Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2206.04894 · Physical Review Letters

Coherent Transfer of Transverse Optical Momentum to the Motion of a Single Trapped Ion

Felix Stopp, Maurizio Verde, Milton S. Katz, Martin Drechsler, Christian Tomás Schmiegelow, Ferdinand Schmidt‐Kaler

Published Dec 23, 2022• 29 citations
arXivHTMLPDF

Abstract

Using a structured light beam carrying orbital angular momentum, we demonstrate excitation of the center-of-mass motion of a single atom in the transverse direction to the beam's propagation. This interaction enables quantum control of atomic motion in all axes with a single beam direction, which leads to applications in quantum computing and simulations with ion crystals. Here we demonstrate all the key features required for these applications, namely, coherent dynamics and strong carrier suppression in a configuration with the ion centered in the beam, which allows for single ion addressing and also provides robustness against pointing instabilities. To quantify transverse momentum transfer, we observe coherent dynamics on the sidebands of the S_{1/2} to D_{5/2} transition near 729 nm of a singly charged ^{40}Ca^{+} ion, cooled near the ground state of motion in the 3D harmonic potential of a Paul trap, and placed at the center of a first-order Laguerre-Gaussian beam. Exchange of quanta in the perpendicular direction to the beam's wave vector k is observed with a centered vortex shaped beam, together reduction of the parasitic carrier excitation by a factor of 40. This is in sharp contrast to the vanishing spin-motion coupling at the center of the Gaussian beam. Further, we characterize the coherent interaction by an effective transverse Lamb-Dicke factor η_{⊥}^{exp}=0.0062(5) which is in agreement with our theoretical prediction η_{⊥}^{theo}=0.0057(1).

DOI
10.1103/physrevlett.129.263603

Related papers

Transfer of optical orbital angular momentum to a bound electron

Christian Tomás Schmiegelow, J. Schulz, Henning Kaufmann +3 more

Photons can carry angular momentum, not only due to their spin, but also due to their spatial structure. This extra twist has been used, for example, to drive circular motion of microscopic particles in optical tweezers as well as to create vortices in quantum gases. Here we excite an atomic transition with a vortex laser beam and demonstrate the transfer of optical orbital angular momentum to the valence electron of a single trapped ion. We observe strongly modified selection rules showing that an atom can absorb two quanta of angular momentum from a single photon: one from the spin and another from the spatial structure of the beam. Furthermore, we show that parasitic ac-Stark shifts from off-resonant transitions are suppressed in the dark centre of vortex beams. These results show how light's spatial structure can determine the characteristics of light-matter interaction and pave the way for its application and observation in other systems.

Nature Communications•Oct 3, 2016•392 citations

Excitation of an Atomic Transition with a Vortex Laser Beam

Christian Tomás Schmiegelow, J. Schulz, Henning Kaufmann +3 more

Photons carry one unit of angular momentum associated with their spin~\cite{Beth1936}. Structured vortex beams carry additional orbital angular momentum which can also be transferred to matter~\cite{Allen1992}. This extra twist has been used for example to drive motion of microscopic particles in optical tweezers as well as to create vortices in degenerate quantum gases~\cite{He1995,Andersen2006}. Here we demonstrate the transfer of optical orbital angular momentum from the transverse spatial structure of the beam to the internal (electronic) degrees of freedom of an atom. Probing a quadrupole transition of a single trapped $^{40}$Ca$^+$ ion localized at the center of the vortex, we observe strongly modified selection rules, accounting for both the photon spin and the vorticity of the field. In particular, we show that an atom can absorb two quanta of angular momentum from a single photon even when rotational symmetry is conserved. In contrast to previous findings~\cite{Araoka2005,Loeffler2011a,Mathevet2013}, our experiment allows for conditions where the vorticity of the laser beam determines the optical excitation, contributing to the long-standing discussion on whether the orbital angular momentum of photons can be transferred to atomic internal degrees of freedom~\cite{VanEnk1994,Babiker2002,Jauregui2004, Schmiegelow2012, Mondal2014, Scholz-Marggraf2014} and paves the way for its use to tailor light-matter interactions.

arXiv:1511.07206•Nov 23, 2015•6 citations

Tunable transverse spin–motion coupling for quantum information processing

Adam West, Randall Putnam, Wesley C. Campbell +1 more

Abstract Laser-controlled entanglement between atomic qubits (‘spins’) and collective motion in trapped ion Coulomb crystals requires conditional momentum transfer from the laser. Since the spin-dependent force is derived from a spatial gradient in the spin–light interaction, this force is typically longitudinal—parallel and proportional to the average laser k -vector (or two beams’ k -vector difference), which constrains both the direction and relative magnitude of the accessible spin–motion coupling. Here, we show how momentum can also be transferred perpendicular to a single laser beam due to the gradient in its transverse profile. By controlling the transverse gradient at the position of the ion through beam shaping, the relative strength of the sidebands and carrier can be tuned to optimize the desired interaction and suppress undesired, off-resonant effects that can degrade gate fidelity. We also discuss how this effect may already be playing an unappreciated role in recent experiments.

arXiv:2007.10437•Quantum Science and Technology•Nov 18, 2020•16 citations

Light with orbital angular momentum interacting with trapped ions

Christian Tomás Schmiegelow, Ferdinand Schmidt‐Kaler

We study the interaction of a light beams carrying angular momentum with a single, trapped and well localized ion. We provide a detailed calculation of selection rules and excitation probabilities for quadrupole transitions. The results show the dependencies on the angular momentum and polarization of the laser beam as well as the direction of the quantization magnetic field. In order to observe optimally the specific effects, focusing the angular momentum beam close to the diffraction limit is required. We discuss a protocol for examining experimentally the effects on the S$_{1/2}$ to D$_{5/2}$ transition using a $^{40}$Ca$^+$ ion. Various applications and advantages are expected when using light carrying angular momentum: In quantum information processing, where qubit states of ion crystals are controlled, parasitic light shifts could be avoided as the ion is excited in the dark zone of the beam at zero electric field amplitude. Such interactions also open the door to high dimensional entanglement between light and matter. In spectroscopy one might access transitions which have escaped excitation so far due to vanishing transition dipole moments.

arXiv:1112.3377•Dec 14, 2011•3 citations

Angular momentum transfer in interaction of Laguerre-Gaussian beams with atoms and molecules

Pradip Kumar Mondal, Bimalendu Deb, Sonjoy Majumder

The exchange of orbital angular momentum between a Laguerre-Gaussian beam of light and the center-of-mass motion of an atom or molecule is well known. We show that the orbital angular momentum of light can also be transferred to the internal electronic or rotational motion of an atom or a molecule provided the internal and center-of-mass motions are coupled. However, this transfer does not happen directly to the internal motion, but via center-of-mass motion. If atoms or molecules are cooled down to the recoil limit, then an exchange of angular momentum between the quantized center-of-mass motion and the internal motion is possible during the interaction of cold atoms or molecules with the Laguerre-Gaussian beam. The orientation of the exchanged angular momentum is determined by the sign of the winding number of the Laguerre-Gaussian beam. We present selective results of numerical calculations for the quadrupole transition rates in the interaction of the Laguerre-Gaussian beam with an atomic Bose-Einstein condensate to illustrate the underlying mechanism of light orbital angular momentum transfer. We discuss how the alignment of diatomic molecules will facilitate exploration of the effects of light orbital angular momentum on the electronic motion of molecules.

arXiv:1403.2881•Physical Review A•Jun 26, 2014•92 citations

Orbital-angular-momentum partition in hydrogen photoionization by a monochromatic vortex beam

Zhongchen Xing, Chengyin Wu, Zheng Li +1 more

Understanding how optical orbital angular momentum (OAM) is transferred to matter requires treating recoil and translational motion alongside the internal electronic dynamics. We develop a center-of-mass-resolved theory of one-photon ionization of hydrogen by a monochromatic Laguerre--Gaussian beam and show that the Bessel-vortex photoelectron predicted in fixed-target models is a preparation-dependent limit. For a sharply defined atomic center-of-mass momentum, the recoil records the photon-cone azimuth, and tracing over it generally destroys the coherence required for a pure electron vortex. In the small-transverse-retardation regime, the optical OAM is transferred predominantly to the center-of-mass motion and hence, in the laboratory frame, to the proton. Finite-retardation corrections redistribute angular momentum between center-of-mass and relative motion, while an additional correlation contribution to the electron and proton angular momenta can be tuned through the spatial uncertainty of the atomic center of mass. These results reveal atomic recoil as a key element of OAM transfer in photoionization.

physics.atom-phCross-listedarXiv:2609.16825•Sep 16, 2026
Using a structured light beam carrying orbital angular momentum, we demonstrate excitation of the center-of-mass motion of a single atom in the transverse direction to the beam's propagation. This interaction enables quantum control of atomic motion in all axes with a single beam direction, which leads to applications in quantum computing and simulations with ion crystals. Here we demonstrate all the key features required for these applications, namely, coherent dynamics and strong carrier suppression in a configuration with the ion centered in the beam, which allows for single ion addressing and also provides robustness against pointing instabilities. To quantify transverse momentum transfer, we observe coherent dynamics on the sidebands of the S_{1/2} to D_{5/2} transition near 729 nm of a singly charged ^{40}Ca^{+} ion, cooled near the ground state of motion in the 3D harmonic potential of a Paul trap, and placed at the center of a first-order Laguerre-Gaussian beam. Exchange of quanta in the perpendicular direction to the beam's wave vector k is observed with a centered vortex shaped beam, together reduction of the parasitic carrier excitation by a factor of 40. This is in sharp contrast to the vanishing spin-motion coupling at the center of the Gaussian beam. Further, we characterize the coherent interaction by an effective transverse Lamb-Dicke factor η_{⊥}^{exp}=0.0062(5) which is in agreement with our theoretical prediction η_{⊥}^{theo}=0.0057(1).
Photons can carry angular momentum, not only due to their spin, but also due to their spatial structure. This extra twist has been used, for example, to drive circular motion of microscopic particles in optical tweezers as well as to create vortices in quantum gases. Here we excite an atomic transition with a vortex laser beam and demonstrate the transfer of optical orbital angular momentum to the valence electron of a single trapped ion. We observe strongly modified selection rules showing that an atom can absorb two quanta of angular momentum from a single photon: one from the spin and another from the spatial structure of the beam. Furthermore, we show that parasitic ac-Stark shifts from off-resonant transitions are suppressed in the dark centre of vortex beams. These results show how light's spatial structure can determine the characteristics of light-matter interaction and pave the way for its application and observation in other systems.
Photons carry one unit of angular momentum associated with their spin~\cite{Beth1936}. Structured vortex beams carry additional orbital angular momentum which can also be transferred to matter~\cite{Allen1992}. This extra twist has been used for example to drive motion of microscopic particles in optical tweezers as well as to create vortices in degenerate quantum gases~\cite{He1995,Andersen2006}. Here we demonstrate the transfer of optical orbital angular momentum from the transverse spatial structure of the beam to the internal (electronic) degrees of freedom of an atom. Probing a quadrupole transition of a single trapped 40^{40}40Ca+^++ ion localized at the center of the vortex, we observe strongly modified selection rules, accounting for both the photon spin and the vorticity of the field. In particular, we show that an atom can absorb two quanta of angular momentum from a single photon even when rotational symmetry is conserved. In contrast to previous findings~\cite{Araoka2005,Loeffler2011a,Mathevet2013}, our experiment allows for conditions where the vorticity of the laser beam determines the optical excitation, contributing to the long-standing discussion on whether the orbital angular momentum of photons can be transferred to atomic internal degrees of freedom~\cite{VanEnk1994,Babiker2002,Jauregui2004, Schmiegelow2012, Mondal2014, Scholz-Marggraf2014} and paves the way for its use to tailor light-matter interactions.
Abstract Laser-controlled entanglement between atomic qubits (‘spins’) and collective motion in trapped ion Coulomb crystals requires conditional momentum transfer from the laser. Since the spin-dependent force is derived from a spatial gradient in the spin–light interaction, this force is typically longitudinal—parallel and proportional to the average laser k -vector (or two beams’ k -vector difference), which constrains both the direction and relative magnitude of the accessible spin–motion coupling. Here, we show how momentum can also be transferred perpendicular to a single laser beam due to the gradient in its transverse profile. By controlling the transverse gradient at the position of the ion through beam shaping, the relative strength of the sidebands and carrier can be tuned to optimize the desired interaction and suppress undesired, off-resonant effects that can degrade gate fidelity. We also discuss how this effect may already be playing an unappreciated role in recent experiments.
We study the interaction of a light beams carrying angular momentum with a single, trapped and well localized ion. We provide a detailed calculation of selection rules and excitation probabilities for quadrupole transitions. The results show the dependencies on the angular momentum and polarization of the laser beam as well as the direction of the quantization magnetic field. In order to observe optimally the specific effects, focusing the angular momentum beam close to the diffraction limit is required. We discuss a protocol for examining experimentally the effects on the S1/2_{1/2}1/2​ to D5/2_{5/2}5/2​ transition using a 40^{40}40Ca+^++ ion. Various applications and advantages are expected when using light carrying angular momentum: In quantum information processing, where qubit states of ion crystals are controlled, parasitic light shifts could be avoided as the ion is excited in the dark zone of the beam at zero electric field amplitude. Such interactions also open the door to high dimensional entanglement between light and matter. In spectroscopy one might access transitions which have escaped excitation so far due to vanishing transition dipole moments.
The exchange of orbital angular momentum between a Laguerre-Gaussian beam of light and the center-of-mass motion of an atom or molecule is well known. We show that the orbital angular momentum of light can also be transferred to the internal electronic or rotational motion of an atom or a molecule provided the internal and center-of-mass motions are coupled. However, this transfer does not happen directly to the internal motion, but via center-of-mass motion. If atoms or molecules are cooled down to the recoil limit, then an exchange of angular momentum between the quantized center-of-mass motion and the internal motion is possible during the interaction of cold atoms or molecules with the Laguerre-Gaussian beam. The orientation of the exchanged angular momentum is determined by the sign of the winding number of the Laguerre-Gaussian beam. We present selective results of numerical calculations for the quadrupole transition rates in the interaction of the Laguerre-Gaussian beam with an atomic Bose-Einstein condensate to illustrate the underlying mechanism of light orbital angular momentum transfer. We discuss how the alignment of diatomic molecules will facilitate exploration of the effects of light orbital angular momentum on the electronic motion of molecules.
Understanding how optical orbital angular momentum (OAM) is transferred to matter requires treating recoil and translational motion alongside the internal electronic dynamics. We develop a center-of-mass-resolved theory of one-photon ionization of hydrogen by a monochromatic Laguerre--Gaussian beam and show that the Bessel-vortex photoelectron predicted in fixed-target models is a preparation-dependent limit. For a sharply defined atomic center-of-mass momentum, the recoil records the photon-cone azimuth, and tracing over it generally destroys the coherence required for a pure electron vortex. In the small-transverse-retardation regime, the optical OAM is transferred predominantly to the center-of-mass motion and hence, in the laboratory frame, to the proton. Finite-retardation corrections redistribute angular momentum between center-of-mass and relative motion, while an additional correlation contribution to the electron and proton angular momenta can be tuned through the spatial uncertainty of the atomic center of mass. These results reveal atomic recoil as a key element of OAM transfer in photoionization.