Quantum behavior of the Duffing oscillator at the dissipative phase transition
Qiming Chen, Michael Fischer, Yuki Nojiri, Michael Renger, Edwar Xie, Matti Partanen, Stefan Pogorzalek, Kirill G. Fedorov, Achim Marx, Frank Deppe, Rudolf Groß
The non-deterministic behavior of the Duffing oscillator is classically attributed to the coexistence of two steady states in a double-well potential. However, this interpretation fails in the quantum-mechanical perspective which predicts a single unique steady state. Here, we measure the non-equilibrium dynamics of a superconducting Duffing oscillator and experimentally reconcile the classical and quantum descriptions as indicated by the Liouvillian spectral theory. We demonstrate that the two classically regarded steady states are in fact quantum metastable states. They have a remarkably long lifetime but must eventually relax into the single unique steady state allowed by quantum mechanics. By engineering their lifetime, we observe a first-order dissipative phase transition and reveal the two distinct phases by quantum state tomography. Our results reveal a smooth quantum state evolution behind a sudden dissipative phase transition and form an essential step towards understanding the intriguing phenomena in driven-dissipative systems.
The non-deterministic behavior of the Duffing oscillator is classically attributed to the coexistence of two steady states in a double-well potential. However, this interpretation fails in the quantum-mechanical perspective which predicts a single unique steady state. Here, we measure the non-equilibrium dynamics of a superconducting Duffing oscillator and experimentally reconcile the classical and quantum descriptions as indicated by the Liouvillian spectral theory. We demonstrate that the two classically regarded steady states are in fact quantum metastable states. They have a remarkably long lifetime but must eventually relax into the single unique steady state allowed by quantum mechanics. By engineering their lifetime, we observe a first-order dissipative phase transition and reveal the two distinct phases by quantum state tomography. Our results reveal a smooth quantum state evolution behind a sudden dissipative phase transition and form an essential step towards understanding the intriguing phenomena in driven-dissipative systems.
We define quantum chaos and integrability in open quantum many-body systems as a dynamical property of single stochastic realizations, referred to as quantum trajectories. This definition relies on the predictions of random matrix theory applied to the subset of the Liouvillian eigenspectrum involved in each quantum trajectory. Our approach, which we name (SSQT), enables a natural distinction between transient and steady-state quantum chaos as general phenomena in open setups. We test the generality and reliability of the SSQT criterion on several dissipative systems, further showing that an open system with a chaotic structure can evolve towards either a chaotic or integrable steady state. We apply our theoretical framework to two driven-dissipative bosonic systems. First, we study the driven-dissipative Bose-Hubbard model, a paradigmatic example of a quantum simulator, clarifying the interplay of integrability, transient, and steady-state chaos across its phase diagram. Our analysis shows the existence of an emergent dissipative quantum chaotic phase, whereas the classical and semiclassical limits display an integrable behavior. In this regime, chaos arises from the quantum and classical fluctuations associated with the dissipation mechanisms. Second, we investigate dissipative quantum chaos in the dispersive readout of a transmon qubit: a measurement technique ubiquitous in superconducting-based quantum hardware. Through the SSQT, we distinguish several regimes where the performance of the measurement instrument can be connected to the integrable or chaotic nature of the underlying driven-dissipative bosonic system. Our work offers a general understanding of the integrable and chaotic dynamics of open quantum systems and paves the way for the investigation of dissipative quantum chaos and its consequences on state-of-the-art noisy intermediate-scale quantum devices.
Motivated by recent experimental progress to readout quantum bits implemented in superconducting circuits via the phenomenon of dynamical bifurcation, transitions between steady orbits in a driven anharmonic oscillator, the Duffing oscillator, are analyzed. In the regime of weak dissipation a consistent diffusion equation in the semiclassical limit is derived to capture the intimate relation between finite tunneling and reflection and bath induced quantum fluctuations. From the corresponding steady-state distribution an analytical expression for the switching probability is obtained. It is shown that a reduction of the transition rate due to finite reflection at the phase-space barrier is overcompensated by an increase due to environmental quantum fluctuations that are specific for diffusion processes over dynamical barriers. The scaling behavior of the rate is discussed and it is revealed that close to the bifurcation threshold the escape dynamics enters an overdamped domain such that the quantum-mechanical energy scale associated with friction even exceeds the thermal energy scale.
We apply a recently developed theory for metastability in open quantum systems to a one-dimensional dissipative quantum Ising model. Earlier results suggest this model features either a nonequilibrium phase transition or a smooth but sharp crossover, where the stationary state changes from paramagnetic to ferromagnetic, accompanied by strongly intermittent emission dynamics characteristic of first-order coexistence between dynamical phases. We show that for a range of parameters close to this transition or crossover point the dynamics of the finite system displays pronounced metastability, i.e., the system relaxes first to long-lived metastable states before eventual relaxation to the true stationary state. From the spectral properties of the quantum master operator we characterize the low-dimensional manifold of metastable states, which are shown to be probability mixtures of two, paramagnetic and ferromagnetic, metastable phases. We also show that for long times the dynamics can be approximated by a classical stochastic dynamics between the metastable phases that is directly related to the intermittent dynamics observed in quantum trajectories and thus the dynamical phases.
For suitable parameters, the classical Duffing oscillator has a known bistability in its stationary states, with low- and high-amplitude branches. As expected from the analogy with a particle in a double-well potential, transitions between these states become possible either at finite temperature, or in the quantum regime due to tunneling. In this analogy, besides local stability, one can also discuss global stability by comparing the two potential minima. For the Duffing oscillator, the stationary states emerge dynamically so that a priori, a potential-minimum criterion for them does not exist. However, global stability is still relevant, and definable as the state containing the majority population for long times, low temperature, and close to the classical limit. Further, the crossover point is the parameter value at which global stability abruptly changes from one state to the other. For the double-well model, the crossover point is defined by potential-minimum degeneracy. Given that this analogy is so effective in other respects, it is thus striking that for the Duffing oscillator, the crossover point turns out to be non-unique. Rather, none of the three aforementioned limits commute with each other, and the limiting behaviour depends on the order in which they are taken. More generally, as both $\hbar\To0$ and $T\To0$, the ratio ℏω0/kBT continues to be a key parameter and can have any nonnegative value. This points to an apparent conceptual difference between equilibrium and nonequilibrium tunneling. We present numerical evidence by studying the pertinent quantum master equation in the photon-number basis. Independent verification and some further understanding are obtained using a semi-analytical approach in the coherent-state representation.
Dissipation is commonly regarded as an obstacle to quantum control, as it induces decoherence and irreversibility. Here we demonstrate that dissipation can instead be exploited as a resource to reshape the dynamics of interacting quantum systems. Using an experimentally realizable Bose-Josephson junction containing two bosonic species, we demonstrate that dissipation enables distinct dynamical behaviors: synchronized phase-locked oscillations, transient chaos with long-time coherence recovery, and steady-state chaos. The emergence of each behavior is determined by experimentally tunable parameters. At weak interactions, the two components synchronize despite dissipation, exhibiting long-lived coherent oscillations reminiscent of a boundary time crystal. Stronger interactions induce a dissipative phase transition into a self-trapped regime accompanied by chaotic dynamics. Remarkably, dissipation regulates the lifetime of chaos and enables the recovery of coherence at long times. By introducing a controlled tilt between the wells, transient chaos can be converted into persistent steady-state chaos. We further show that standard spectral diagnostics fail to distinguish between the two chaotic regimes, revealing that spectral statistics primarily reflect short-time instability. These results establish dissipation as a powerful tool for engineering dynamical phases, restoring quantum coherence, and controlling the duration of chaotic behavior and information scrambling.
In open quantum systems, dissipative phase transitions (DPTs) emerge from the interplay between unitary evolution, drive, and dissipation. While second-order DPTs have been predominantly investigated theoretically, first-order DPTs have been observed in single-photon-driven Kerr resonators. We present here an experimental and theoretical analysis of both first and second-order DPTs in a two-photon-driven superconducting Kerr resonator. We characterize the steady state at the critical points, showing squeezing below vacuum and the coexistence of phases with different photon numbers. Through time resolved measurements, we study the dynamics across the critical points and observe hysteresis cycles at the first-order DPT and spontaneous symmetry breaking at the second-order DPT. Extracting the timescales of the critical phenomena reveals slowing down across five orders of magnitude when scaling towards the thermodynamic limit. Our results showcase the engineering of criticality in superconducting circuits, advancing the use of parametric resonators for critically-enhanced quantum information applications.