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arXiv:2205.13053 · Nature

An optical atomic clock based on a highly charged ion

S. A. King, Lukas J. Spieß, P. Micke, Alexander Wilzewski, Tobias Leopold, Erik Benkler, R. Lange, Nils Huntemann, A. Surzhykov, Vladimir A. Yerokhin, J. R. Crespo López-Urrutia, Piet O. Schmidt

Published Nov 2, 2022• 130 citations
arXivHTMLPDF
DOI
10.1038/s41586-022-05245-4

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With the development of optical frequency comb and ultra-stable laser techniques, the performance of optical frequency standards has been improved significantly over the past decades. Single charged Yb ions have an alkali-like atomic structure and have ultra-long storage time. And the ytterbium single-ion optical frequency standards have two clock transitions (E2 & E3). In this paper, we will introduce the progress in the development of a highly accurate optical frequency standard based on single ytterbium-171 ion at the National Institute of Metrology (NIM), China.
Optical clocks have garnered widespread attention due to their unparalleled precision in time-frequency standards, geodetic measurements, and fundamental physics research. Among emerging developments, highly charged ion (HCI)-based optical clocks have attracted significant scientific interest owing to their exceptional resilience against electromagnetic perturbations and enhanced sensitivity to variations in the fine-structure constant (ααα). While the recent successful demonstration of an Ar13+^{13+}13+ optical clock has validated the feasibility of HCI-based systems, Ni12+^{12+}12+ -- featuring an ultranarrow clock transition linewidth -- stands out as a superior candidate for achieving HCI optical clocks with 10−1910^{-19}10−19 level uncertainty and stability. In this work, we report the Coulomb crystallization of nickel highly charged ions (Ni-HCIs). Through a precision deceleration and sympathetic cooling protocol in a room-temperature Paul trap, high-energy Ni-HCI bunches were sympathetically cooled from megakelvin to the 100-millikelvin range using laser-cooled Be+^{+}+ ions. This work represents a pivotal step toward the realization of an optical clock based on the Ni12+^{12+}12+ ion.