed in these states that resemble the noisy GHZ/W states.
Gradual loss of the entanglement of a twin beam containing around 25 photon pairs with the increasing external noise is experimentally investigated. The entanglement is quantified by the nonclassicality depths and the nonclassicality counting parameters related to several nonclassicality criteria. The reduction of intensity moments of the analyzed multimode twin beams to single-mode ones allows determination of the negativity as another quantifier of the entanglement. Both the raw photocount histograms and the reconstructed photon-number distributions are analyzed in parallel.
Gaussian states are an essential building block for various applications in quantum optics and quantum information science, yet the precise relation between their second- and third-order correlation functions remains not fully explored. We discuss connections between these correlation functions by constructing an explicit decomposition formula for arbitrary sixth-order moments of ladder operators for general Gaussian states and demonstrate how the derived relations enable state classification from correlation data alone. Whereas violating these relations certifies non-Gaussianity, satisfying them provides evidence for a Gaussian-state description and allows a direct distinction among nondisplaced, nonsqueezed, and displaced-squeezed sectors of the Gaussian state space. Furthermore, we show that it is not possible to uniquely extract state parameters solely from correlation-function measurements without prior assumptions about the Gaussian state. Resolving this ambiguity requires additional loss-sensitive information, e.g., measuring the mean intensity or the vacuum overlap of each mode. In particular, we show under which circumstances these measurements can be used to reconstruct a generic Gaussian state.
Two-beam states obtained by partial photon-number-resolving detection in one beam of a multi-mode twin beam are experimentally investigated using an intensified CCD camera. In these states, sub-Poissonian photon-number distributions in one beam are accompanied by sub-shot-noise fluctuations in the photon-number difference of both beams. Multi-mode character of the twin beam implying the beam nearly Poissonian statistics is critical for reaching sub-Poissonian photon-number distributions, which contrasts with the use of a two-mode squeezed vacuum state. Relative intensities of both nonclassical effects as they depend on the generation conditions are investigated both theoretically and experimentally using photon-number distributions of these fields. Fano factor, noise-reduction parameter, local and global nonclassicality depths, degree of photon-number coherence, mutual entropy as a non-Gaussianity quantifier, and negative quasi-distributions of integrated intensities are used to characterize these fields. Spatial photon-pair correlations as means for improving the field properties are employed. These states are appealing for quantum metrology and imaging including the virtual-state entangled-photon spectroscopy.
Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteria provide for two relevant entanglement measures: the best separable approximation and the generalized robustness. This yields a practical method for quantifying entanglement in realistic experimental situations, in particular, when only few measurements of simple observables are available. As a concrete application of this method, we quantify bipartite and multipartite entanglement in spin-squeezed Bose-Einstein condensates of ∼500 atoms, by lower bounding the best separable approximation and the generalized robustness only from measurements of first and second moments of the collective spin operator.