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arXiv:2209.02583 · Physical Review Applied

Rydberg-Atom-Based Electrometry Using a Self-Heterodyne Frequency-Comb Readout and Preparation Scheme

Katelyn Dixon, Kent A. Nickerson, Donald W. Booth, James P. Shaffer

Published Mar 23, 2023• 35 citations
arXivHTMLPDF

Abstract

Atom-based radio-frequency (rf) electromagnetic field sensing using atomic Rydberg states is a promising technique that has recently attracted significant interest. Its unique advantages, such as extraordinary bandwidth, self-calibration, and all-dielectric sensors, are a tangible improvement over antenna-based methods in applications such as test and measurement and development of broad-bandwidth receivers. Here, we demonstrate how an optical-frequency comb can be used to acquire data in the Autler-Townes regime of Rydberg-atom-based electrometry in a massively parallel fashion, eliminating the need for laser scanning. Two-photon electromagnetically induced transparency readout and preparation of cesium is used for the demonstration. A flat quasicontinuous optical comb is generated with the probe laser at 852 nm using an electro-optic modulator and arbitrary waveform generator. A single-frequency coupling laser at 509 nm is tuned to the Rydberg launch state. An enhanced transmission signal is obtained using self-heterodyne spectroscopy, where the comb signal is beat against a local oscillator derived from the single-frequency probe laser on a fast photodiode. The transmission of each probe-laser comb tooth is observed. We resolve electromagnetically induced transparency peaks with line widths below 5 MHz, with and without laser locking. Radio-frequency electromagnetic fields as low as $66\phantom{\rule{0.2em}{0ex}}\text{\ensuremath{\mu}}{\mathrm{Vcm}}^{\ensuremath{-}1}$ are detected, with sensitivities of $2.3\phantom{\rule{0.2em}{0ex}}\text{\ensuremath{\mu}}{\mathrm{Vcm}}^{\ensuremath{-}1}{\mathrm{Hz}}^{\ensuremath{-}1/2}$. The method offers a significant advantage for reading out electromagnetically induced transparency and Autler-Townes splitting, as neither laser needs to be scanned and slow frequency drifts can be tolerated in some applications. The method enables the detection of the amplitude of a pulsed rf electromagnetic field when the incoming pulse Autler-Townes splits the electromagnetically induced transparency peak.

DOI
10.1103/physrevapplied.19.034078

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Rydberg atom radio-frequency sensors are a unique platform for precision electromagnetic field measurement; e.g., they have extraordinary carrier bandwidth spanning MHz to THz and can be self-calibrated. These photonic sensors use lasers to prepare and read out the atomic response to a radio-frequency electromagnetic field. Most work on Rydberg atom sensors centers on radio-frequency electric field strength because the sensor functions as a square law detector, unless an external radio-frequency heterodyning field is used. A heterodyning field acts as a local oscillator and enables phase readout at the expense of the radio-frequency equipment necessary to generate it. In order to overcome the disadvantages of a radio-frequency local oscillator, we investigate all-optical phase-sensitive detection using a five-level closed-loop excitation scheme. We show that under finite detuning of the loop fields, the atomic response oscillates at the frequency of the detuning. The oscillation is transferred to a probe laser absorption signal. The phase, frequency, and amplitude of the radio-frequency signal are imprinted on the oscillatory dynamics and can be determined using demodulation and matched filter techniques applied to the probe laser transmission signal.
Rydberg atom-based electrometry is a pivotal technology that enables radio-frequency (rf) field measurements traceable to the International System of Units. This is typically accomplished by converting the direct rf power measurement of classical probes to a frequency measurement referenced to two well-defined spectral features, a commercial wavemeter, or narrow cavity lines produced via clock disciplined electro-optic modulators, although there exist cases where none of these are available. In this article, we demonstrate that a known rf frequency scale can be used to infer a laser's frequency scan using Autler-Townes (AT) splitting. In other words, we show that frequency-axis calibration can be achieved using the avoided-crossing behavior of near-resonant rf radiation. The relative separation between AT-split features is measured as a function of an applied rf field's power and detuning from atomic resonance. These peak separations are then fit to a simple, two-level model using a weighted nonlinear least-squares regression analysis that utilizes three fitting parameters, one of which is the desired calibration factor. While we do not benchmark this method against an absolute frequency reference, we do show that this method is (1) consistent with calibration via known fine-structure separation to within approximately 1.11% or better, and (2) robust against substantial experimental deviation from the system's known rf power dependence.
Rydberg atoms are neutral atoms excited to high principal quantum number states, which endows them with exaggerated properties such as large electric dipole moments, long lifetimes, and extreme sensitivity to external electromagnetic fields. These characteristics form the foundation of Rydberg atom-based sensors, an emerging class of quantum devices capable of optically detecting electric fields across frequencies from DC to the terahertz regime. Rydberg-based electrometry operates through both Autler–Townes (AT) splitting of resonant Rydberg transitions and Stark-shift measurements for high-frequency or far-detuned fields, enabling broadband field sensing from DC to the THz regime. Using ladder-type electromagnetically induced transparency (EIT) and AT splitting, these sensors enable non-invasive, SI-traceable measurements of field amplitude, frequency, phase, and polarization. Recent developments have demonstrated broadband electric field probes, voltage calibration standards, and compact RF receivers based on thermal vapor cells and integrated photonic architectures. Furthermore, innovations in multi-photon EIT, superheterodyne readout, and multi wave mixing have expanded the dynamic range and bandwidth of Rydberg-based electrometry. Despite challenges related to environmental perturbations, linewidth broadening, and laser stabilization, ongoing advances in atomic control, hybrid photonic integration, and EIT-based readout promise scalable, chip-compatible sensors. This review summarizes the physical principles, experimental progress, and emerging applications of Rydberg atom-based sensing, emphasizing their potential for next generation quantum metrology, wireless communication, and precision field mapping.
Rydberg atoms have been used for measuring radio-frequency (RF) electric (E)-fields due to their strong dipole moments over the frequency range of 500 MHz-1 THz. For this, electromagnetically induced transparency (EIT) within the Autler-Townes (AT) regime is used such that the detected E-field is proportional to AT splitting. However, for weak E-fields AT peak separation becomes unresolvable thus limiting the minimum detectable E-field. Here, we demonstrate using the Rydberg atoms as an RF mixer for weak E-field detection well below the AT regime with frequency discrimination better than 1 Hz resolution. A heterodyne detection scenario with two E-fields incident on a vapor cell filled with cesium atoms is used. One E-field at 19.626000 GHz drives the 34D5/2 → 35P3/2 Rydberg transition and acts as a local oscillator (LO) and a second signal E-field (Sig) of interest is at 19.626090 GHz. In the presence of the LO, the Rydberg atoms naturally down convert the Sig field to a 90 kHz intermediate frequency (IF) signal. This IF signal manifests as an oscillation in the probe laser intensity through the Rydberg vapor and is easily detected with a photodiode and lock-in amplifier. In the configuration used here, E-field strength down to ≈ 46 μV/m ± 2 μV/m were detected with a sensitivity of ≈ 79 μVm−1Hz−1/2. Furthermore, neighboring fields 0.1 Hz away and equal in strength to Sig could be discriminated without any leakage into the lock-in signal. For signals 1 Hz away and as high as +60 dB above Sig, leakage into the lock-in signal could be kept below -3 dB.
Rydberg atom-based radio frequency electromagnetic field sensors are drawing wide-spread interest because of their unique properties, such as small size, dielectric construction, and self-calibration. These photonic sensors use lasers to prepare atoms and read out the atomic response to a radio frequency electromagnetic field based on electromagnetically induced transparency, or related phenomena. Much of the theoretical work has focused on the Autler-Townes splitting induced by the radio frequency wave. The amplitude regime, where the change in transmission observed on resonance is measured to determine electric field strength, has received less attention. In this paper, we deliver analytic expressions that are useful for calculating the absorption coefficient in the amplitude regime. Our main goal is to describe the analytic expressions for the absorption coefficient and demonstrate their validity over a large range of the interesting parameter space. The effect of the thermal motion of the atoms is explicitly addressed. The analytic formulas for the absorption coefficient for different types of Doppler broadening are compared to estimate the sensitivity under conditions where it is limited by the laser shot noise. Residual Doppler shifts are shown to limit sensitivity. The expressions, approximations and descriptions presented in the paper are important for understanding the absorption of Rydberg atom-based sensors in the amplitude regime. This provides insight into the physics of multi-level interference phenomena.
Significant progress has been made in atom-based measurements of length, time, gravity and electromagnetic fields in recently years. Rydberg atom-based microwave electric field measurement, using electromagnetically induced transparency (EIT) in room temperature alkali-metal vapors, has been extensively investigated and aroused the broad interest. This approach may establish a new standard for the measurements of microwave (MW) and radio frequency (RF) electric fields.In this review, we describe the work on a new method of measuring electric fields based on quantum interference by using either cesium or rubidium atoms contained in a dielectric vapor cell. Rydberg atoms with principal quantum number n >>1 have large direct current (DC) polarizabilities and microwave transition dipole moments, thereby making them extremely sensitive to external electric fields. Using the Rydberg three-level EIT to detect the level splitting and shift that is induced by the external field, we can realize a rapid and robust self-calibration method of measuring the electric field in a frequency range from 0.01 GHz to 1000 GHz. For the MW electric field (frequency range > 1 GHz), the MW field causes the Rydberg states to split, known as an Autler-Townes splitting (A-T) effect when the applied microwave can resonate with adjacent Rydberg states. The MW coupled A-T splitting is proportional to the applied electric field strength, from which the field strength is measured. Using the EIT window, a high sensitivity of 3 μV·cm-1·Hz-1/2 and small electric field of 1 μV/cm are expected to be achieved with a modest setup, and the limitations of the sensitivity are also addressed in the review. For the RF field at frequency mj EIT lines, and avoided crossings formed with the fine-structure levels of equal mj and different J's, which is used to calibrate and measure the RF field amplitude. On the other hand, the dependence of the EIT-line strength on the RF field polarization provides a fast and robust polarization measurement of RF fields based on matching experimental data with a theoretical simulation. The measurements of minimum strengths and sensitivity of RF fields based on Rydberg atoms are one order magnitude below the values obtained by traditional antenna methods. The atom-based field measurement paves the way for determining fields through calibration-free, invariable atomic properties and miniaturization. We also propose its various potential applications in the future.