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arXiv:2207.13655 · Journal of Magnetism and Magnetic Materials

Effective and asymptotic criticality of structurally disordered magnets

M. Dudka, Mariana Krasnytska, Juan Jesus Ruiz-Lorenzo, Yurij V. Holovatch

Published Apr 5, 2023• 3 citations
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Abstract

Changes in magnetic critical behaviour of quenched structurally-disordered magnets are usually exemplified in experiments and in MC simulations by diluted systems consisting of magnetic and non-magnetic components. In our study we aim to show that similar effects can be observed not only for diluted magnets with non-magnetic impurities but may be implemented, e.g., by the presence of two (and more) chemically different magnetic components as well. Therefore we consider a model of the structurally-disordered quenched magnet where all lattice sites are occupied by Ising-like spins of different lengths L. In such a random spin length Ising model, the length L of each spin is a random variable governed by the distribution function p(L). We demonstrate that this model belongs to the universality class of the site-diluted Ising model. This proves that both models are described by the same values of asymptotic critical exponents. However, their effective critical behaviour differs. As a case study, we consider a quenched mixture of two different magnets with values of elementary magnetic moments L1=1 and L2=s, and of concentration c and 1−c, correspondingly. We apply field-theoretical renormalization group approach to analyse the renormalization group flow for different initial conditions, triggered by s and c, and to calculate effective critical exponents further away from the fixed points of the renormalization group transformation. We show how the effective exponents are governed by difference in properties of the magnetic components.

DOI
10.1016/j.jmmm.2023.170718

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Changes in magnetic critical behaviour of quenched structurally-disordered magnets are usually exemplified in experiments and in MC simulations by diluted systems consisting of magnetic and non-magnetic components. In our study we aim to show that similar effects can be observed not only for diluted magnets with non-magnetic impurities but may be implemented, e.g., by the presence of two (and more) chemically different magnetic components as well. Therefore we consider a model of the structurally-disordered quenched magnet where all lattice sites are occupied by Ising-like spins of different lengths L. In such a random spin length Ising model, the length L of each spin is a random variable governed by the distribution function p(L). We demonstrate that this model belongs to the universality class of the site-diluted Ising model. This proves that both models are described by the same values of asymptotic critical exponents. However, their effective critical behaviour differs. As a case study, we consider a quenched mixture of two different magnets with values of elementary magnetic moments L1=1 and L2=s, and of concentration c and 1−c, correspondingly. We apply field-theoretical renormalization group approach to analyse the renormalization group flow for different initial conditions, triggered by s and c, and to calculate effective critical exponents further away from the fixed points of the renormalization group transformation. We show how the effective exponents are governed by difference in properties of the magnetic components.
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Some physical systems, although dierent by their microscopic nature, in the vicinity of critical points can have similar thermodynamic and structural properties governed by universal power laws.Such systems are grouped into the so-called universality classes.The latter are determined by such global characteristics as the type of interaction, space dimensionality, symmetry, and the number of components of the order parameter.Therefore, it is interesting to investigate how the mutual inuence of these characteristics can aect the critical features of the system.The goal of our research is to analyze the changes in the critical behavior of a many-particle magnetic system under the inuence of two competing factors: long-range interaction and weak structural disorder.Using the example of an n-vector model in a d-dimensional space, we will investigate ferromagnetic ordering in a structurally disordered magnet with the long-range interaction decaying with the distance x as J(x) ∼ x -d-σ , with the control parameter σ.The analysis is carried out using the eld-theoretical renormalization group methods, which makes it possible to identify the universality classes of the system under consideration, their change with global parameters, and to determine the universal characteristics of critical behavior (critical exponents and marginal dimensions).It will be shown that there exists such a region of parameters (d, n, σ), where the long-range interaction and structural disorder lead to a synergistic eect and the appearance of a new, random long-range universality class.We obtain the renormalization group functions in the three-loop approximation, and calculate the correlation length critical exponent ν(ϵ ′ , n) as a perturbation theory series in ϵ ′ = 2σ -d.Quantitative estimates are obtained using asymptotic series resummation methods.
We analyse the critical properties of a weakly diluted (random) Ising model with the long-range interaction decaying with distance x as ∼ x - d - σ in a d-dimensional space. It is known to belong to a new long-range random universality class for certain values of the decay parameter σ. Exploiting the field-theoretic renormalization group approach within the minimal subtraction scheme, we compute the three-loop renormalization group functions. On their basis, with the help of asymptotic series resummation methods, we estimate the correlation length critical exponent ν characterising the new universality class for d = 3 and for those values of σ for which long-range interactions are relevant for the critical behaviour.
Disorder is an inevitable part of any condensed matter system and therefore its study has always been of great importance. The effect of quenched randomness on a system that exhibits a continuous phase transition in the absence of any impurity has been studied in the past and the results are relatively well understood. However, the effect of quenched randomness on \\emph{first-order} phase transitions is still not well understood. In this dissertation, we study the effect of quenched bond-randomness on the classical and quantum first-order phase transitions.In Chapter 2, we study the effect of the disordered three-color Ashkin-Teller model, whose pure version undergoes a first-order phase transition. We show that the rounding of the first-order transition of the pure model due to the impurities is manifested as a critical point. We conclusively rule out that the model belongs to the universality class of the two-dimensional Ising model. Furthermore, we find that the exponents beta\\betabeta and nu\\nunu vary with disorder and the four-spin coupling strength.In Chapter 3, we extend our study of the disordered three-color Ashkin-Teller model. Utilizing extensive cluster Monte Carlo simulations on large lattice sizes of up to 128times128128 \\times 128128times128 spins, each of which is represented by three colors taking values pm1\\pm 1pm1, we show that the rounding of the first-order phase transition is an emergent criticality.We find that the critical exponents, nu\\nunu and beta\\betabeta, change as the strength of disorder or the four-spin coupling varies, and we show that the correlation length critical exponent violates the lower bound 2/Dlenu2/D \\le \\nu2/Dlenu, where DDD is the dimension of the system.In Chapter 4, we study the \\emph{quantum} three-color Ashkin--Teller model and show that the quantum critical point in (1+1)(1+1)(1+1) dimension is an unusual one, with activated scaling at the critical point and Griffiths-McCoy phase away from it. We find that the behavior is similar to the transverse random field Ising model, even though the pure system has a first-order transition in this case.
We study the correlated-disorder-driven zero-temperature equilibrium phase transition of the random-field Ising magnet (RFIM) using exact numerical ground-state calculations for cubic lattices. We consider correlations of the quenched disorder decaying proportionally to ra{r}^{a}ra, where rrr is the distance between two lattice sites and a<0a<0a<0. To obtain exact ground states, we use a well-established mapping to the graph-theoretical maximum-flow problem, which allows us to study large system sizes of more than $2\ifmmode\times\else\texttimes\fi{}{10}^{6}$ spins. We use finite-size-scaling analyses for values $a={\ensuremath{-}1,\ensuremath{-}2,\ensuremath{-}3,\ensuremath{-}7}$ to calculate the critical point and the critical exponents characterizing the behavior of the specific heat, magnetization, susceptibility, and the correlation length close to the critical point. We find basically the same critical behavior as for the RFIM with $\ensuremath{\delta}$-correlated disorder, except for the finite-size exponent of the susceptibility and for the case $a\ensuremath{\ge}\ensuremath{-}2$, where the results are also compatible with a phase transition at infinitesimal disorder strength. We numerically confirm earlier predictions.