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arXiv:2208.11505 · npj Quantum Information

Probing resonating valence bonds on a programmable germanium quantum simulator

Chien-An Wang, Corentin Déprez, Hanifa Tidjani, William I. L. Lawrie, Nico W. Hendrickx, Amir Sammak, Giordano Scappucci, Menno Veldhorst

Published Jun 17, 2023• 33 citations
arXivHTMLPDF

Abstract

Abstract Simulations using highly tunable quantum systems may enable investigations of condensed matter systems beyond the capabilities of classical computers. Quantum dots and donors in semiconductor technology define a natural approach to implement quantum simulation. Several material platforms have been used to study interacting charge states, while gallium arsenide has also been used to investigate spin evolution. However, decoherence remains a key challenge in simulating coherent quantum dynamics. Here, we introduce quantum simulation using hole spins in germanium quantum dots. We demonstrate extensive and coherent control enabling the tuning of multi-spin states in isolated, paired, and fully coupled quantum dots. We then focus on the simulation of resonating valence bonds and measure the evolution between singlet product states which remains coherent over many periods. Finally, we realize four-spin states with s-wave and d-wave symmetry. These results provide means to perform non-trivial and coherent simulations of correlated electron systems.

DOI
10.1038/s41534-023-00727-3

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Abstract Simulations using highly tunable quantum systems may enable investigations of condensed matter systems beyond the capabilities of classical computers. Quantum dots and donors in semiconductor technology define a natural approach to implement quantum simulation. Several material platforms have been used to study interacting charge states, while gallium arsenide has also been used to investigate spin evolution. However, decoherence remains a key challenge in simulating coherent quantum dynamics. Here, we introduce quantum simulation using hole spins in germanium quantum dots. We demonstrate extensive and coherent control enabling the tuning of multi-spin states in isolated, paired, and fully coupled quantum dots. We then focus on the simulation of resonating valence bonds and measure the evolution between singlet product states which remains coherent over many periods. Finally, we realize four-spin states with s-wave and d-wave symmetry. These results provide means to perform non-trivial and coherent simulations of correlated electron systems.
Quantum-mechanical correlations of interacting fermions result in the emergence of exotic phases.Magnetic phases naturally arise in the Mott-insulator regime of the Fermi-Hubbard model, where charges are localized and the spin degree of freedom remains.In this regime, the occurrence of phenomena such as resonating valence bonds, frustrated magnetism, and spin liquids is predicted.Quantum systems with engineered Hamiltonians can be used as simulators of such spin physics to provide insights beyond the capabilities of analytical methods and classical computers.To be useful, methods for the preparation of intricate many-body spin states and access to relevant observables are required.Here, we show the quantum simulation of magnetism in the Mott-insulator regime with a linear quantum-dot array.We characterize the energy spectrum for a Heisenberg spin chain, from which we can identify when the conditions for homogeneous exchange couplings are met.Next, we study the multispin coherence with global exchange oscillations in both the singlet and triplet subspace of the Heisenberg Hamiltonian.Last, we adiabatically prepare the low-energy global singlet of the homogeneous spin chain and probe it with two-spin singlettriplet measurements on each nearest-neighbor pair and the correlations therein.The methods and control presented here open new opportunities for the simulation of quantum magnetism benefiting from the flexibility in tuning and layout of gate-defined quantum-dot arrays.
Quantum dots can confine single electrons or holes to define spin qubits that can be operated with high fidelity. Experimental work has progressed from linear to two-dimensional arrays of quantum dots, enabling qubit interactions that are essential for quantum simulation and computation. Here, we explore architectures beyond planar geometries by constructing quantum dot arrays in three dimensions. We realize an eight-quantum dot system in a silicon-germanium heterostructure comprising two stacked germanium quantum wells, where quantum dots are positioned at the vertices of a cuboid. Using electrostatic gate control, we load a single hole into any of the eight quantum dots. To demonstrate the potential of multilayer quantum dot systems, we show coherent spin control and hopping-induced spin rotations by shuttling between the quantum wells. The ability to extend quantum dot arrays in three dimensions provides opportunities for novel quantum hardware and high-connectivity quantum circuits.
Understanding collective phases of strongly correlated quantum magnets relies on theoretically tractable model systems with precise microscopic control. Antiferromagnetic spin ladders provide such a setting, hosting field-tunable gapped and gapless phases at half filling and unconventional pairing tendencies upon doping. Here, we realize a programmable Heisenberg spin ladder in a half-filled germanium quantum dot array featuring site-resolved, continuously tunable exchange interactions. Under a fixed magnetic field, we vary the rung and leg coupling to map the rung-singlet, canted antiferromagnetic, and fully polarized phases. Hamiltonian-learning protocols combining equilibrium and dynamical measurements quantitatively characterize the ladder, incorporating spin-orbit interactions to reproduce the observed crossover behavior. Measurements of higher-order spin correlators -- including four-point correlations inaccessible to conventional bulk probes -- reveal signatures of the underlying phase structure despite the finite size. Our results establish germanium quantum dot arrays as a controllable platform for quantum magnetism, opening routes to investigate unconventional superconductivity in doped ladders.
Quantum simulators are capable of calculating properties of quantum systems unfeasible for classical computers. Here we report the analog quantum simulation of arbitrary Heisenberg-type interactions among four spin-1/2 particles. This spin-1/2 tetramer is the two-dimensional archetype system whose ground state belongs to the class of valence-bond states. Depending on the interaction strength, frustration within the system emerges such that the ground state evolves from a localized to a resonating valence-bond state. This spin-1/2 tetramer is created using the polarization states of four photons. We utilize the particular advantages of the precise single-particle addressability and a tunable measurement-induced interaction to obtain fundamental insights into entanglement dynamics among individual particles. We also directly extract ground-state energies and pair-wise quantum correlations, which enable our quantum simulator to investigate the frustration of entanglement. Remarkably, the pair-wise correlations are restricted by quantum monogamy.
Quasi-particle dynamics in interacting systems in the presence of disorder challenges the notion of internal thermalization, but proves difficult to investigate theoretically for large particle numbers. Engineered quantum systems may offer a viable alternative, as witnessed in experimental demonstrations in a variety of physical platforms, each with its own capabilities and limitations. Semiconductor gate-defined quantum dot arrays are of particular interest since they offer both a direct mapping of their Hamiltonian to Fermi-Hubbard and Heisenberg models and the in-situ tunability of (magnetic) interactions and onsite potentials. In this work, we use an array of germanium quantum dots to simulate the dynamics of both single-spin excitations (magnons) and two-spin excitations (triplons). We develop a methodology that combines digital spin qubit operations for state preparation and readout with analog evolution under the full system Hamiltonian. Using these techniques, we can reconstruct quantum walk plots for both magnons and triplons, and for various configurations of Heisenberg exchange couplings. We furthermore explore the effect of single-site disorder and its impact on the propagation of spin excitations. The obtained results can provide a basis for simulating disorder-based solid-state phenomena such as many-body localization.
The coherent control of interacting spins in semiconductor quantum dots is of strong interest for quantum information processing and for studying quantum magnetism from the bottom up. Here we present a 2 × 4 germanium quantum dot array with full and controllable interactions between nearest-neighbour spins. As a demonstration of the level of control, we define four singlet-triplet qubits in this system and show two-axis single-qubit control of each qubit and SWAP-style two-qubit gates between all neighbouring qubit pairs, yielding average single-qubit gate fidelities of 99.49(8)-99.84(1)% and Bell state fidelities of 73(1)-90(1)%. Combining these operations, we experimentally implement a circuit designed to generate and distribute entanglement across the array. A remote Bell state with a fidelity of 75(2)% and concurrence of 22(4)% is achieved. These results highlight the potential of singlet-triplet qubits as a competing platform for quantum computing and indicate that scaling up the control of quantum dot spins in extended bilinear arrays can be feasible.