Abstract Nonlinear optics processes lie at the heart of photonics and quantum optics for their indispensable role in light sources and information processing. During the past decades, the three- and four-wave mixing (χ(2) and χ(3)) effects have been extensively studied, especially in the micro-/nano-structures by which the photon-photon interaction strength is greatly enhanced. So far, the high-order nonlinearity beyond the χ(3) has rarely been studied in dielectric materials due to their weak intrinsic nonlinear susceptibility, even in high-quality microcavities. Here, an effective five-wave mixing process (χ(4)) is synthesized by incorporating χ(2) and χ(3) processes in a single microcavity. The coherence of the synthetic χ(4) is verified by generating time-energy entangled visible-telecom photon pairs, which requires only one drive laser at the telecom waveband. The photon-pair generation rate from the synthetic process shows an estimated enhancement factor over 500 times upon intrinsic five-wave mixing. Our work demonstrates a universal approach of nonlinear synthesis via photonic structure engineering at the mesoscopic scale rather than material engineering, and thus opens a new avenue for realizing high-order optical nonlinearities and exploring functional photonic devices.
Abstract Nonlinear optics processes lie at the heart of photonics and quantum optics for their indispensable role in light sources and information processing. During the past decades, the three- and four-wave mixing (χ(2) and χ(3)) effects have been extensively studied, especially in the micro-/nano-structures by which the photon-photon interaction strength is greatly enhanced. So far, the high-order nonlinearity beyond the χ(3) has rarely been studied in dielectric materials due to their weak intrinsic nonlinear susceptibility, even in high-quality microcavities. Here, an effective five-wave mixing process (χ(4)) is synthesized by incorporating χ(2) and χ(3) processes in a single microcavity. The coherence of the synthetic χ(4) is verified by generating time-energy entangled visible-telecom photon pairs, which requires only one drive laser at the telecom waveband. The photon-pair generation rate from the synthetic process shows an estimated enhancement factor over 500 times upon intrinsic five-wave mixing. Our work demonstrates a universal approach of nonlinear synthesis via photonic structure engineering at the mesoscopic scale rather than material engineering, and thus opens a new avenue for realizing high-order optical nonlinearities and exploring functional photonic devices.
Correlated photon-pair sources are key components for quantum computing, networking, synchronization, and sensing applications. Integrated photonics has enabled chip-scale sources using nonlinear processes, producing high-rate time-energy and polarization entanglement at telecom wavelengths with sub-100 microwatt pump power. Many quantum systems operate in the visible or near-infrared ranges, necessitating visible-telecom entangled-pair sources for connecting remote systems via entanglement swapping and teleportation. This study evaluates biphoton pair generation and time-energy entanglement through spontaneous four-wave mixing in various nonlinear integrated photonic materials, including silicon nitride, lithium niobate, aluminum gallium arsenide, indium gallium phosphide, and gallium nitride. We demonstrate how geometric dispersion engineering facilitates phase-matching for each platform and reveals unexpected results, such as robust designs to fabrication variations and a Type-1 cross-polarized phase-matching condition for III-V materials that expands the operational wavelength range.
Correlated photon-pair sources are key components for quantum computing, networking, and sensing applications. Integrated photonics has enabled chip-scale sources using nonlinear processes, producing high-rate entanglement with sub-100 microwatt power at telecom wavelengths. Many quantum systems operate in the visible or near-infrared ranges, necessitating broadband visible-telecom entangled-pair sources for connecting remote systems via entanglement swapping and teleportation. This study evaluates broadband entanglement generation through spontaneous four-wave mixing in various nonlinear integrated photonic materials, including silicon nitride, lithium niobate, aluminum gallium arsenide, indium gallium phosphide, and gallium nitride. We demonstrate how geometric dispersion engineering facilitates phase-matching for each platform and reveals unexpected results, such as robust designs to fabrication variations and a Type-1 cross-polarized phase-matching condition for III-V materials that expands the operational bandwidth. With experimentally attainable parameters, integrated photonic microresonators with optimized designs can achieve pair generation rates greater than ~1 THz/mW2.
Cryogenic integrated nonlinear photonics can provide fundamental building blocks for scalable photonic quantum computing and optical interfacing among different platforms. Here, we investigate the spontaneous four-wave mixing effect in an integrated silicon waveguide with cryogenic operating conditions (4 K) and employ the system to generate the entangled photon-pair source, one of the key elements of photonic quantum information applications. We experimentally prove that even at cryogenic temperatures, the four-wave mixing effect in silicon waveguides is still an effective method to generate quantum photonic sources. The cryogenic photon-pair source is verified over multiple frequency channels within a bandwidth of ∼2THz. Furthermore, the source is used to generate high-quality frequency-multiplexed energy–time entangled states. Our results will advance the development of cryogenic nonlinear photonics and scalable integrated photonics for quantum information processing.
The efficient and controllable generation of entangled photon pairs is a cornerstone for advancing quantum technologies, including quantum computing, communication, and sensing. Traditional methods, primarily relying on spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing (SFWM) in bulk nonlinear crystals or waveguides, often suffer from low efficiency, bulky form factors, and limited control over the spectral and spatial properties of the generated photons. This paper explores a transformative approach leveraging resonant Bound States in the Continuum (BICs) within nanophotonic structures to overcome these limitations. BICs are extraordinary optical resonances characterized by theoretically infinite quality (Q) factors, enabling extreme light localization and immense field enhancement within subwavelength volumes. By integrating nonlinear optical materials into BIC-supporting structures, such as photonic crystal slabs or metasurfaces, the local electric field strength experienced by the nonlinear medium can be dramatically increased, boosting the efficiency of entangled photon generation. Furthermore, the sharp, tailor-able spectral response of BICs offers unprecedented control over the joint spectral amplitude of the photon pairs, promising high degrees of spectral purity and entanglement fidelity. This work outlines the theoretical underpinnings, potential device architectures, and anticipated advantages of BIC-enhanced entangled photon sources, paving the way for compact, high-brightness, and spectrally engineered quantum light sources critical for next-generation quantum technologies.
Integrated quantum photonics leverages the on-chip generation of nonclassical states of light to realize key functionalities of quantum devices. Typically, the generation of such nonclassical states relies on whispering gallery mode resonators, such as integrated optical micro-rings, which enhance the efficiency of the underlying spontaneous nonlinear processes. While these kinds of resonators excel in maximizing either the temporal confinement or the spatial overlap between different resonant modes, they are usually associated with large mode volumes, imposing an intrinsic limitation on the efficiency and footprint of the device. Here, we engineer a source of time-energy entangled photon pairs based on a silicon photonic crystal cavity, implemented in a fully CMOS-compatible platform. In this device, resonantly enhanced spontaneous four-wave mixing converts pump photon pairs into signal/idler photon pairs under the energy-conserving condition in the telecommunication C-band. The design of the resonator is based on an effective bichromatic confinement potential, allowing it to achieve up to nine close-to-equally spaced modes in frequency, while preserving small mode volumes, and the whole chip, including grating couplers and access waveguides, is fabricated in a single run on a silicon-on-insulator platform. Besides demonstrating efficient photon pair generation, we also implement a Franson-type interference experiment, demonstrating entanglement between signal and idler photons with a Bell inequality violation exceeding five standard deviations. The high generation efficiency combined with the small device footprint in a CMOS-compatible integrated structure opens a pathway toward the implementation of compact quantum light sources in all-silicon photonic platforms.
Entangled photons generation is an interesting field of research, since progress in this area will directly affect the development of photonic quantum technologies, including quantum computing, simulation and sensing. Several methods have been sifted to increase the performances of entangled photon sources and the integrated optics approach represents a promising strategy. In particular, integrated waveguide sources represent a robust tool, thanks to their stability and the enhancement of nonlinear light-crystal interaction provided by waveguide field confinement. Here, we show the versatility of a hybrid approach, realizing an integrated optical source for the generation of entangled photon-pairs at telecom wavelength. The nonlinear active medium used is lithium niobate, while the routing and manipulation of the generated signal is performed in aluminum-borosilicate glass photonic circuits. The system is composed of three cascaded devices. First, a balanced directional coupler at the fundamental wavelength equally splits the pump in the lithium niobate waveguides, which generate single-photon pairs through type 0 spontaneous parametric down-conversion process. A third chip, encompassing directional couplers and waveplates, closes the interferometer and recombines the generated photons, thus giving access to different quantum states of light: path-entangled or polarization-entangled states. A thermal phase shifter, which controls the relative phase between the interferometer arms, gives an additional degree of freedom for engineering the output state of the presented photon pairs source. All these components are entirely fabricated by femtosecond laser micromachining, a direct and very versatile technique that allows to process different kind of materials and realize high quality optical circuits.