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arXiv:2204.10329 · Physical review. B./Physical review. B

Chiral broken symmetry descendants of the kagome lattice chiral spin liquid

Anjishnu Bose, Arijit Haldar, Erik Schwartz Sørensen, Arun Paramekanti

Published Jan 25, 2023• 9 citations
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Abstract

The breaking of chiral and time-reversal symmetries provides a pathway to exotic quantum phenomena and topological phases. Recent work has extensively explored the resulting emergence of chiral charge orders and chiral spin liquids (CSLs) on the kagome lattice. Such CSLs are closely tied to bosonic fractional quantum Hall states with anyonic quasiparticles; however, their connection to nearby ordered states has remained a mystery. Here, we use spin-wave theory, parton Gutzwiller wave functions, and exact diagonalization to show that two distinct magnetic orders with uniform scalar chirality---the XYZ umbrella state and the octahedral spin crystal--emerge as competing orders in close proximity to the CSL. In this letter, we highlight the intimate link between a topologically ordered liquid and broken symmetry states with nontrivial real-space topology.

DOI
10.1103/physrevb.107.l020411

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The breaking of chiral and time-reversal symmetries provides a pathway to exotic quantum phenomena and topological phases. Recent work has extensively explored the resulting emergence of chiral charge orders and chiral spin liquids (CSLs) on the kagome lattice. Such CSLs are closely tied to bosonic fractional quantum Hall states with anyonic quasiparticles; however, their connection to nearby ordered states has remained a mystery. Here, we use spin-wave theory, parton Gutzwiller wave functions, and exact diagonalization to show that two distinct magnetic orders with uniform scalar chirality---the XYZ umbrella state and the octahedral spin crystal--emerge as competing orders in close proximity to the CSL. In this letter, we highlight the intimate link between a topologically ordered liquid and broken symmetry states with nontrivial real-space topology.
The fractional quantum Hall effect (FQHE) realized in two-dimensional electron systems under a magnetic field is one of the most remarkable discoveries in condensed matter physics. Interestingly, it has been proposed that FQHE can also emerge in time-reversal invariant spin systems, known as the chiral spin liquid (CSL) characterized by the topological order and the emerging of the fractionalized quasiparticles. A CSL can naturally lead to the exotic superconductivity originating from the condense of anyonic quasiparticles. Although CSL was highly sought after for more than twenty years, it had never been found in a spin isotropic Heisenberg model or related materials. By developing a density-matrix renormalization group based method for adiabatically inserting flux, we discover a FQHE in a spin-½ isotropic kagome Heisenberg model. We identify this FQHE state as the long-sought CSL with a uniform chiral order spontaneously breaking time reversal symmetry, which is uniquely characterized by the half-integer quantized topological Chern number protected by a robust excitation gap. The CSL is found to be at the neighbor of the previously identified Z2 spin liquid, which may lead to an exotic quantum phase transition between two gapped topological spin liquids.
Topological phases in frustrated quantum magnetic systems have captivated researchers for decades, with the chiral spin liquid (CSL) standing out as one of the most compelling examples. Featuring long-range entanglement, topological order, and exotic fractional excitations, the CSL has inspired extensive exploration for practical realizations. In this Letter, we demonstrate that CSLs can emerge in a kagome lattice driven by vacuum quantum fluctuations over the noninteracting vacuum within a single-mode gyrotropic cavity. The gyrotropic cavity imprints quantum fluctuations with time-reversal symmetry breaking and stabilizes a robust CSL phase without external laser excitation. Moreover, we identify experimentally accessible observables-such as average photon number and transport properties-that reveal connections between photon dynamics and the emergent chiral order. Our findings establish a novel pathway for creating, controlling, and probing topological and symmetry-breaking quantum phases in strongly correlated systems.
Kalmeyer-Laughlin (KL) chiral spin liquid (CSL) is a type of quantum spin liquid without time-reversal symmetry, and it is considered as the parent state of an exotic type of superconductor--anyon superconductor. Such an exotic state has been sought for more than twenty years; however, it remains unclear whether it can exist in a realistic system where time-reversal symmetry is breaking (T breaking) spontaneously. By using the density matrix renormalization group, we show that KL CSL exists in a frustrated anisotropic kagome Heisenberg model, which has spontaneous T breaking. We find that our model has two topological degenerate ground states, which exhibit nonvanishing scalar chirality order and are protected by finite excitation gap. Furthermore, we identify this state as KL CSL by the characteristic edge conformal field theory from the entanglement spectrum and the quasiparticles braiding statistics extracted from the modular matrix. We also study how this CSL phase evolves as the system approaches the nearest-neighbor kagome Heisenberg model.
We consider the spin rotationally invariant Kalmeyer-Laughlin chiral spin liquid (CSL) in systems with broken time-reversal symmetry and explore symmetry constraints on possible conventional spin crystal states accessible via a direct transition. These constraints provide a framework to identify topological invariants of the magnetically ordered state. We show that the existence of a direct transition from a CSL requires a precise compatibility condition between the topological invariants of the ordered state and the anomaly of the CSL. The lattice symmetries also constrain the functional form of the low-energy theory to describe these transitions. This allows us to construct explicit Chern-Simons-matter field theories for the transition into a class of noncoplanar orders identified as candidates directly accessible from the CSL, including the octahedral spin crystal on the kagom\'e lattice and the tetrahedral order on the triangular and honeycomb lattice. These transitions can either be described using coupled fractionalized CP1{\mathbb{CP}}^{1}CP1 theories or fractionalized matrix principal chiral models. We also discuss extensions to more general magnetic ordering transitions out of the CSL.
Quantum spin liquids (QSLs) are highly entangled states of quantum magnets which lie beyond the Landau paradigm of classifying phases of matter via broken symmetries. A physical route to arriving at QSLs is via frustration-induced quantum melting of ordered states such as valence bond crystals or magnetic orders. Here we show, using extensive exact diagonalization (ED) and density-matrix renormalization group (DMRG) studies of concrete SU(2)SU(2)SU(2) invariant spin models on honeycomb, triangular, and square lattices, that chiral spin liquids (CSLs) emerge as descendants of triple-QQQ spin crystals with tetrahedral magnetic order and a large scalar spin chirality. Such ordered-to-CSL melting transitions may yield lattice realizations of effective Chern-Simons-Higgs field theories. Our work provides a distinct unifying perspective on the emergence of CSLs and suggests that materials with certain noncoplanar magnetic orders might provide a good starting point to search for CSLs.