Two-dimensional (2D) quantum magnetism is a paradigm in strongly correlated many-body physics. The understanding of 2D quantum magnetism can be expedited by employing a controllable quantum simulator that faithfully maps 2D-spin Hamiltonians. The 2D quantum simulators can exhibit exotic phenomena such as frustrated quantum magnetism and topological order and can be used to show quantum computational advantages. Many experimental platforms are being developed, including Rydberg atoms and superconducting annealers. However, with trapped-ion systems, which showed the most advanced controllability and quantum coherence, quantum magnetism was explored in one-dimensional chains. Here, we report simulations of frustrated quantum magnetism with 2D ion crystals. We create a variety of spin-spin interactions for quantum magnets, including those that exhibit frustration by driving different vibrational modes and adiabatically prepare the corresponding ground states. The experimentally measured ground states are consistent with the theoretical predictions and are highly degenerate for geometrically frustrated spin models in two dimensions. Quantum coherence of the ground states is probed by reversing the time evolution of the B-field to the initial value and then measuring the extent to which the remaining state coincides with the initial state. Our results open the door for quantum simulations with 2D ion crystals.
Two-dimensional (2D) quantum magnetism is a paradigm in strongly correlated many-body physics. The understanding of 2D quantum magnetism can be expedited by employing a controllable quantum simulator that faithfully maps 2D-spin Hamiltonians. The 2D quantum simulators can exhibit exotic phenomena such as frustrated quantum magnetism and topological order and can be used to show quantum computational advantages. Many experimental platforms are being developed, including Rydberg atoms and superconducting annealers. However, with trapped-ion systems, which showed the most advanced controllability and quantum coherence, quantum magnetism was explored in one-dimensional chains. Here, we report simulations of frustrated quantum magnetism with 2D ion crystals. We create a variety of spin-spin interactions for quantum magnets, including those that exhibit frustration by driving different vibrational modes and adiabatically prepare the corresponding ground states. The experimentally measured ground states are consistent with the theoretical predictions and are highly degenerate for geometrically frustrated spin models in two dimensions. Quantum coherence of the ground states is probed by reversing the time evolution of the B-field to the initial value and then measuring the extent to which the remaining state coincides with the initial state. Our results open the door for quantum simulations with 2D ion crystals.
We study quantum (T = 0) phases of strongly-correlated matter, and their possible implementation in a quantum simulator. We focus on the non-perturbative regimes of 1D spin-boson models. As a reference physical system we consider trapped-ion chains. We realize complex many-body states, such as a ground state exhibiting magnetic frustration, a lattice gauge theory, and a topological insulator. The exquisite control over these phases offered by a quantum simulator opens up exciting possibilities for exploring the exotic phenomena emerging in these systems, such as enhanced fluctuations and correlations. We address the non-perturbative regimes of the phase diagrams by means of mean-field theories and the numerical algorithm DMRG. We have established the universality class of the continuous transition in the spin-boson chain, the existence of a first order phase transition when the system is endowed with a gauge symmetry, and the possibility of probing topological states of matter in these systems. Our results show that some of the most exotic phases of quantum matter can be readily realized in trapped-ion quantum simulators. This offers the possibility of exploring these physical models beyond their original realm of applicability, which may provide us with new insights on both theoretical and applied fields of physics, ranging from high-energy processes to low-energy cooperative phenomena.
The computational difficulty of solving fully quantum many-body spin problems is a significant obstacle to understanding the behavior of strongly correlated quantum matter. Experimental ion trap quantum simulation is a promising approach for studying these lattice spin models, but has so far been limited to one-dimensional systems. This work argues that such quantum simulation techniques are extendable to a two-dimensional (2D) ion crystal confined in a radio-frequency (rf) trap. Using appropriately chosen parameters, driven ion motion due to the rf fields can be made small and will not limit the types of quantum spin models that can be experimentally encoded. The rf-driven motion is calculated to modestly reduce the stability region of a 2D crystal and must be considered when designing the 2D trap. The system will be scalable to 100+ quantum particles, far beyond the realm of classical intractability, while maintaining the traditional ion trap strengths of individual-ion control, long quantum coherence times, and site-resolved projective spin measurements.
Quantum simulation of interacting many-body spin systems is routinely performed with cold trapped ions, and systems with hundreds of spins have been studied in one and two dimensions. In the most common realizations of these platforms, spin degrees of freedom are encoded in low-lying electronic levels, and interactions among the spins are mediated through crystal vibrations. Here we propose a new approach which enables the quantum simulation of two-dimensional spin systems with interaction strengths that are increased by orders of magnitude. This, together with the unprecedented longevity of trapped ions, opens an avenue for the exploration of phenomena that take place on long timescales, e.g., slow and collective relaxation in frustrated and kinetically constrained systems. Our platform makes use of the strong dipolar interactions among electronic Rydberg states and planar confinement provided by a Penning trap. We investigate how the strong electric and magnetic fields that form this trap affect the properties of the Rydberg states and show that spin-spin interaction strengths on the order of MHz are achievable under experimentally realistic conditions. As a brief illustration of the capabilities of this quantum simulator, we study the entanglement in a frustrated spin system realized by three ions.
This thesis investigates quantum magnetism in two-dimensional synthetic systems, where strong correlations, geometric frustration, and enhanced quantum fluctuations produce unconventional magnetic phases. I focus on two major classes of engineered platforms: moiré materials and quantum simulators, which offer precise control over lattice geometry, interaction strengths, and dynamics, enabling access to regimes beyond conventional condensed-matter approaches. The first project studies moiré magnetism in strained multilayers of CrBr₃, where strain generates a spatial modulation of the interlayer exchange alternating between ferromagnetic and antiferromagnetic. With S=3/2 moments, the system admits a classical bilayer description with competing interactions. I develop a theoretical framework capturing the resulting non-collinear orders and reproducing experimental signatures, demonstrating how moiré engineering stabilizes non-trivial magnetic textures. The second project examines quantum magnetism in a WSe₂/WS₂ heterobilayer at three-quarters filling, where electrons form an effective kagome lattice. From the underlying Hubbard model, I derive a frustrated Heisenberg Hamiltonian with competing exchanges. Using Schwinger-boson mean-field theory, I map a phase diagram of non-collinear orders and spin-liquid phases. For realistic parameters, the ground state is a chiral spin liquid, highlighting transition-metal dichalcogenide moiré materials as platforms for topological and strongly correlated magnetism. The third project investigates quantum phase-transition dynamics with superconducting circuit quantum simulators, focusing on Hamiltonian ramps in the 2D XY model. An analogue-digital protocol drives the system from a gapped staggered state to the gapless XY phase. Analysis of correlations reveals scaling of the correlation length with ramp rate, broadly consistent with Kibble–Zurek predictions, with deviations reflecting finite-size, dimensionality, and experimental constraints. The fourth project develops a Holstein–Primakoff spin-wave description for the same XY ramps. Adapting the quantization axis to the instantaneous magnetization, this solvable quadratic theory provides magnon dispersions, time- and space-dependent correlations, and single-magnon dynamics, including decay and scattering. This framework offers a detailed picture of non-equilibrium quasiparticle behavior in a 2D magnet under time-dependent fields. Together, these projects show how moiré materials and quantum simulators enable controlled studies of frustrated and strongly correlated magnetism in two dimensions. By combining analytical modeling with experimentally relevant conditions, this thesis advances understanding of how frustration, topology, and non-equilibrium dynamics shape quantum magnetic phenomena in low-dimensional systems.
Quantum simulations using AMO systems promise a new way to experimentally study emergent quantum phenomena, but few systems have demonstrated the capability to control ensembles in which quantum effects cannot be directly computed. The 2D array of 100s of 9Be+ ions in a Penning trap, crystallized in a triangular lattice when laser cooled, is a promising platform for intractable quantum simulations using the 9Be+ valence electron spin as a qubit [1]. Spin-dependent forces are employed to modify the strong Coulomb interaction of the ions, mimicking a quantum magnetic interaction. The range of the magnetic interaction can be tuned from infinite to a dipole-dipole like coupling. Combining the application of the spin-dependent force with a transverse magnetic field should lead to the development of quantum correlations between the spins, which can be measured through optical readout of the spin state, both globally and with site-resolved imaging. In this way, trapped atomic ions can be used to probe novel and intractable aspects of quantum magnetism, including the effects of long-range interactions and simulations of quantum non-equilibrium phenomena [2]. In addition to a general overview, I will discuss recent work from a new Penning trap set-up at NIST.
The quest for experimental platforms that allow for the exploration, and even control, of the interplay of low dimensionality and frustration is a fundamental challenge in several fields of quantum many-body physics, such as quantum magnetism. Here, we propose the use of cold crystals of trapped ions to study a variety of frustrated quantum spin ladders. By optimizing the trap geometry, we show how to tailor the low dimensionality of the models by changing the number of legs of the ladders. Combined with a method for selectively hiding ions provided by laser addressing, it becomes possible to synthesize stripes of both triangular and Kagome lattices. Besides, the degree of frustration of the phonon-mediated spin interactions can be controlled by shaping the trap frequencies. We support our theoretical considerations by initial experiments with planar ion crystals, where a high and tunable anisotropy of the radial trap frequencies is demonstrated. We take into account an extensive list of possible error sources under typical experimental conditions, and describe explicit regimes that guarantee the validity of our scheme.