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arXiv:2205.07176 · Physical review. B./Physical review. B

Interaction-induced spatial correlations in a disordered glass

Zvi Ovadyahu

Published Jun 2, 2022• 3 citations
arXivHTMLPDF

Abstract

Sufficiently strong disorder localizes the wave functions of a degenerate Fermi gas. The Coulomb interaction in such a medium renders the system a glass, exhibiting slow relaxation and a rich variety of memory effects. These establish the electron glass as a versatile system for the study of the interplay between disorder and interaction. Here, the author reports on a reversible charge-ordering process in an amorphous electron glass. This occurs while the disorder is considerably stronger than the interaction, which may suggest the relevance of quantum coherent effects.

DOI
10.1103/physrevb.105.235101

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Sufficiently strong disorder localizes the wave functions of a degenerate Fermi gas. The Coulomb interaction in such a medium renders the system a glass, exhibiting slow relaxation and a rich variety of memory effects. These establish the electron glass as a versatile system for the study of the interplay between disorder and interaction. Here, the author reports on a reversible charge-ordering process in an amorphous electron glass. This occurs while the disorder is considerably stronger than the interaction, which may suggest the relevance of quantum coherent effects.
We consider an electron system under conditions of strong Anderson localization, taking into account interelectron long-range Coulomb repulsion. We have established that with the electron density going to zero the Coulomb interaction brings the arrangement of the Anderson localized electrons closer and closer to an ideal (Wigner) crystal lattice, provided the temperature is sufficiently low and the dimension of the system is > 1. The ordering occurs despite the fact that a random spread of the energy levels of the localized one-electron states, exceeding the mean Coulomb energy per electron, renders it impossible the electrons to be self-localized due to their mutual Coulomb repulsion This differs principally the Coulomb ordered Anderson localized electron system (COALES) from Wigner crystal, Wigner glass, and any other ordered electron or hole system that results from the Coulomb self-localization of electrons/holes. The residual disorder inherent to COALES is found to bring about a multi-valley ground-state degeneration akin to that in spin glass. With the electron density increasing, COALES is revealed to turn into Wigner glass or a glassy state of a Fermi-glass type depending on the width of the random spread of the electron levels.
We study the Coulomb glass emerging from the interplay of strong interactions and disorder in a model of spinless fermions on the Bethe lattice. In the infinite coordination number limit, strong interactions induce a metallic Coulomb glass phase with a pseudogap structure at the Fermi energy. Quantum and thermal fluctuations both melt this glass and induce a disordered quantum liquid phase. We combine self-consistent diagrammatic perturbation theory with continuous time quantum Monte-Carlo simulations to obtain the complete phase diagram of the electron glass and to characterize its dynamical properties in the quantum liquid, as well as in the replica symmetry broken glassy phase. Tunneling spectra display an Efros-Shklovskii pseudogap upon decreasing temperatures, but the density of states remains finite at the Fermi energy due to residual quantum fluctuations. Our results bear relevance to the metallic glass phase observed in Si inversion layers.
A longstanding open problem in condensed matter physics is whether or not a strongly disordered interacting insulator can be mapped to a system of effectively non-interacting localized excitations. We investigate this issue on the insulating side of the 3D metal-insulator transition (MIT) in phosphorus doped silicon using the new technique of terahertz two dimensional coherent spectroscopy. Despite the intrinsically disordered nature of these materials, we observe coherent excitations and strong photon echoes that provide us with a powerful method for the study of their decay processes. We extract the first measurements of energy relaxation (T1T_1T1​) and decoherence (T2T_2T2​) times close to the MIT in this classic system. We observe that (i) both relaxation rates are linear in excitation frequency with a slope close to unity, (ii) the energy relaxation timescale T1T_1T1​ counterintuitively increases with increasing temperature and (iii) the coherence relaxation timescale T2T_2T2​ has little temperature dependence between 5 K and 25 K, but counterintuitively increases as the material is doped towards the MIT. We argue that these features imply that (a) the system behaves as a well isolated electronic system on the timescales of interest, and (b) relaxation is controlled by electron-electron interactions. We discuss the potential relaxation channels that may explain the behavior. Our observations constitute a qualitatively new phenomenology, driven by the interplay of strong disorder and strong electron-electron interactions, which we dub the marginal Fermi glass.
We observe the emergence of a disorder-induced insulating state in a strongly interacting atomic Fermi gas trapped in an optical lattice. This closed quantum system free of a thermal reservoir realizes the disordered Fermi-Hubbard model, which is a minimal model for strongly correlated electronic solids. In measurements of disorder-induced localization obtained via mass transport, we detect interaction-driven delocalization and localization that persists as the temperature of the gas is raised. These behaviors are consistent with many-body localization, which is a novel paradigm for understanding localization in interacting quantum systems at non-zero temperature.
For intermediate Coulomb energy to Fermi energy ratios rsr_srs​, spinless fermions in a two-dimensional random potential form a new quantum phase, different from the Fermi glass (weakly interacting Anderson localized states) and the Wigner crystal (regular array of charges pinned by the disorder). The intermediate phase is characterized by an ordered flow of persistent currents with a typical value decreasing with excitation energy. Extending finite size scaling analysis to the many body ground state, we find that electron-electron interactions can drive the Fermi glass towards an intermediate metallic phase (Coulomb metal).
We study the interplay of disorder localization and strong local interactions within the Anderson-Hubbard model. Taking into account local Mott-Hubbard physics and static screening of the disorder potential, the system is mapped onto an effective single-particle Anderson model, which is studied within the self-consistent theory of electron localization. For fermions, we find rich nonmonotonic behavior of the localization length ξ, particularly in two-dimensional systems, including an interaction-induced exponential enhancement of ξ for small and intermediate disorders and a strong reduction of ξ due to hopping suppression by strong interactions. In three dimensions, we identify for half filling a Mott-Hubbard-assisted Anderson localized phase existing between the metallic and the Mott-Hubbardgapped phases. For small U there is re-entrant behavior from the Anderson localized phase to the metallic phase. For bosons, the unrestricted particle occupation number per lattice site yields a monotonic enhancement of ξ as a function of decreasing interaction, which we assume to persist until the superfluid Bose- Einstein condensate phase is entered. Besides, we study cold atomic gases expanding, by a diffusion process, in a weak random potential. We show that the density-density correlation function of the expanding gas is strongly affected by disorder and we estimate the typical size of a speckle spot, i.e., a region of enhanced or depleted density. Both a Fermi gas and a Bose-Einstein condensate (in a mean-field approach) are considered.