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arXiv:1605.00640 · Physical Review Letters

Spectral Shearing of Quantum Light Pulses by Electro-Optic Phase Modulation

Laura Jayne Wright, Michał Karpiński, Christoph Söller, Brian J. Smith

Published Jan 9, 2017• 94 citations
arXivHTMLPDF

Abstract

Frequency conversion of nonclassical light enables robust encoding of quantum information based upon spectral multiplexing that is particularly well-suited to integrated-optics platforms. Here we present an intrinsically deterministic linear-optics approach to spectral shearing of quantum light pulses and show it preserves the wave-packet coherence and quantum nature of light. The technique is based upon an electro-optic Doppler shift to implement frequency shear of heralded single-photon wave packets by ±200 GHz, which can be scaled to an arbitrary shift. These results demonstrate a reconfigurable method to controlling the spectral-temporal mode structure of quantum light that could achieve unitary operation.

DOI
10.1103/physrevlett.118.023601

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Frequency conversion of nonclassical light enables robust encoding of quantum information based upon spectral multiplexing that is particularly well-suited to integrated-optics platforms. Here we present an intrinsically deterministic linear-optics approach to spectral shearing of quantum light pulses and show it preserves the wave-packet coherence and quantum nature of light. The technique is based upon an electro-optic Doppler shift to implement frequency shear of heralded single-photon wave packets by ±200 GHz, which can be scaled to an arbitrary shift. These results demonstrate a reconfigurable method to controlling the spectral-temporal mode structure of quantum light that could achieve unitary operation.
Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.
Creating and controlling well-defined single-photon states is important for many quantum enhanced technologies. Information can be encoded in any degree of freedom associated with a single-photon field excitation, for example in the polarization or transverse spatial mode structure. The ability to encode multiple qubits in these states is desirable for high data transmission rates and increased information processing capacity. The spectral-temporal domain offers a large Hilbert space for encoding information, well suited to integrated optical architectures owing to the low cross-talk between channels. Indeed, time-frequency encoding is an integral component of existing information technologies infrastructure. Thus, complete, coherent control of the spectral-temporal mode structure of light is essential to advancing optical quantum technologies. Arbitrary control of single-photon states has been demonstrated in the polarization and spatial-momentum degrees of freedom however, is yet to be established in the spectral-temporal domain. Recently it was shown that spectral-temporal pulse shaping is experimentally feasible using nonlinear optical methods. However, such techniques can introduce noise photons, are challenging to implement deterministically and require specially prepared auxiliary pump pulses. Furthermore, they are typically only possible at relatively low repetition rates to avoid damage of nonlinear optical materials. Here, we demonstrate deterministic pulse shaping of single-photon wave packets by introducing a time-varying phase. Applying linear or quadratic phase to the wave packet introduces a spectral shift or spectral broadening, respectively. Achieving significant spectral manipulation requires temporal-phase modulation on the order of π. The phase must also vary on the same time scale as the optical pulses, approximately 1 ps in duration here. This relatively rapid phase variation is achieved using a fast electro-optic phase modulator. The modulator is driven by a time-varying voltage that is synchronized with a pulse train of single-photon wave packets for accurate temporal phase control. In this thesis, we experimentally demonstrate control of the spectral-temporal state of single-photon wave packets using this method. Heralded single-photon wave packets are generated by spontaneous parametric down conversion pumped by a frequency-doubled Titanium-Sapphire laser oscillator with 80 MHz repetition rate. To achieve significant modulation of single-photon pulses a 10 V peak-to-peak radio-frequency signal of 40 GHz drives the phase modulator, which requires approximately 3.6 V to achieve a π phase shift. The signal is synchronized with the oscillator pulse train using custom designed electronics. Details of these electronics are presented, resulting in a robust phase and amplitude controllable 40 GHz voltage source, phase locked to the single-photon pulse train. To demonstrate the utility of this pulse-shaping method we experimentally show spectral shearing of almost 1 nm for single-photon wave packets with 830 nm central wavelength and 1 nm bandwidth. Measurement of the second-order intensity correlation before and after the wave-packet manipulation remains constant within uncertainty of the measurement, showing that the quantum nature of the single-photon source is not deteriorated by the modulator. Preservation of the wave-packet coherence is verified by two-photon interference between spectrally sheared and non-modulated single-photons.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
Abstract Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of nonclassical light using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (± 641 GHz or ± 5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of light has recently emerged as an essential means for quantum information science. Here we experimentally demonstrate a self-referencing technique to completely determine the pulse-mode structure of single photons by means of spectral shearing interferometry. We detail the calibration and resolution of the measurement and discuss challenges and critical requirements for future advances of this method.