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arXiv:2208.10093 · Physical review. B./Physical review. B

Unified intermediate coupling description of pseudogap and strange metal phases of cuprates

Hsien-Chung Kao, Dingping Li, B. Rosenstein

Published Feb 24, 2023• 9 citations
arXivHTMLPDF

Abstract

A one band Hubbard model with intermediate coupling is shown to describe the two most important unusual features of a normal state: linear resistivity strange metal and the pseudogap. Both the spectroscopic and transport properties of the cuprates are considered on the same footing by employing a relatively simple post-Gaussian approximation valid for the intermediate couplings $U/t=1.5--4$ in relevant temperatures $T>100\phantom{\rule{3.33333pt}{0ex}}\mathrm{K}.$ In the doping range $\phantom{\rule{4pt}{0ex}}p=0.1--0.3$, the value of $U$ is smaller than that in the parent material. For a smaller doping, especially in the Mott insulator phase, the coupling is large compared to the effective tight binding scale and a different method is required. This scenario provides an alternative to the paradigm that the coupling should be strong, say $U/t>6$, in order to describe the strange metal. We argue that, to obtain phenomenologically acceptable underdoped normal state characteristics like ${T}^{*}$, pseudogap values, and spectral weight distribution, a large value of $U$ is detrimental. Surprisingly the resistivity in the above temperature range is linear, $\ensuremath{\rho}={\ensuremath{\rho}}_{0}+\ensuremath{\alpha}\frac{{m}^{*}}{{e}^{2}n\ensuremath{\hbar}}T$, with the ``Planckian'' coefficient $\ensuremath{\alpha}$ of order 1.

DOI
10.1103/physrevb.107.054508

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A one band Hubbard model with intermediate coupling is shown to describe the two most important unusual features of a normal state: linear resistivity strange metal and the pseudogap. Both the spectroscopic and transport properties of the cuprates are considered on the same footing by employing a relatively simple post-Gaussian approximation valid for the intermediate couplings U/t=1.5−−4U/t=1.5--4U/t=1.5−−4 in relevant temperatures T>100K.T>100\phantom{\rule{3.33333pt}{0ex}}\mathrm{K}.T>100K. In the doping range p=0.1−−0.3\phantom{\rule{4pt}{0ex}}p=0.1--0.3p=0.1−−0.3, the value of UUU is smaller than that in the parent material. For a smaller doping, especially in the Mott insulator phase, the coupling is large compared to the effective tight binding scale and a different method is required. This scenario provides an alternative to the paradigm that the coupling should be strong, say U/t>6U/t>6U/t>6, in order to describe the strange metal. We argue that, to obtain phenomenologically acceptable underdoped normal state characteristics like T∗{T}^{*}T∗, pseudogap values, and spectral weight distribution, a large value of UUU is detrimental. Surprisingly the resistivity in the above temperature range is linear, \ensuremathρ=\ensuremathρ0+\ensuremathαm∗e2n\ensuremathℏT\ensuremath{\rho}={\ensuremath{\rho}}_{0}+\ensuremath{\alpha}\frac{{m}^{*}}{{e}^{2}n\ensuremath{\hbar}}T\ensuremathρ=\ensuremathρ0​+\ensuremathαe2n\ensuremathℏm∗​T, with the ``Planckian'' coefficient \ensuremathα\ensuremath{\alpha}\ensuremathα of order 1.
Central to the normal state of cuprate high-temperature superconductors is the collapse of the pseudo-gap, briefly reviewed here, at a critical point and the subsequent onset of the strange metal characterized by a resistivity that scales linearly with temperature. A possible clue to the resolution of this problem is the inter-relation between two facts: (i) a robust theory of T-linear resistivity resulting from quantum criticality requires an additional length scale outside the standard one-parameter scaling scenario and (ii) breaking the Landau correspondence between the Fermi gas and an interacting system with short-range repulsions requires non-fermionic degrees. We show that a low-energy theory of the Hubbard model that correctly incorporates dynamical spectral weight transfer has the extra degrees of freedom needed to describe this physics. The degrees of freedom that mix into the lower band as a result of dynamical spectral weight transfer are shown to either decouple beyond a critical doping, thereby signalling Mottness collapse, or unbind above a critical temperature, yielding strange metal behaviour characterized by T-linear resistivity.
To clarify the origin of the pseudogap and strange metal states as well as their mutual relationship in cuprate superconductors, a comprehensive study on the spectral function, Fermi surface, resistivity and dynamical spin susceptivity of the Hubbard model on the square lattice has been conducted by means of the ladder dual-fermion approximation with an electron self-energy correction. It is found that the appearance of these two states requires that the characteristic hole concentration below which the Mott-Heisenberg and Slater mechanisms of electron localization occurs pMSp_{\rm MS}pMS​ nearly coincides with the hole concentration where the Van Hove singularity (VHS) point is placed at the vicinity of the Fermi level. When this condition is met the VHS point is pinned at which the nesting condition of the antiferromagnetic (AFM) fluctuation is fulfilled almost everywhere on the Fermi surface in wide range of the hole concentration in a metallic state, i.e., the strange metal state. The spin fluctuation of the strange metal state is nearly quantum critical and the dynamical spin susceptivity is well described by overdamped spin wave having the ω/Tω/Tω/T scaling with the relaxation rate at the Planckian limit. Because of these distinctive features of the strange metal state, the kkk dependence of scattering rate of electrons is small and electrons behave as the marginal Fermi liquid, resulting in TTT-linear resistivity. In contrast, the pseudogap state is magnetically in the renormalized classical regime and the pseudogap is formed near the X point where the nesting condition of the short-range AFM order is fulfilled.
We review the intermediate coupling model for treating electronic correlations in the cuprates. Spectral signatures of the intermediate coupling scenario are identified and used to adduce that the cuprates fall in the intermediate rather than the weak or the strong coupling limits. A robust, ‘beyond local-density approximation’ framework for obtaining wide-ranging properties of the cuprates via a GW-approximation based self-consistent self-energy correction for incorporating correlation effects is delineated. In this way, doping- and temperature-dependent spectra, from the undoped insulator to the overdoped metal, in the normal as well as the superconducting state, with features of both weak and strong coupling can be modeled in a material-specific manner with very few parameters. Efficacy of the model is shown by considering available spectroscopic data on electron- and hole-doped cuprates from angle-resolved photoemission, scanning tunneling microscopy/spectroscopy, neutron scattering, inelastic light scattering, optical and other experiments. Generalizations to treat systems with multiple correlated bands such as the heavy-fermions, the ruthenates and the actinides are discussed.
We propose that the nonequilibrium current measured in the aaa-bbb plane of an underdoped cuprate (in either the strange metal or pseudogap regime) in contact with either an overdoped cuprate or a standard Fermi liquid can be used to diagnose how different the pseudogap and strange metals are from a Fermi liquid. Naively, one expects the strange metal to be more different from a Fermi liquid than the pseudogap is. We compute the expected nonequilibrium transport signal with the three Green's functions that are available in the literature: (1) marginal Fermi-liquid theory, (2) the phenomenological ansatz for the pseudogap regime, and (3) the Wilsonian reduction of the Hubbard model which contains both the strange metal and pseudogap. All three give linear III-VVV curves at low bias voltages. Significant deviations from linearity at higher voltages obtain only in the marginal Fermi-liquid approach. The key finding, however, is that III-VVV curves for the strange metal/Fermi-liquid contact exceed that of the pseudogap/Fermi-liquid system. If this is borne out experimentally, this implies that the strange metal is less orthogonal to a Fermi liquid than the pseudogap is. Within the Wilsonian reduction of the Hubbard model, this result is explained in terms of a composite-particle picture. Namely, the pseudogap corresponds to a confinement transition of the charge degrees of freedom present in the strange metal. In the strange metal the composite excitations break up and electron quasiparticles scatter off bosons. The bosons here, however, do not arise from phonons but from the charge degrees of freedom responsible for dynamical spectral weight transfer.
Abstract The pseudogap in high-temperature superconducting cuprates is an exotic state of matter, displaying emerging Fermi arcs and a momentum-selective suppression of spectral weight upon cooling. We show how these phenomena are captured in the three-band Emery model by performing dynamical vertex approximation calculations for its normal state. For the hole-doped parent compound, our results demonstrate the formation of a pseudogap due to short-ranged commensurate antiferromagnetic fluctuations. At larger doping values, progressively, incommensurate correlations and a metallic regime appear. Our results are in qualitative agreement with this doping trend in the normal state of cuprates, and hence, represent a step towards the uniform description of their phase diagrams within a single theoretical framework.
An intricate interplay between superconductivity, pseudogap, and Mott transition, either bandwidth driven or doping driven, occurs in materials. Layered organic conductors and cuprates offer two prime examples. We provide a unified perspective of this interplay in the two-dimensional Hubbard model within cellular dynamical mean-field theory on a 2×2 plaquette and using the continuous-time quantum Monte Carlo method as impurity solver. Both at half filling and at finite doping, the metallic normal state close to the Mott insulator is unstable to d-wave superconductivity. Superconductivity can destroy the first-order transition that separates the pseudogap phase from the overdoped metal, yet that normal state transition leaves its marks on the dynamic properties of the superconducting phase. For example, as a function of doping one finds a rapid change in the particle-hole asymmetry of the superconducting density of states. In the doped Mott insulator, the dynamical mean-field superconducting transition temperature T(c)(d) does not scale with the order parameter when there is a normal-state pseudogap. T(c)(d) corresponds to the local pair formation temperature observed in tunneling experiments and is distinct from the pseudogap temperature.