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arXiv:1006.2396 · Philosophical Transactions of the Royal Society A Mathematical Physical and Engineering Sciences

Mottness collapse and T -linear resistivity in cuprate superconductors

Philip Phillips

Published Mar 21, 2011• 22 citations
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Abstract

Central to the normal state of cuprate high-temperature superconductors is the collapse of the pseudo-gap, briefly reviewed here, at a critical point and the subsequent onset of the strange metal characterized by a resistivity that scales linearly with temperature. A possible clue to the resolution of this problem is the inter-relation between two facts: (i) a robust theory of T-linear resistivity resulting from quantum criticality requires an additional length scale outside the standard one-parameter scaling scenario and (ii) breaking the Landau correspondence between the Fermi gas and an interacting system with short-range repulsions requires non-fermionic degrees. We show that a low-energy theory of the Hubbard model that correctly incorporates dynamical spectral weight transfer has the extra degrees of freedom needed to describe this physics. The degrees of freedom that mix into the lower band as a result of dynamical spectral weight transfer are shown to either decouple beyond a critical doping, thereby signalling Mottness collapse, or unbind above a critical temperature, yielding strange metal behaviour characterized by T-linear resistivity.

DOI
10.1098/rsta.2011.0004

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arXiv:1004.1164•Apr 7, 2010•0 citations
Central to the normal state of cuprate high-temperature superconductors is the collapse of the pseudo-gap, briefly reviewed here, at a critical point and the subsequent onset of the strange metal characterized by a resistivity that scales linearly with temperature. A possible clue to the resolution of this problem is the inter-relation between two facts: (i) a robust theory of T-linear resistivity resulting from quantum criticality requires an additional length scale outside the standard one-parameter scaling scenario and (ii) breaking the Landau correspondence between the Fermi gas and an interacting system with short-range repulsions requires non-fermionic degrees. We show that a low-energy theory of the Hubbard model that correctly incorporates dynamical spectral weight transfer has the extra degrees of freedom needed to describe this physics. The degrees of freedom that mix into the lower band as a result of dynamical spectral weight transfer are shown to either decouple beyond a critical doping, thereby signalling Mottness collapse, or unbind above a critical temperature, yielding strange metal behaviour characterized by T-linear resistivity.
We review several of the normal state properties of the cuprates in an attempt to establish an organizing principle from which pseudogap phenomena, broad spectral features, T−T-T−linear resistivity, and spectral weight transfer emerge. We first show that standard field theories with a single critical length scale cannot capture the T−T-T−linear resistivity as long as the charge carriers are critical. What seems to be missing is an additional length scale, which may or may not be critical. Second, we prove a generalised version of Luttinger's theorem for a Mott insulator. Namely, regardless of the spatial dimension, the Fermi surface of the non-interacting system is converted into a surface of zeros of the single-particle Green function when the Mott insulator posesses particle-hole symmetry. Only in the presence of particle-hole symmetry does the volume of the surface of zeros equal the particle density. The surface of zeros persists at finite doping and is shown to provide a framework from which pseudogaps, broad spectral features, spectral weight transfer on the Mott gap scale can be understood.
A one band Hubbard model with intermediate coupling is shown to describe the two most important unusual features of a normal state: linear resistivity strange metal and the pseudogap. Both the spectroscopic and transport properties of the cuprates are considered on the same footing by employing a relatively simple post-Gaussian approximation valid for the intermediate couplings U/t=1.5−−4U/t=1.5--4U/t=1.5−−4 in relevant temperatures T>100K.T>100\phantom{\rule{3.33333pt}{0ex}}\mathrm{K}.T>100K. In the doping range p=0.1−−0.3\phantom{\rule{4pt}{0ex}}p=0.1--0.3p=0.1−−0.3, the value of UUU is smaller than that in the parent material. For a smaller doping, especially in the Mott insulator phase, the coupling is large compared to the effective tight binding scale and a different method is required. This scenario provides an alternative to the paradigm that the coupling should be strong, say U/t>6U/t>6U/t>6, in order to describe the strange metal. We argue that, to obtain phenomenologically acceptable underdoped normal state characteristics like T∗{T}^{*}T∗, pseudogap values, and spectral weight distribution, a large value of UUU is detrimental. Surprisingly the resistivity in the above temperature range is linear, $\ensuremath{\rho}={\ensuremath{\rho}}_{0}+\ensuremath{\alpha}\frac{{m}^{*}}{{e}^{2}n\ensuremath{\hbar}}T$, with the ``Planckian'' coefficient $\ensuremath{\alpha}$ of order 1.
To clarify the origin of the pseudogap and strange metal states as well as their mutual relationship in cuprate superconductors, a comprehensive study on the spectral function, Fermi surface, resistivity and dynamical spin susceptivity of the Hubbard model on the square lattice has been conducted by means of the ladder dual-fermion approximation with an electron self-energy correction. It is found that the appearance of these two states requires that the characteristic hole concentration below which the Mott-Heisenberg and Slater mechanisms of electron localization occurs pMSp_{\rm MS}pMS​ nearly coincides with the hole concentration where the Van Hove singularity (VHS) point is placed at the vicinity of the Fermi level. When this condition is met the VHS point is pinned at which the nesting condition of the antiferromagnetic (AFM) fluctuation is fulfilled almost everywhere on the Fermi surface in wide range of the hole concentration in a metallic state, i.e., the strange metal state. The spin fluctuation of the strange metal state is nearly quantum critical and the dynamical spin susceptivity is well described by overdamped spin wave having the ω/Tω/Tω/T scaling with the relaxation rate at the Planckian limit. Because of these distinctive features of the strange metal state, the kkk dependence of scattering rate of electrons is small and electrons behave as the marginal Fermi liquid, resulting in TTT-linear resistivity. In contrast, the pseudogap state is magnetically in the renormalized classical regime and the pseudogap is formed near the X point where the nesting condition of the short-range AFM order is fulfilled.
Abstract. The normal state metallic behavior above the superconducting transition temperature (Tsc) remains one of the least understood properties since its discovery in cuprates by Bednorz and Müller [1]. Apart from the pseudogap (T ∗) phenomenon above Tsc, there is this T-linear resistivity that was first recognized by Anderson [2] as strange simply because it does not obey the low-temperature T 2 electron-electron scattering rate predicted from the Fermi liquid theory. Here, we prove that the finite temperature continu-ous quantum phase transition (CTQPT) is responsible for the transition from a strange metal to a Fermi liquid for a given chemical composition. Our proof follows the Green function formalism and the energy-level spacing renormal-ization group method. Interestingly, the CTQPT stated above can be related to the proof derived by Parameswaran, Shankar and Sondhi [3], in which, the one-to-one correspondence between the Fermi gas and Fermi liquid is indeed a special case. The theory is further exploited to give unambiguous explanations as to why and how doping gives rise to spectral weight transfer observed in the soft X-ray absorption spectroscopic measurements for the La-Sr-Cu-O system. PACS: 74.72.-h, 71.10.Hf, 74.25.F-, 74.25.Jb 1.
Metallic quantum states coined strange metal (SM), with robust linear-TTT resistivity, have been widely observed in many quantum materials under strong electron correlations, ranging from high-Tc{T}_{c}Tc​ cuprate superconductors and organic superconductors to twisted multilayer graphene and MoTe2/WSe2{\mathrm{MoTe}}_{2}/{\mathrm{WSe}}_{2}MoTe2​/WSe2​ superlattices. Despite decades of intensive studies, the mystery of SM still defies any sensible theoretical explanation and has been a key puzzle in modern condensed matter physics. Here, we solve a doped Mott insulator model called an Ising-Kondo lattice, which includes static spin fluctuation. With Monte Carlo simulation, the Ising-Kondo lattice unambiguously exhibits SM phenomena accompanied with quantum critical scaling in observables, e.g., resistivity, susceptibility, and specific heat. A closer look at SM reveals the breakdown of Landau's Fermi liquid theory without any symmetry breaking, i.e., the violation of Luttinger theorem. Our paper reveals that the long-overlooked static fluctuations in literature may play an essential role in non-Fermi liquid behaviors in correlated electron systems.
A description of the electronic correlations contained in the Hubbard model on the square-lattice perturbed by very weak three-dimensional uniaxial anisotropy in terms of the residual interactions of charge ccc fermions and spin-neutral composite two-spinon s1s1s1 fermions is used to access further information on the origin of quantum critical behavior in the hole-doped cuprate superconductors. Excellent quantitative agreement with their anisotropic linear-ωωω one-electron scattering rate and normal-state linear-TTT resistivity is achieved. Our results provide strong evidence that the normal-state linear-TTT resistivity is indeed a manifestation of low-temperature scale-invariant physics.