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arXiv:2307.01149 · Physical review. B./Physical review. B

Piercing the Dirac spin liquid: From a single monopole to chiral states

Sasank Budaraju, Yasir Iqbal, Federico Becca, Didier Poilblanc

Published Nov 21, 2023• 7 citations
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Abstract

The parton approach for quantum spin liquids gives a transparent description of low-energy elementary excitations, e.g., spinons and emergent gauge-field fluctuations. The latter ones are directly coupled to the hopping/pairing of spinons. By using the fermionic representation of the $U(1)$ Dirac state on the kagome lattice and variational Monte Carlo techniques to include the Gutzwiller projection, we analyze the effect of modifying the gauge fields in the spinon kinematics. In particular, we construct low-energy monopole excitations, which are shown to be gapless in the thermodynamic limit. States with a finite number of monopoles or with a finite density of them are also considered, with different patterns of the gauge fluxes. We show that these chiral states are not stabilized in the Heisenberg model with nearest-neighbor superexchange couplings, and the Dirac state corresponds to the lowest-energy ansatz within this family of variational wave functions. Our results support the idea that spinons with a gapless conical spectrum coexist with gapless monopole excitations, even for the spin-1/2 case.

DOI
10.1103/physrevb.108.l201116

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The parton approach for quantum spin liquids gives a transparent description of low-energy elementary excitations, e.g., spinons and emergent gauge-field fluctuations. The latter ones are directly coupled to the hopping/pairing of spinons. By using the fermionic representation of the U(1)U(1)U(1) Dirac state on the kagome lattice and variational Monte Carlo techniques to include the Gutzwiller projection, we analyze the effect of modifying the gauge fields in the spinon kinematics. In particular, we construct low-energy monopole excitations, which are shown to be gapless in the thermodynamic limit. States with a finite number of monopoles or with a finite density of them are also considered, with different patterns of the gauge fluxes. We show that these chiral states are not stabilized in the Heisenberg model with nearest-neighbor superexchange couplings, and the Dirac state corresponds to the lowest-energy ansatz within this family of variational wave functions. Our results support the idea that spinons with a gapless conical spectrum coexist with gapless monopole excitations, even for the spin-1/2 case.
The U(1)U(1)U(1) Dirac spin liquid might realize an exotic phase of matter whose low-energy properties are described by quantum electrodynamics in 2+12+12+1 dimensions, where gapless modes exist but spinons and gauge fields are strongly coupled. Its existence was proposed in frustrated Heisenberg models in the presence of frustrating superexchange interactions by the (Abrikosov) fermionic representation of the spin operators [Wen, Phys. Rev. B 65, 165113 (2002)], supplemented by the Gutzwiller projection. Here, we construct charge-QQQ monopole excitations in the Heisenberg model on the triangular lattice with nearest-neighbor (J1{J}_{1}J1​) and next-nearest-neighbor (J2{J}_{2}J2​) couplings. In the highly frustrated regime, singlet and triplet monopoles with Q=1Q=1Q=1 become gapless in the thermodynamic limit; in addition, the energies for generic QQQ agree with field-theoretical predictions, obtained for a large number of gapless fermion modes. Finally, we consider localized gauge excitations, in which magnetic $\ensuremath{\pi}$ fluxes are concentrated in the triangular plaquettes (in analogy with Z2{\mathbb{Z}}_{2}Z2​ visons), showing that these kinds of states do not play a relevant role at low energies. All our findings lend support to a stable U(1)U(1)U(1) Dirac spin liquid in the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ Heisenberg model on the triangular lattice.
We investigate the impact of spin-phonon coupling on the S=1/2S=1/2S=1/2 Heisenberg model on the kagome lattice. For the pure spin model, there is increasing evidence that the low-energy properties can be correctly described by a Dirac spin liquid, in which spinons with a conical dispersion are coupled to emergent gauge fields. Within this scenario, the ground-state wave function is well approximated by a Gutzwiller-projected fermionic state [Ran, Hermele, Lee, and Wen, Phys. Rev. Lett. 98, 117205 (2007)]. However, the existence of U(1)U(1)U(1) gauge fields may naturally lead to instabilities when small perturbations are included. Phonons are ubiquitous in real materials and may play a relevant role in the determination of the actual physical properties of the kagome antiferromagnet. Therefore, we perform a step forward in this direction, including phonon degrees of freedom (at the quantum level) and applying a variational approach based upon Gutzwiller-projected fermionic Ans\"atze. Our results suggest that the Dirac spin liquid is stable for small spin-phonon couplings, while valence-bond solids are obtained at large couplings. Even though different distortions can be induced by the spin-phonon interaction, the general aspect is that the energy is lowered by maximizing the density of perfect hexagons in the dimerization pattern.
We investigate the extended Heisenberg model on the kagome lattice by using Gutzwiller projected fermionic states and the variational Monte Carlo technique. In particular, when both second- and third-neighbor superexchanges are considered, we find that a gapped spin liquid described by nontrivial magnetic fluxes and long-range chiral-chiral correlations is energetically favored compared to the gapless U(1) Dirac state. Furthermore, the topological Chern number, obtained by integrating the Berry curvature, and the degeneracy of the ground state, by constructing linearly independent states, lead us to identify this flux state as the chiral spin liquid with a C=1/2C=1/2C=1/2 fractionalized Chern number.
We perform a Gutzwiller projected-wave-function study for the spin-1/2 Heisenberg model on the Kagomé lattice to compare energies of several spin-liquid states. The result indicates that a U(1)-Dirac spin-liquid state has the lowest energy. Furthermore, even without variational parameters, the energy turns out to be very close to that found by exact diagonalization. We show that such a U(1)-Dirac state represents a quantum phase whose low-energy physics is governed by four flavors of two-component Dirac fermions coupled to a U(1) gauge field. These results are discussed in the context of recent experiments on ZnCu(3)(OH)(6)Cl(2).
A complicating factor in the realization and observation of quantum spin liquids in materials is the ubiquitous presence of other degrees of freedom, in particular lattice distortion modes (phonons). These provide additional routes for relieving magnetic frustration, thereby possibly destabilizing spin-liquid ground states. In this work, we focus on triangular-lattice Heisenberg antiferromagnets, where recent numerical evidence suggests the presence of an extended U(1) Dirac spin liquid phase which is described by compact quantum electrodynamics in 2+1 dimensions (QED3_33​), featuring gapless spinons and monopoles as gauge excitations, and believed to flow to a strongly-coupled fixed point with conformal symmetry. Using complementary perturbation theory and scaling arguments, we show that a symmetry-allowed coupling between (classical) finite-wavevector lattice distortions and monopole operators of the U(1) Dirac spin liquid generally induces a spin-Peierls instability towards a (confining) 12-site valence-bond solid state. We support our theoretical analysis with state-of-the-art density matrix renormalization group simulations. Away from the limit of static distortions, we demonstrate that the phonon energy gap establishes a parameter regime where the spin liquid is expected to be stable, and show that the monopole-lattice coupling leads to softening of the phonon in analogy to the Kohn anomaly. We discuss the applicability of our results to similar systems, in particular the Dirac spin liquid on the Kagome lattice.
Motivated by recent density-matrix renormalization group (DMRG) calculations [Yan, Huse, and White, Science 332, 1173 (2011)], which claimed that the ground state of the nearest-neighbor spin-1/21/21/2 Heisenberg antiferromagnet on the kagome lattice geometry is a fully gapped spin liquid with numerical signatures of Z2{\mathbb{Z}}_{2}Z2​ gauge structure, and a further theoretical work [Lu, Ran, and Lee, Phys. Rev. B 83, 224413 (2011)], which gave a classification of all Schwinger-fermion mean-field fully symmetric Z2{\mathbb{Z}}_{2}Z2​ spin liquids on the kagome lattice, we have thoroughly studied Gutzwiller-projected fermionic wave functions by using quantum variational Monte Carlo techniques, hence implementing exactly the constraint of one fermion per site. In particular, we investigated the energetics of all Z2{\mathbb{Z}}_{2}Z2​ candidates (gapped and gapless) that lie in the neighborhood of the energetically competitive U(1) gapless spin liquids. By using a state-of-the-art optimization method, we were able to conclusively show that the U(1) Dirac state is remarkably stable with respect to all Z2{\mathbb{Z}}_{2}Z2​ spin liquids in its neighborhood, and in particular for opening a gap toward the so-called ${\mathbb{Z}}_{2}[0,\ensuremath{\pi}]\ensuremath{\beta}$ state, which was conjectured to describe the ground state obtained by the DMRG method. Finally, we also considered the addition of a small second nearest-neighbor exchange coupling of both antiferromagnetic and ferromagnetic type, and obtained similar results, namely, a U(1) Dirac spin-liquid ground state.