The chiral spin liquid is a canonical state of quantum spins combining topological and symmetry-breaking order, and possible experimental realizations have attracted growing interest. We examine the physics at interfaces between chiral spin liquid domains of opposite chirality. We show that a self-consistent mean-field description of spinons remains possible in the vicinity of a domain wall and use this to formulate a Ginzburg-Landau theory of the domain wall. The bulk of a chiral spin liquid contains gapped spinon excitations and gauge fluctuations, set by a finite spinon mass and a nonzero spinon Chern number. A third class of excitations consists of amplitude fluctuations of the spinon hoppings, which admit a geometric interpretation in terms of effective vielbein fields. These fluctuations are usually neglected because they are irrelevant for a homogeneous chiral spin liquid and are suppressed in standard large-[Formula: see text] treatments. Going beyond the purely topological Chern-Simons limit, we incorporate these fluctuations into an effective field theoretic framework and show that they generate momentum-dependent corrections, including Chern-Simons-like linear terms and higher-order contributions, beyond the universal topological limit. We then analyze nontopological properties, including domain wall tension and edge velocity, and explain how they modify observables relative to the uniform case. These results connect measurable, nonuniversal quantities such as domain wall width, domain wall tension, and edge velocity to microscopic parameters and provide concrete targets for experiments.
The chiral spin liquid is a canonical state of quantum spins combining topological and symmetry-breaking order, and possible experimental realizations have attracted growing interest. We examine the physics at interfaces between chiral spin liquid domains of opposite chirality. We show that a self-consistent mean-field description of spinons remains possible in the vicinity of a domain wall and use this to formulate a Ginzburg-Landau theory of the domain wall. The bulk of a chiral spin liquid contains gapped spinon excitations and gauge fluctuations, set by a finite spinon mass and a nonzero spinon Chern number. A third class of excitations consists of amplitude fluctuations of the spinon hoppings, which admit a geometric interpretation in terms of effective vielbein fields. These fluctuations are usually neglected because they are irrelevant for a homogeneous chiral spin liquid and are suppressed in standard large-[Formula: see text] treatments. Going beyond the purely topological Chern-Simons limit, we incorporate these fluctuations into an effective field theoretic framework and show that they generate momentum-dependent corrections, including Chern-Simons-like linear terms and higher-order contributions, beyond the universal topological limit. We then analyze nontopological properties, including domain wall tension and edge velocity, and explain how they modify observables relative to the uniform case. These results connect measurable, nonuniversal quantities such as domain wall width, domain wall tension, and edge velocity to microscopic parameters and provide concrete targets for experiments.
Topological phases of matter are purely quantum mechanical and have no classical analogue. Most phases in nature can be classified and studied classically through the concept of symmetry breaking and its theoretical description, Landau-Ginzburg field theory. In contrast to the general wisdom of Landau-Ginzburg field theory, the topological phases share the same symmetry as a trivial insulator and still are different phases. Having gapped spectrum in bulk, they support a metallic edge excition robust against symmetry-respecting perturbation or an emergent fractional excitation in bulk. Following after fractional quantum Hall fluids, many topologically orderd phases, such as spin liquids and topological insulators, have been found and studied. Spin liquids are disordered phases of frustrated antiferromagnets and do not freeze and order even at the lowest temperature. They support an electrically neutral spin-1/2 excitation, which does not exist in a microscopic scale, with emergent dynamical gauge field in bulk and do not have an adiabatic path to a trivial paramagnet phase. The topological insulators are time-reversal symmetric band insulators which cannot evolve smoothly into a trivial insulator with the symmetry, and they have been intensely studied theoretically and experimetally for the last decade. Though the topological insulators are inherently non-interacting systems, they have exotic gapless edge and surface states which demonstrate many interesting quantum phenomena such as fractionalization, axionic electromagnetism, and half quantum Hall effect. In this thesis, we study various quantum phenomena of the topological phases, mainly of the topological insulator and its close relatives in which the physics of spin liquids has been merged into. As they are intrinsically quantum many-body states, the quantum field theory is an invaluable tool to explore the venue of the phases and will be used thorougly in this work. First, we present a topological field theoretic description of the topological insulators and translational symmetric Z2 spin liquid. We demostrate that abelian BF theory is an effective field theory for the two and three dimensional topological insulators. We show that the phenomenologies of BF theory are consistent with those of the topological insulators such as gapless edge and surface excitations and response functions to external gauge field. The same form of the BF theory is also applicable to study the certain classes of Z2 spin liquids with the gapless edge states. We closely examine the possible gapless edge theory of the BF theory and the translational symmetric spin liquids, and we show that the effective BF theories capture the bulk properties as well as the gapless edge spectrum of the spin liquid. Also we discuss the zero-temperature phase diagram of a thin film three dimensional topological insulators with two competing mass terms: time-reversal symmetric exciton condensation and time-reversal symmetry breaking Zeeman effect. There are two phases, quantum spin Hall phase and quantum anomalous Hall phase, and both phases support fractional excitations. We derive an effective topological field theory for the fractional excitations and examine the origin of the fractional excitations. Next we consider the relatives of the topological insulators. First we discuss the proximate symmetry broken phases of topological Mott insulator, a U(1) spin liquid with fermionic spinons in the topological insulator state. The topologically non-trivial band structure of the spinon generates the axion term for the gauge field, and we show that the axion term changes the nature of the confined phase of the spin liquid. Contrast to the conventional confined phase which has only a bond order, the confined phase of the spin liquid is in general a coexisting phase of the two different orders : a current order and a bond order. We then consider another relative of the topological insulator: a bosonic symmetry protected topological phase in two dimensional space, with both PSU(N) and time reversal symmetry. We develop an effective field theory for the phase, which is a SU(N) principal chiral model with a theta-term, and reveal the physics of the topological phase in detail.Finally we consider a topological semimetal, namely a Weyl semimetal. We first demonstrate that the Weyl semimetal can be realized in the magnetically doped topological band insulators. We explicitly derive the low energy theory of Weyl points from the general continuum Hamiltonian and tight-binding model of the topological insulators. Then we study superconducting instabilities of doped Weyl semimetals. We consider a minimal model for a Weyl semimetal and study the superconducting instabilities induced by a short-ranged attractive interaction. With the interaction, we find two competing states: a fully gapped finite-momentum pairing state and a nodal even-parity pairing state. We show that, in a mean field approximateion, the finite-momentum pairing state wins energetically against the usual even-parity paired state. We also show that exotic modes are localized at the full and half quantum vortices of the finite-momentum pairing state.
Quantum spin liquids are novel phases of matter whose physical properties cannot be captured within the conventional framework of phase transitions. These quantum states are characterized by excitations, called spinons, carrying a fractional value of the integer spin. A description based on a mean-field approximation leads to effective gauge theory. Due to this gauge freedom symmetry group operations act via projective symmetry group (PSG) representations, which can be used to classify quantum states beyond the conventional method. This introducing discussion is found in Chapters 2-6. A preceding PSG classification on the square lattice, which took spin rotational symmetry breaking terms into account, showed that the resulting mean-field states could exhibit topologically non-trivial spinon bands. In Chapter 7, only those el- ements of this Classification are studied, which lead to short-ranged mean-field models. The mutual effect of spinons and visons is scrutinized by adding static configurations of a background gauge field. Spinons and visons form composite ob- jects, which in the case of topological spinon bands, are described by Majorana zero modes. An exact mapping corroborates the relation to topological supercon- ductors and vortices. The effect of multiple visons is investigated, and a possible experimental signature is exposed. Chapter 8 explains how spinon mean-field theory can be used to derive a phe- nomenological effective model for the compound Ca 10 Cr 7 O 28 . A material that was recently proposed as a quantum spin liquid. This low-energy theory consists of spinon hopping processes. The underlying bilayer kagome structure can be simpli- fied to an effective honeycomb lattice. The dynamical spin structure factor is calcu- lated and compared to neutron scattering data. It is discussed how f -wave pairing of spinons can explain small deviations from a linear temperature dependency observed in heat capacity measurements at the low temperatures. This pairing mechanism breaks the U (1) invariance group of the pure hopping model and renders a coherent picture of Ca 10 Cr 7 O 28 being a Z 2 quantum spin liquid. Chapter 9 carries out a PSG classification for the simple-, body centered-, and face centered cubic lattices. Despite a large number of possible PSG representations, only very few describe short-ranged mean-field states. These mean-field models are constructed up to third neighbor couplings and calculated in a self-consistent manner. It is found that the energy is lower for non-trivial sign patterns induced by non-trivial representations of the symmetry generators. Higher neighbor extensions, including pairing terms, yield lower mean-field ground state energies compared to extensions with only hopping terms. For the fcc lattice, a first neighbor state could be identified, which exhibits symmetry protected zero-energy modes.
Chiral spin liquids realize a topological state whose universal response is a fractional spin Hall conductance νs. The three quantities that determine this response, the integer Chern number of the fractionalized spinons, the level of the emergent Chern--Simons gauge field, and the physically measured spin pump, are related but distinct, and their relation is often stated only schematically. Here we derive it from a single object: the parity-odd determinant of a gapped Dirac cone on a spatial cylinder, resummed exactly to all orders in the compact holonomy. This determinant fixes the map from spinon topology to measurable response, and proves that finite-size corrections to the topological pump are strictly exponential, with no universal 1/L term. We test the resulting predictions on the kagome chiral spin liquid at three independent levels: the exact one-loop field theory, a parton band-structure calculation (C=−1, converging exponentially over cylinders four to twelve sites wide), and an interacting density-matrix renormalization group flux pump on the explicitly chiral J--Jχ Hamiltonian (νs=−0.500±0.011). All three agree with the analytic prediction without adjustable parameters, providing a fully quantitative bridge between microscopic topology and observable fractional response.
Frustrated magnetism provides a rich platform for realizing exotic quantum phases in condensed matter systems. Among these, quantum spin liquids (QSLs) are a particularly intriguing class of states that exhibit no magnetic ordering and preserve all symmetries down to zero temperature. Just as conventional magnets can be thought of as spin crystals,QSLs represent their liquid analogs. This thesis explores two broad types of QSLs in two-dimensional magnets, with a focus on their dynamic properties and the nature of transitions from conventional magnetic states into QSL phases. QSLs are topological phases that host fractionalized excitations known as spinons. In these states, mobile spinons are coupled to an emergent gauge field, forming a highly entangled phase of matter. The first part of this thesis focuses on Dirac spin liquids (DSLs), a class of QSLs where spinons exhibit a gapless Dirac dispersion. To study the dynamicsof these spin liquids beyond leading-order mean-field theory, we develop a novel large-N fermionic limit of gapless spinons. In this limit, all gauge excitations are suppressed, and the leading-order corrections instead arise from order parameter fluctuations, which may condense and drive transitions into symmetry-broken phases from the parent DSL. Incorporating random phase approximation (RPA) corrections to the spin susceptibility, we find that sharp, spin-wave–like modes are recovered in the excitation spectrum. This methodology successfully captures characteristic features of the dynamics near phase transitions and in weakly symmetry-broken phases proximate to a DSL. We apply this approach to microscopic models, including the J1-J2 XXZ model on the triangular lattice and the J1-J3 XXZ model on the honeycomb lattice. These models closely represent a wide range of frustrated materials, such as triangular and honeycomb cobaltates and triangular ytterbium compounds. Our theoretical predictions show excellent agreement with experimentally measured inelastic neutron scattering spectra from these materials. Gapless spinons can also sometimes become gapped through chiral symmetry breaking, leading to the formation of a chiral spin liquid (CSL). The CSL is an archetypal bosonic realization of a fractional quantum Hall (FQH) state at half-filling, and has been proposed as a time-reversal–breaking ground state in a variety of frustrated spin models. The second part of this thesis addresses the intriguing possibility of realizing a CSL through the "melting" of a chiral spin crystal—a conventional magnet with non-coplanar ordering. Such a transition offers a physically appealing analogue to the melting of a Wigner crystal into a fermionic FQH liquid. Focusing on the kagome lattice, where chiral interactions are knownto stabilize a CSL ground state, we study the effects of additional long-range Heisenberg interactions and demonstrate a phase transition into a non-coplanar octahedral magnetic order. To describe the universal class of transition between a CSL and a non-coplanar anti-ferromagnetic order, we then develop a novel Chern-Simons–matter field theory framework, constrained by symmetry principles and symmetry fractionalization patterns. This thesis thus provides new insights into the dynamical signatures and phase transitions of quantum spin liquids, offering a bridge between theoretical models and experimental observations in frustrated magnetic systems.
Inspired by the recent discovery of a new instability towards a chiral phase of the classical Heisenberg model on the kagome lattice, we propose a specific chiral spin liquid that reconciles different, well-established results concerning both the classical and quantum models. This proposal is analyzed in an extended mean-field Schwinger boson framework encompassing time reversal symmetry breaking phases, which allows both a classical and a quantum phase description. At low temperatures, we find that quantum fluctuations favor this chiral phase, which is stable against small perturbations of second- and third-neighbor interactions. For spin-1/2, this phase may be, beyond the mean field, a chiral gapped spin liquid. Such a phase is consistent with the density matrix renormalization group results of Yan et al. [Science 332, 1173 (2011)]. Mysterious features of the low-lying excitations of exact diagonalization spectra also find an explanation in this framework. Moreover, thermal fluctuations compete with quantum ones and induce a transition from this flux phase to a planar zero flux phase at a nonzero value of the renormalized temperature (T/S2), reconciling these results with those obtained for the classical system.
The parton approach for quantum spin liquids gives a transparent description of low-energy elementary excitations, e.g., spinons and emergent gauge-field fluctuations. The latter ones are directly coupled to the hopping/pairing of spinons. By using the fermionic representation of the U(1) Dirac state on the kagome lattice and variational Monte Carlo techniques to include the Gutzwiller projection, we analyze the effect of modifying the gauge fields in the spinon kinematics. In particular, we construct low-energy monopole excitations, which are shown to be gapless in the thermodynamic limit. States with a finite number of monopoles or with a finite density of them are also considered, with different patterns of the gauge fluxes. We show that these chiral states are not stabilized in the Heisenberg model with nearest-neighbor superexchange couplings, and the Dirac state corresponds to the lowest-energy ansatz within this family of variational wave functions. Our results support the idea that spinons with a gapless conical spectrum coexist with gapless monopole excitations, even for the spin-1/2 case.