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arXiv:2207.14049 · Optics Express

Variable electro-optic shearing interferometry for ultrafast single-photon-level pulse characterization

Stanisław Kurzyna, Marcin Jastrzębski, Nicolas Fabre, Wojciech Wasilewski, Michał Lipka, Michal P. Parniak

Published Oct 3, 2022• 11 citations
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Abstract

Despite the multitude of available methods, the characterization of ultrafast pulses remains a challenging endeavor, especially at the single-photon level. We introduce a pulse characterization scheme that maps the magnitude of its short-time Fourier transform. Contrary to many well-known solutions it does not require nonlinear effects and is therefore suitable for single-photon-level measurements. Our method is based on introducing a series of controlled time and frequency shifts, where the latter is performed via an electro-optic modulator allowing a fully-electronic experimental control. We characterized the full spectral and temporal width of a classical and single-photon-level pulse and successfully tested the applicability of the reconstruction algorithm of the spectral phase and amplitude. The method can be extended by implementing a phase-sensitive measurement and is naturally well-suited to partially-incoherent light.

DOI
10.1364/oe.471108

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Despite the multitude of available methods, the characterization of ultrafast pulses remains a challenging endeavor, especially at the single-photon level. We introduce a pulse characterization scheme that maps the magnitude of its short-time Fourier transform. Contrary to many well-known solutions it does not require nonlinear effects and is therefore suitable for single-photon-level measurements. Our method is based on introducing a series of controlled time and frequency shifts, where the latter is performed via an electro-optic modulator allowing a fully-electronic experimental control. We characterized the full spectral and temporal width of a classical and single-photon-level pulse and successfully tested the applicability of the reconstruction algorithm of the spectral phase and amplitude. The method can be extended by implementing a phase-sensitive measurement and is naturally well-suited to partially-incoherent light.
The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of light has recently emerged as an essential means for quantum information science. Here we experimentally demonstrate a self-referencing technique to completely determine the pulse-mode structure of single photons by means of spectral shearing interferometry. We detail the calibration and resolution of the measurement and discuss challenges and critical requirements for future advances of this method.
Quantum physics holds promise to revolutionise a number of technologies by enabling performance beyond what is feasible with classical resources, such as secure communications, precision measurement and high-speed simulation and computation. To realise this, quantum information must be encoded into one of the physical degrees of freedom of light. The time-frequency (TF) domain provides a infinite-dimensional space which is naturally compatible with integrated optical platforms. Additionally, future quantum networks will require coherent coupling of quantum systems that do not necessarily exhibit TF mode overlap. The ability to generate, coherently control and measure a variety of TF states of quantum light is therefore a necessary step towards implementing optical quantum technologies. Developing the building blocks for future optical quantum applications calls for an assortment of methods for measuring the properties of TF states of quantum light. Whilst much progress has been made towards this goal recently, deficiencies with existing methods remain. Efficient spectrally-resolved detection away from the telecoms wavelength range and a robust approach to single-photon state characterisation that is sensitive to the spectral phase have so far proven challenging. Additionally, accessing quantum advantages requires measurements that are sensitive to the nonclassical correlations that can exist between separate subsystems. However, until now a flexible approach to determining the full quantum state of systems of multiple time/frequency entangled photons has been lacking. Here we develop a toolbox of techniques for the measurement of TF quantum states of light for few-photon systems, and apply these to the task of precision measurement. Firstly, we propose, construct and demonstrate efficient single-photon spectrometers based on dispersive time-to-frequency mapping, using chirped fibre Bragg gratings to apply the necessary group delay dispersion. We use two such devices operating in coincidence to realise a full phase-sensitive reconstruction of the TF state of a single photon, by spectrally resolving the output of a nonclassical interference process with an external reference. We also demonstrate a complementary, optical reference-free method. This characterisation tool, an implementation of electro-optic spectral shearing interferometry with coincident spectrally-resolved single-photon detection, melds techniques from ultrafast metrology and quantum optics. We proceed to demonstrate the flexibility of this device by reconstructing a wide range of test pulses generated with a pulse shaper. By implementing this technique in conjunction with spectrally-resolved detection of a second photon, we realise complete characterisation of the TF wave function of a spectrally-entangled broadband photon pair. This method is robust to a wide range of inputs and is generalisable to spectrally mixed states and across a wide range of wavelengths, including to spectrally non-degenerate photon pairs. To demonstrate, we generate an entangled photon pair with controllable TF entanglement and perform a full reconstruction. Lastly, we present a new technique for using TF entangled photon pairs to realise quantum-enhanced measurement of a time delay in a quantum channel in the presence of environmental noise. This scheme is based on entanglement-enhanced rejection of background light. A simple experiment demonstrating the feasibility of such a measurement is presented.
Ultrafast single-photon pulses with tailored time-frequency properties are highly attractive for quantum information science, offering high-dimensional encoding and compatibility with integrated optics platforms. However, accurate characterization of such pulses, including spectral coherence, remains challenging because current methods require substantial experimental resources and complex reconstruction algorithms. Here, we introduce frequency-bin interferometry for reconstructing electric fields with low intensity (FIREFLY), a technique that directly provides spectral amplitude, phase, and coherence profiles of single-photon pulses without requiring intensive reconstruction algorithms. Our approach measures the two-point spectral correlation function of the pulse by interfering its different frequency components using a quantum pulse gate (QPG) driven by a reference pump pulse. We demonstrate its compatibility with quantum light by characterizing partially coherent pulses generated by a type-0 parametric down-conversion process. We also overcome this requirement of a known pump pulse by introducing spectral shear into our interferometric scheme using a multi-output QPG (mQPG). This enables simultaneous characterization of a single-photon-level input pulse alongside an unknown pump pulse. Notably, our method achieves theory-experiment similarity above 95\% across all retrieved profiles, which demonstrates the reliability of this scheme for quantum information applications based on time-frequency encodings.
The Fractional Fourier Transform (FRT) corresponds to an arbitrary-angle rotation in the phase space, e.g., the time-frequency (TF) space, and generalizes the fundamentally important Fourier Transform. FRT applications range from classical signal processing (e.g., time-correlated noise optimal filtering) to emerging quantum technologies (e.g., super-resolution TF sensing) which rely on or benefit from coherent low-noise TF operations. Here a versatile low-noise single-photon-compatible implementation of the FRT is presented. Optical TF FRT can be synthesized as a series of a spectral disperser, a time-lens, and another spectral disperser. Relying on the state-of-the-art electro-optic modulators (EOM) for the time-lens, our method avoids added noise inherent to the alternatives based on non-linear optical interactions (such as wave-mixing, cross-phase modulation, or parametric processes). Precise control of the EOM-driving radio-frequency signal enables fast all-electronic control of the FRT angle. In the experiment, we demonstrate FRT angles of up to 1.63 rad for pairs of coherent temporally separated 11.5 ps-wide pulses in the near-infrared (800 nm). We observe a good agreement between the simulated and measured output spectra in the bright-light and single-photon-level regimes, and for a range of pulse separations (20 ps to 26.7 ps). Furthermore, a tradeoff is established between the maximal FRT angle and optical bandwidth, with the current setup accommodating up to 248 GHz of bandwidth. With the ongoing progress in EOM on-chip integration, we envisage excellent scalability and vast applications in all-optical TF processing both in the classical and quantum regimes.
Frequency conversion of nonclassical light enables robust encoding of quantum information based upon spectral multiplexing that is particularly well-suited to integrated-optics platforms. Here we present an intrinsically deterministic linear-optics approach to spectral shearing of quantum light pulses and show it preserves the wave-packet coherence and quantum nature of light. The technique is based upon an electro-optic Doppler shift to implement frequency shear of heralded single-photon wave packets by ±200 GHz, which can be scaled to an arbitrary shift. These results demonstrate a reconfigurable method to controlling the spectral-temporal mode structure of quantum light that could achieve unitary operation.