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arXiv:2207.02603 · Optics Letters

Single-photon nonlinearities and blockade from a strongly driven photonic molecule

Davide Nigro, Marco Clementi, Camille‐Sophie Brès, Marco Liscidini, Dario Gerace

Published Sep 22, 2022• 2 citations
arXivHTMLPDF

Abstract

Achieving the regime of single-photon nonlinearities in photonic devices by just exploiting the intrinsic high-order susceptibilities of conventional materials would open the door to practical semiconductor-based quantum photonic technologies. Here we show that this regime can be achieved in a triply resonant integrated photonic device made of two coupled ring resonators, in a material platform displaying an intrinsic third-order nonlinearity. By strongly driving one of the three resonances of the system, a weak coherent probe at one of the others results in a strongly suppressed two-photon probability at the output, evidenced by an antibunched second-order correlation function at zero-time delay under continuous wave driving.

DOI
10.1364/ol.468546

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Achieving the regime of single-photon nonlinearities in photonic devices by just exploiting the intrinsic high-order susceptibilities of conventional materials would open the door to practical semiconductor-based quantum photonic technologies. Here we show that this regime can be achieved in a triply resonant integrated photonic device made of two coupled ring resonators, in a material platform displaying an intrinsic third-order nonlinearity. By strongly driving one of the three resonances of the system, a weak coherent probe at one of the others results in a strongly suppressed two-photon probability at the output, evidenced by an antibunched second-order correlation function at zero-time delay under continuous wave driving.
In a recent work [Liew and Savona, Phys. Rev. Lett. 104, 183601 (2010)] it was numerically shown that a resonantly driven photonic ``molecule'' consisting of two coupled cavities can exhibit strong photon antibunching with a surprisingly weak Kerr nonlinearity. Here, we analytically identify the subtle quantum interference effect that is responsible for the predicted efficient photon blockade effect. We then extend the theory to the experimentally relevant Jaynes-Cummings system consisting of a single quantum emitter in a coupled-cavity structure and predict the strong antibunching even for single-atom cooperativity on the order of or smaller than unity. The potential of this quantum interference effect in the realization of strongly correlated photonic systems with only weak material nonlinearities is assessed by comparing on-site and inter-site correlations in a ring of three coupled photonic molecules.
We propose the use of weakly nonlinear passive materials for prospective applications in integrated quantum photonics. It is shown that strong enhancement of native optical nonlinearities by electromagnetic field confinement in photonic crystal resonators can lead to single-photon generation only exploiting the quantum interference of two coupled modes and the effect of photon blockade under resonant coherent driving. For realistic system parameters in state of the art microcavities, the efficiency of such a single-photon source is theoretically characterized by means of the second-order correlation function at zero-time delay as the main figure of merit, where major sources of loss and decoherence are taken into account within a standard master equation treatment. These results could stimulate the realization of integrated quantum photonic devices based on non-resonant material media, fully integrable with current semiconductor technology and matching the relevant telecom band operational wavelengths, as an alternative to single-photon nonlinear devices based on cavity quantum electrodynamics with artificial atoms or single atomic-like emitters.
Photon statistics in a weakly driven optomechanical photonic crystal cavity, with Kerr-type nonlinearity, is analyzed both analytically and numerically. Single-photon blockade effect is demonstrated via calculations of the zero-time-delay second-order correlation function g(2)(0)g^{(2)}(0)g(2)(0). The analytical results obtained by solving the Schrödinger equation are in complete conformity with the results obtained through numerical solution of the quantum master equation. The experimental feasibility with state-of-the-art device parameters is discussed. It is observed that photon blockade could be generated at the telecommunication wavelength, even at lower values of the nonlinear susceptibility parameters and in the weak single-photon optomechanical coupling regime.The system is found to be robust against pure dephasing-induced decoherences.
Analogous to Coulomb blockade for electrons, photon blockade is a key quantum optical effect in which the presence of one photon prevents the transmission of subsequent ones through a nonlinear medium. Beyond its fundamental interest, photon and multi-photon blockade are actively studied as mechanisms for generating technologically-relevant quantum states of light. Although photon blockade typically requires achieving strong light-matter coupling, increasing the number of atoms fails to enhance antibunching. Here, we analyze the optical transmission properties of a quantum resonator that embeds a two-photon-coupled ensemble of emitters, combining an approximate analytical approach with full quantum numerical simulations. We show that when light and matter are coupled via a two-photon interaction, both single- and multi-photon blockade can benefit from a collective enhancement. We propose different driving schemes in which the second or third-order correlation functions are strongly suppressed with increasing atom number. Differently from established methods, this collective enhancement of non-classical properties occurs with unitary transmission and is ultimately constrained only by decoherence. This demonstrates that collective two-photon couplings are a powerful mechanism for realizing photon blockade even in platforms where individual strong coupling is not achievable.
A deterministic and scalable array of single photon nonlinearities in the solid state holds great potential for both fundamental physics and technological applications, but its realization has proved extremely challenging. Despite significant advances, leading candidates such as quantum dots and group III-V quantum wells have yet to overcome their respective bottlenecks in random positioning and weak nonlinearity. Here we consider a hybrid light-matter platform, marrying an atomically thin two-dimensional material to a photonic crystal cavity, and analyze its second-order coherence function. We identify several mechanisms for photon antibunching under different system parameters, including one characterized by large dissipation and weak nonlinearity. Finally, we show that by patterning the two-dimensional material into different sizes, we can drive our system dynamics from a coherent state into a regime of strong antibunching with second-order coherence function ${g}^{(2)}(0)\ensuremath{\sim}{10}^{\ensuremath{-}3}$, opening a possible route to scalable, on-chip quantum simulations with correlated photons.
Universal photon blockade in a two-mode Jaynes-Cummings model incorporating third-order Kerr nonlinearity is demonstrated with a single two-level atom coupled to a waveguide microcavity. Realization of this universal photon blockade is attributed to the cooperative effects of field-atom coupling and Kerr nonlinearity. More importantly, this antibunching is found to be robust against the atomic spontaneous emission, driving field strength, and defect-induced cavity mode coupling. The strong antibunching effect in this resonance-driven scheme is essentially different from those without Kerr nonlinearity. Moreover, this work expands the platform for achieving universal photon blockade and reveals the cooperative advantages of nonlinearities in enhancing the purity and brightness of single-photon sources, representing a novel strategy toward high-performance single-photon sources in integrated quantum optical devices.